Review of iodine behavior from nuclear fuel dissolution to environmental release

Beck, Chelsie L.; Cervantes, Juan; Chiswell, Steven; Greaney, Allison T.; Johnson, Katherine R.; Levitskaia, Tatiana G.; Martin, Leigh R.; McDaniel, Gavin; Noble, Stephen; Rakos, Jason M.; Riley, Brian J.; Ritzmann, Andrew; Tingey, Joel M.

doi:10.1039/D4RA06494A

Title: Review of iodine behavior from nuclear fuel dissolution to environmental release

Journal Article · 04 November 2024 · RSC Advances

DOI: https://doi.org/10.1039/D4RA06494A · OSTI ID:2476750

^[1]; Cervantes, Juan ^[1]; Chiswell, Steven ^[2];

^[3];

^[1];

^[3]; McDaniel, Gavin ^[4]; Noble, Stephen ^[2]; Rakos, Jason M. ^[1];

^[1]; Ritzmann, Andrew ^[1]; Tingey, Joel M. ^[1]

Pacific Northwest National Laboratory, Richland, WA 99354, USA
Savannah River National Laboratory, Aiken, SC 29831, USA
Oak Ridge National Laboratory, Oak Ridge, TN 37830, USA
ENSCO, Vienna, VA 22180, USA

During nuclear fuel reprocessing, radioiodine, can be released.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States); Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Savannah River National Laboratory (SRNL), Aiken, SC (United States)

Sponsoring Organization:: USDOE; USDOE National Nuclear Security Administration (NNSA), Office of Defense Nuclear Nonproliferation; USDOE Office of Environmental Management (EM)

Grant/Contract Number:: 89303321CEM000080; AC05-00OR22725; AC05-76RL01830

OSTI ID:: 2476750

Report Number(s):: PNNL-SA--203176

Journal Information:: RSC Advances, Journal Name: RSC Advances Journal Issue: 48 Vol. 14; ISSN 2046-2069; ISSN RSCACL

Publisher:: Royal Society of Chemistry (RSC)Copyright Statement

Country of Publication:: United Kingdom

Language:: English

References (108)

Injection of iodine to the stratosphere Saiz‐Lopez, A.; Baidar, S.; Cuevas, C. A. Geophysical Research Letters, Vol. 42, Issue 16 https://doi.org/10.1002/2015GL064796	journal	August 2015
Inorganic reactions of iodine(+1) in acidic solutions Schmitz, Guy International Journal of Chemical Kinetics, Vol. 36, Issue 9 https://doi.org/10.1002/kin.20020	journal	June 2004
Radiolysis of solutions of iodine in tributyl phosphate Zagorets, P. A.; Raskina, Z. I.; Bulgakova, G. P. Soviet Atomic Energy, Vol. 32, Issue 5 https://doi.org/10.1007/BF01173228	journal	May 1972
The influence of iodine on the radiolysis of purex solvent Nowak, Z. Journal of Radioanalytical and Nuclear Chemistry Letters, Vol. 127, Issue 5 https://doi.org/10.1007/BF02166610	journal	July 1988
Particle and gas dry deposition: A review Sehmel, George A. Atmospheric Environment (1967), Vol. 14, Issue 9 https://doi.org/10.1016/0004-6981(80)90031-1	journal	January 1980
The chemical states of fission-product iodine emanating into a high temperature aqueous environment Castleman, A. W.; Tang, I. N.; Munkelwitz, H. R. Journal of Inorganic and Nuclear Chemistry, Vol. 30, Issue 1 https://doi.org/10.1016/0022-1902(68)80055-7	journal	January 1968
The reaction of iodine with concentrated nitric acid Mailen, J. C.; Tiffany, T. O. Journal of Inorganic and Nuclear Chemistry, Vol. 37, Issue 1 https://doi.org/10.1016/0022-1902(75)80139-4	journal	January 1975
The hydrolysis of iodine: Equilibria at high temperatures Palmer, Donald A.; Ramette, Richard W.; Mesmer, Robert E. Journal of Nuclear Materials, Vol. 130 https://doi.org/10.1016/0022-3115(85)90317-4	journal	February 1985
The chemical state of the fission products in oxide fuels Kleykamp, H. Journal of Nuclear Materials, Vol. 131, Issue 2-3, p. 221-246 https://doi.org/10.1016/0022-3115(85)90460-X	journal	April 1985
Fundamental aspects of defective nuclear fuel behaviour and fission product release Lewis, B. J. Journal of Nuclear Materials, Vol. 160, Issue 2-3 https://doi.org/10.1016/0022-3115(88)90049-9	journal	December 1988
Surface analysis using X-ray photoelectron spectroscopy of iodine deposits on 17% Cr/12% Ni and mild steel surfaces oxidised in gas mixtures Tyler, J. W. Journal of Nuclear Materials, Vol. 161, Issue 1 https://doi.org/10.1016/0022-3115(89)90463-7	journal	January 1989
Pellet-clad interaction (PCI) failures of zirconium alloy fuel cladding — A review Cox, B. Journal of Nuclear Materials, Vol. 172, Issue 3 https://doi.org/10.1016/0022-3115(90)90282-R	journal	August 1990
Dissolution study of spent PWR fuel: Dissolution behavior and chemical properties of insoluble residues Adachi, T.; Ohnuki, M.; Yoshida, N. Journal of Nuclear Materials, Vol. 174, Issue 1, p. 60-71 https://doi.org/10.1016/0022-3115(90)90421-I	journal	November 1990
The distribution and transformations of iodine in the environment Whitehead, D. C. Environment International, Vol. 10, Issue 4 https://doi.org/10.1016/0160-4120(84)90139-9	journal	January 1984
Iodine-129 in the environment of a nuclear fuel reprocessing plant: I. 127I and 127I contents of soils, food crops and animal products Robens, E.; Aumann, D. C. Journal of Environmental Radioactivity, Vol. 7, Issue 2 https://doi.org/10.1016/0265-931X(88)90005-7	journal	January 1988
Iodine-129 in the environment of a nuclear fuel reprocessing plant: III. Soil-to-plant concentration factors for iodine-129 and iodine-127 and their transfer factors to milk, eggs and pork Robens, E.; Hauschild, J.; Aumann, D. C. Journal of Environmental Radioactivity, Vol. 8, Issue 1 https://doi.org/10.1016/0265-931X(88)90013-6	journal	January 1988
Iodine-129 in the environment of a nuclear fuel reprocessing plant: II. Iodine-129 and iodine-127 contents of soils, forage plants and deer thyroids Robens, E.; Hauschild, J.; Aumann, D. C. Journal of Environmental Radioactivity, Vol. 7, Issue 3 https://doi.org/10.1016/0265-931X(88)90032-X	journal	January 1988
Iodine-129 in the Environment of a nuclear fuel reprocessing plant: VI. Comparison of measurements of 129I concentrations in soil and vegetation with predictions from a radiological assessment model Robens-Palavinskas, E.; Hauschild, J.; Aumann, D. C. Journal of Environmental Radioactivity, Vol. 10, Issue 1 https://doi.org/10.1016/0265-931X(89)90005-2	journal	January 1989
Iodine-129 in the environment of a nuclear fuel reprocessing plant: VII. Concentrations and chemical forms of 129I and 127I in the atmosphere Wershofen, H.; Aumann, D. C. Journal of Environmental Radioactivity, Vol. 10, Issue 2 https://doi.org/10.1016/0265-931X(89)90011-8	journal	January 1989
Iodine-129 in the environment of a nuclear fuel reprocessing plant: V. The transfer of 129I and 127I in the soil-pasture-cow-milk/meat pathway, as obtained by field measurements Hauschild, J.; Aumann, D. C. Journal of Environmental Radioactivity, Vol. 9, Issue 2 https://doi.org/10.1016/0265-931X(89)90021-0	journal	January 1989
Iodine-129 in the environment of a nuclear fuel reprocessing plant: IV. 129I and 127I in undisturbed surface soils Robens, E.; Hauschild, J.; Aumann, D. C. Journal of Environmental Radioactivity, Vol. 9, Issue 1 https://doi.org/10.1016/0265-931X(89)90035-0	journal	January 1989
Iodine-129 in the environment of a nuclear fuel reprocessing plant: VIII. Comparison of measured 129I concentrations in the atmosphere with those predicted by a radiological assessment code Wershofen, H.; Aumann, D. C.; Hübschmann, W. G. Journal of Environmental Radioactivity, Vol. 13, Issue 2 https://doi.org/10.1016/0265-931X(91)90052-H	journal	January 1991
Studies of iodine in nitric acid and of iodine adsorbed onto silver-impregnated silica Berry, Frank J.; Collins, Robert D.; Parish, R. V. Inorganica Chimica Acta, Vol. 126, Issue 1 https://doi.org/10.1016/S0020-1693(00)81251-7	journal	January 1987
Direct investigations of the kinetics of the reactions of CN radicals with N atoms and 3CH2 radicals with NO Atakan, Burak; Kocis, Daniel; Wolfrum, Jürgen Symposium (International) on Combustion, Vol. 24, Issue 1 https://doi.org/10.1016/S0082-0784(06)80085-8	journal	January 1992
LIRIC 3.2 an updated model for iodine behaviour in the presence of organic impurities Wren, J. C.; Ball, J. M. Radiation Physics and Chemistry, Vol. 60, Issue 6 https://doi.org/10.1016/S0969-806X(00)00385-6	journal	March 2001
Iodine concentration and availability in atmospheric aerosol Baker, A. R.; Thompson, D.; Campos, M. L. A. M. Atmospheric Environment, Vol. 34, Issue 25 https://doi.org/10.1016/S1352-2310(00)00208-9	journal	July 2000
Neutronic analysis for accident tolerant cladding candidates in CANDU-6 reactors Naceur, A.; Marleau, G. Annals of Nuclear Energy, Vol. 113 https://doi.org/10.1016/j.anucene.2017.11.016	journal	March 2018
Iodine and human health, the role of environmental geochemistry and diet, a review Fuge, Ron; Johnson, Christopher C. Applied Geochemistry, Vol. 63 https://doi.org/10.1016/j.apgeochem.2015.09.013	journal	December 2015
Development of the SAPRC-07 chemical mechanism Carter, William P. L. Atmospheric Environment, Vol. 44, Issue 40 https://doi.org/10.1016/j.atmosenv.2010.01.026	journal	December 2010
Atmospheric iodine, selenium and caesium depositions in France: I. Spatial and seasonal variations Roulier, Marine; Bueno, Maïté; Coppin, Frédéric Chemosphere, Vol. 273 https://doi.org/10.1016/j.chemosphere.2020.128971	journal	June 2021
Thermodynamic properties of organic iodine compounds Richard, Laurent; Gaona, Xavier Geochimica et Cosmochimica Acta, Vol. 75, Issue 22 https://doi.org/10.1016/j.gca.2011.07.030	journal	November 2011
Measurement and modelling of gaseous elemental iodine (I2) dry deposition velocity on grass in the environment Telly Bah, Oumar; Hebert, Didier; Connan, Olivier Journal of Environmental Radioactivity, Vol. 219 https://doi.org/10.1016/j.jenvrad.2020.106253	journal	August 2020
Performance of radio-iodine discharge control methods of nuclear reprocessing plants Umadevi, K.; Mandal, D. Journal of Environmental Radioactivity, Vol. 234 https://doi.org/10.1016/j.jenvrad.2021.106623	journal	August 2021
Porous organic materials for iodine adsorption Kurisingal, Jintu Francis; Yun, Hongryeol; Hong, Chang Seop Journal of Hazardous Materials, Vol. 458 https://doi.org/10.1016/j.jhazmat.2023.131835	journal	September 2023
Reactions between reactive metals and iodine in aqueous solutions Glänneskog, Henrik; Liljenzin, Jan-Olov; Sihver, Lembit Journal of Nuclear Materials, Vol. 348, Issue 1-2 https://doi.org/10.1016/j.jnucmat.2005.09.004	journal	January 2006
Thermal diffusion of iodine in UO2 and UO2+x Saidy, Madiba; Hocking, William H.; Mouris, Jozef F. Journal of Nuclear Materials, Vol. 372, Issue 2-3 https://doi.org/10.1016/j.jnucmat.2007.03.272	journal	January 2008
Fuel clad chemical interactions in fast reactor MOX fuels Viswanathan, R. Journal of Nuclear Materials, Vol. 444, Issue 1-3 https://doi.org/10.1016/j.jnucmat.2013.09.044	journal	January 2014
Materials and processes for the effective capture and immobilization of radioiodine: A review Riley, Brian J.; Vienna, John D.; Strachan, Denis M. Journal of Nuclear Materials, Vol. 470 https://doi.org/10.1016/j.jnucmat.2015.11.038	journal	March 2016
Sequestration of radioactive iodine in silver-palladium phases in commercial spent nuclear fuel Buck, Edgar C.; Mausolf, Edward J.; McNamara, Bruce K. Journal of Nuclear Materials, Vol. 482 https://doi.org/10.1016/j.jnucmat.2016.10.029	journal	December 2016
Molecular iodine interactions with metal substrates: Towards the understanding of iodine interactions in the environment following a nuclear accident Beck, Chelsie L.; Riley, Brian J.; Chong, Saehwa Journal of Nuclear Materials, Vol. 546 https://doi.org/10.1016/j.jnucmat.2020.152771	journal	April 2021
Adsorption of iodine on metal coupons in humid and dry environments Beck, Chelsie L.; Smith, Nathaniel P.; Riley, Brian J. Journal of Nuclear Materials, Vol. 556 https://doi.org/10.1016/j.jnucmat.2021.153204	journal	December 2021
Solid sorbents for gaseous iodine capture and their conversion into stable waste forms Pénélope, R.; Campayo, L.; Fournier, M. Journal of Nuclear Materials, Vol. 563 https://doi.org/10.1016/j.jnucmat.2022.153635	journal	May 2022
The PSIodine Code: A computer program to model experimental data on iodine and other species in irradiated CsI solutions sparged with argon, air, or nitrous oxide Cripps, R. C.; Güntay, S.; Jäckel, B. Nuclear Engineering and Design, Vol. 241, Issue 10 https://doi.org/10.1016/j.nucengdes.2011.08.010	journal	October 2011
Molten salt reactor waste and effluent management strategies: A review Riley, Brian J.; McFarlane, Joanna; DelCul, Guillermo D. Nuclear Engineering and Design, Vol. 345 https://doi.org/10.1016/j.nucengdes.2019.02.002	journal	April 2019
Review of molten salt reactor off-gas management considerations Andrews, Hunter B.; McFarlane, Joanna; Chapel, A. Shay Nuclear Engineering and Design, Vol. 385 https://doi.org/10.1016/j.nucengdes.2021.111529	journal	December 2021
Dry deposition of gaseous radioiodine and particulate radiocaesium onto leafy vegetables Tschiersch, Jochen; Shinonaga, Taeko; Heuberger, Heidi Science of The Total Environment, Vol. 407, Issue 21 https://doi.org/10.1016/j.scitotenv.2009.06.025	journal	October 2009
An overview of Fukushima radionuclides measured in the northern hemisphere Thakur, P.; Ballard, S.; Nelson, R. Science of The Total Environment, Vol. 458-460 https://doi.org/10.1016/j.scitotenv.2013.03.105	journal	August 2013
Iodine immobilization by materials through sorption and redox-driven processes: A literature review Moore, Robert C.; Pearce, Carolyn I.; Morad, Joseph W. Science of The Total Environment, Vol. 716 https://doi.org/10.1016/j.scitotenv.2019.06.166	journal	May 2020
Role of Iodine-Assisted Aerosol Particle Formation in Antarctica Xavier, Carlton; de jonge, Robin Wollesen; Jokinen, Tuija Environmental Science & Technology, Vol. 58, Issue 17 https://doi.org/10.1021/acs.est.3c09103	journal	April 2024
Atmospheric Iodine (¹²⁷I and ¹²⁹I) Record in Spruce Tree Rings in the Northeast Qinghai-Tibet Plateau Zhao, Xue; Hou, Xiaolin; Zhou, Weijian Environmental Science & Technology, Vol. 53, Issue 15 https://doi.org/10.1021/acs.est.9b01160	journal	July 2019
Molecular Iodine Interactions with Fe, Ni, Cr, and Stainless Steel Alloys Beck, Chelsie L.; Riley, Brian J.; Chong, Saehwa Industrial & Engineering Chemistry Research, Vol. 60, Issue 6 https://doi.org/10.1021/acs.iecr.0c04590	journal	February 2021
Atmospheric Chemistry of Iodine Saiz-Lopez, Alfonso; Plane, John M. C.; Baker, Alex R. Chemical Reviews, Vol. 112, Issue 3 https://doi.org/10.1021/cr200029u	journal	October 2011
Transfer of ¹³¹ I from Fukushima to the Vegetation and Milk in France Parache, V.; Pourcelot, L.; Roussel-Debet, S. Environmental Science & Technology, Vol. 45, Issue 23 https://doi.org/10.1021/es202242g	journal	December 2011
¹²⁹I Dispersion in Argentina: Concentrations in Fresh and Marine Water and Deposition Fluences in Patagonia Negri, Agustín E.; Fernández Niello, Jorge O.; Wallner, Anton Environmental Science & Technology, Vol. 47, Issue 17 https://doi.org/10.1021/es400610h	journal	August 2013
Time Series of¹²⁹I and¹²⁷I Speciation in Precipitation from Denmark Hou, Xiaolin; Aldahan, Ala; Nielsen, Sven P. Environmental Science & Technology, Vol. 43, Issue 17 https://doi.org/10.1021/es9012678	journal	August 2009
Atmospheric Dispersal of ¹²⁹ Iodine from Nuclear Fuel Reprocessing Facilities Moran, Jean E.; Oktay, Sarah; Santschi, Peter H. Environmental Science & Technology, Vol. 33, Issue 15 https://doi.org/10.1021/es9900050	journal	August 1999
Reaction Rate Constants (295 K) for 3CH2 with H2S, SO2, and NO2: Upper Bounds for Rate Constants with Less Reactive Partners Darwin, David C.; Moore, C. Bradley The Journal of Physical Chemistry, Vol. 99, Issue 36 https://doi.org/10.1021/j100036a022	journal	September 1995
Solubility and decomposition kinetics of nitrous acid in aqueous solution Park, Jong Yoon; Lee, Yin Nan The Journal of Physical Chemistry, Vol. 92, Issue 22 https://doi.org/10.1021/j100333a025	journal	November 1988
Molecular Complexes and their Spectra. XI. The Interaction of Iodide with Tri-n-Butyl Phosphate¹ Tsubomura, Hiroshi; Kliegman, Jonathan M. Journal of the American Chemical Society, Vol. 82, Issue 6 https://doi.org/10.1021/ja01491a010	journal	March 1960
Reversible Iodine Capture by Nonporous Pillar[6]arene Crystals Jie, Kecheng; Zhou, Yujuan; Li, Errui Journal of the American Chemical Society, Vol. 139, Issue 43 https://doi.org/10.1021/jacs.7b09850	journal	October 2017
Kinetics of the Reactions of n-Alkyl (C₂H₅, n-C₃H₇, and n-C₄H₉) Radicals with CH₃ Knyazev, Vadim D.; Slagle, Irene R. The Journal of Physical Chemistry A, Vol. 105, Issue 26 https://doi.org/10.1021/jp010878s	journal	June 2001
Effect of Molecular Hydrogen on Hydrogen Peroxide in Water Radiolysis Pastina, Barbara; LaVerne, Jay A. The Journal of Physical Chemistry A, Vol. 105, Issue 40 https://doi.org/10.1021/jp012245j	journal	October 2001
Iodine Chemistry and its Role in Halogen Activation and Ozone Loss in the Marine Boundary Layer: A Model Study Vogt, Rainer; Sander, Rolf; von Glasow, Roland Journal of Atmospheric Chemistry, Vol. 32, Issue 3, p. 375-395 https://doi.org/10.1023/A:1006179901037	journal	March 1999
Solubility of Iodine in the System Water-Nitric Acid Lutsyk, A. I.; Suikov, S. Yu.; Chuprina, V. S. Russian Journal of Applied Chemistry, Vol. 77, Issue 7 https://doi.org/10.1023/B:RJAC.0000044174.73998.82	journal	July 2004
A modeling study of iodine chemistry in the marine boundary layer McFiggans, Gordon; Plane, John M. C.; Allan, Beverley J. Journal of Geophysical Research: Atmospheres, Vol. 105, Issue D11 https://doi.org/10.1029/1999JD901187	journal	June 2000
Iodine speciation and deposition fluxes from the marine atmosphere Baker, A. R.; Tunnicliffe, C.; Jickells, T. D. Journal of Geophysical Research: Atmospheres, Vol. 106, Issue D22 https://doi.org/10.1029/2000JD000004	journal	November 2001
What is the effect of cloud inhomogeneities on actinic fluxes and chemical species concentrations? Bouet, Christel; Szczap, Frédéric; Leriche, Maud Geophysical Research Letters, Vol. 33, Issue 1 https://doi.org/10.1029/2005GL024727	journal	January 2006
A large terrestrial source of methyl iodide Sive, Barkley C.; Varner, Ruth K.; Mao, Huiting Geophysical Research Letters, Vol. 34, Issue 17 https://doi.org/10.1029/2007GL030528	journal	September 2007
Spatial and Temporal Variability of Iodine in Aerosol Gómez Martín, Juan Carlos; Saiz‐Lopez, Alfonso; Cuevas, Carlos A. Journal of Geophysical Research: Atmospheres, Vol. 126, Issue 9 https://doi.org/10.1029/2020JD034410	journal	May 2021
Role of Iodine Recycling on Sea‐Salt Aerosols in the Global Marine Boundary Layer Li, Qinyi; Tham, Yee Jun; Fernandez, Rafael P. Geophysical Research Letters, Vol. 49, Issue 6 https://doi.org/10.1029/2021GL097567	journal	March 2022
On the Speciation of Iodine in Marine Aerosol Gómez Martín, Juan Carlos; Saiz‐Lopez, Alfonso; Cuevas, Carlos A. Journal of Geophysical Research: Atmospheres, Vol. 127, Issue 4 https://doi.org/10.1029/2021JD036081	journal	February 2022
Temperature dependence of UV absorption cross sections and atmospheric implications of several alkyl iodides Roehl, Coleen M.; Burkholder, James B.; Moortgat, Geert K. Journal of Geophysical Research: Atmospheres, Vol. 102, Issue D11 https://doi.org/10.1029/97JD00530	journal	June 1997
Atmospheric iodine levels influenced by sea surface emissions of inorganic iodine Carpenter, Lucy J.; MacDonald, Samantha M.; Shaw, Marvin D. Nature Geoscience, Vol. 6, Issue 2 https://doi.org/10.1038/ngeo1687	journal	January 2013
Rapid increase in atmospheric iodine levels in the North Atlantic since the mid-20th century Cuevas, Carlos A.; Maffezzoli, Niccolò; Corella, Juan Pablo Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-03756-1	journal	April 2018
Porous sorbents for the capture of radioactive iodine compounds: a review Huve, Joffrey; Ryzhikov, Andrey; Nouali, Habiba RSC Advances, Vol. 8, Issue 51 https://doi.org/10.1039/C8RA04775H	journal	January 2018
CCCXCVI.—The salting-out effect. The influence of electrolytes on the solubility of iodine in water Carter, John Stanley J. Chem. Soc., Trans., Vol. 127, Issue 0 https://doi.org/10.1039/CT9252702861	journal	January 1925
Adsorption-based capture of iodine and organic iodides: status and challenges Pan, Tingting; Yang, Kaijie; Dong, Xinglong Journal of Materials Chemistry A, Vol. 11, Issue 11 https://doi.org/10.1039/D2TA09448G	journal	January 2023
γ-Radiolysis study of concentrated nitric acid solutions Jiang, Pei-Yun; Nagaishi, Ryuji; Yotsuyanagi, Tadasu J. Chem. Soc., Faraday Trans., Vol. 90, Issue 1 https://doi.org/10.1039/FT9949000093	journal	January 1994
Formation of organic nitro-compounds in flowing H2O2+ NO2+ N2+ organic vapour systems. Part 3.—Effects of O2 addition on H2O2+ NO2+ N2+ alkane systems Baulch, Donald L.; Campbell, Ian M.; Chappel, Jonathan M. Journal of the Chemical Society, Faraday Transactions 1: Physical Chemistry in Condensed Phases, Vol. 80, Issue 3 https://doi.org/10.1039/f19848000617	journal	January 1984
Dissolution of uranium dioxide in nitric acid media: what do we know? Marc, Philippe; Magnaldo, Alastair; Vaudano, Aimé EPJ Nuclear Sciences & Technologies, Vol. 3 https://doi.org/10.1051/epjn/2017005	journal	January 2017
Fundamental and applied aspects of the chemistry of radioactive iodine in gas and aqueous media Kulyukhin, Sergei A. Russian Chemical Reviews, Vol. 81, Issue 10 https://doi.org/10.1070/RC2012v081n10ABEH004269	journal	October 2012
Alpine ice evidence of a three-fold increase in atmospheric iodine deposition since 1950 in Europe due to increasing oceanic emissions Legrand, Michel; McConnell, Joseph R.; Preunkert, Susanne Proceedings of the National Academy of Sciences, Vol. 115, Issue 48 https://doi.org/10.1073/pnas.1809867115	journal	November 2018
Potential for the Use of Hydrochloric Acid in Fission Reactor Fuel Recycle Mailen, J. C.; Bell, J. T. Separation Science and Technology, Vol. 22, Issue 2-3 https://doi.org/10.1080/01496398708068957	journal	February 1987
Behavior of Iodine-131 in Dissolution of Irradiated Uranium Dioxide Sakurai, Tsutomu; Izumo, Mishiroku; Takahashi, Akira Journal of Nuclear Science and Technology, Vol. 24, Issue 11 https://doi.org/10.1080/18811248.1987.9733524	journal	November 1987
Thermochemical and Experimental Considerations of NO_xComposition and Iodine Species in the Dissolution of Spent PWR-Fuel Specimens Sakurai, Tsutomu; Takahashi, Akira; Ishikawa, Niroh Journal of Nuclear Science and Technology, Vol. 30, Issue 6 https://doi.org/10.1080/18811248.1993.9734515	journal	June 1993
Interaction of Iodine with an Extractant of 30% TBP/70% n -Dodecane Sakurai, Tsutomu; Takahashi, Akira; Ishikawa, Niroh Journal of Nuclear Science and Technology, Vol. 32, Issue 7 https://doi.org/10.1080/18811248.1995.9731757	journal	July 1995
Deposition Velocity of Gaseous Organic Iodine from the Atmosphere to Rice Plants Muramatsu, Yasuyuki; Uchida, Shigeo; Sumiya, Misako Health Physics, Vol. 71, Issue 5 https://doi.org/10.1097/00004032-199611000-00018	journal	November 1996
Marine iodine emissions in a changing world Carpenter, Lucy J.; Chance, Rosie J.; Sherwen, Tomás Proceedings of the Royal Society A: Mathematical, Physical and Engineering Sciences, Vol. 477, Issue 2247 https://doi.org/10.1098/rspa.2020.0824	journal	March 2021
Ozone depletion due to dust release of iodine in the free troposphere Koenig, Theodore K.; Volkamer, Rainer; Apel, Eric C. Science Advances, Vol. 7, Issue 52 https://doi.org/10.1126/sciadv.abj6544	journal	December 2021
Role of iodine oxoacids in atmospheric aerosol nucleation He, Xu-Cheng; Tham, Yee Jun; Dada, Lubna Science, Vol. 371, Issue 6529 https://doi.org/10.1126/science.abe0298	journal	February 2021
Chemistry of radioactive iodine in aqueous media: Basic and applied aspects Kulyukhin, S. A.; Kamenskaya, A. N.; Konovalova, N. A. Radiochemistry, Vol. 53, Issue 2 https://doi.org/10.1134/S1066362211020020	journal	April 2011
Leaching of¹³⁷Cs,¹³⁴Cs, and¹²⁹I from Irradiated UO₂Fuel Johnson, L. H.; Burns, K. I.; Joling, H. H. Nuclear Technology, Vol. 63, Issue 3 https://doi.org/10.13182/NT83-A33273	journal	December 1983
The Behavior of Iodine in a Simulated Spent-Fuel Solution Sakurai, Tsutomu; Takahashi, Akira; Ishikawa, Niro Nuclear Technology, Vol. 85, Issue 2 https://doi.org/10.13182/NT89-A34241	journal	May 1989
The Interaction of Iodine with Insoluble Residue in the Dissolution of Simulated Spent-Fuel Pellets Sakurai, Tsutomu; Takahashi, Akira; Ishikawa, Niroh Nuclear Technology, Vol. 94, Issue 1 https://doi.org/10.13182/NT91-A16225	journal	April 1991
The Iodine Species and Their Behavior in the Dissolution of Spent-Fuel Specimens Sakurai, Tsutomu; Takahashi, Akira; Ishikawa, Niroh Nuclear Technology, Vol. 99, Issue 1 https://doi.org/10.13182/NT92-A34704	journal	July 1992
Influence of NO _x and HNO ₂ on Iodine Quantity in Spent-Fuel Solutions Sakurai, Tsutomu; Takahashi, Akira; Ishikawa, Niroh Nuclear Technology, Vol. 116, Issue 3 https://doi.org/10.13182/NT96-A35287	journal	December 1996
Radioiodine in Nitric Acid Lieser, Κ. Η.; Georgoulas, P.; Hoffmann, P. ract, Vol. 48, Issue 3-4 https://doi.org/10.1524/ract.1989.48.34.193	journal	September 1989
Two-Step Procedure for the Iodine Removal from Nuclear Fuel Solutions Boukis, N.; Henrich, E. ract, Vol. 55, Issue 1 https://doi.org/10.1524/ract.1991.55.1.37	journal	July 1991
Abatement of radioiodine in aqueous reprocessing off-gas Greaney, Allison T.; Ngelale, Randy O.; Bruffey, Stephanie H. Frontiers in Chemistry, Vol. 10 https://doi.org/10.3389/fchem.2022.1078668	journal	January 2023
Soluble Iodine Speciation in Marine Aerosols Across the Indian and Pacific Ocean Basins Droste, Elise S.; Baker, Alex R.; Yodle, Chan Frontiers in Marine Science, Vol. 8 https://doi.org/10.3389/fmars.2021.788105	journal	December 2021
Review on the physical chemistry of iodine transformations in the oceans Luther, George W. Frontiers in Marine Science, Vol. 10 https://doi.org/10.3389/fmars.2023.1085618	journal	February 2023
Transport of iodine from atmosphere to ground Chamberlain, A. C.; Chadwick, R. C. Tellus A: Dynamic Meteorology and Oceanography, Vol. 18, Issue 2-3 https://doi.org/10.3402/tellusa.v18i2-3.9676	journal	January 1966
Bromine and iodine chemistry in a global chemistry-climate model: description and evaluation of very short-lived oceanic sources Ordóñez, C.; Lamarque, J. -F.; Tilmes, S. Atmospheric Chemistry and Physics, Vol. 12, Issue 3 https://doi.org/10.5194/acp-12-1423-2012	journal	January 2012
Iodine's impact on tropospheric oxidants: a global model study in GEOS-Chem Sherwen, T.; Evans, M. J.; Carpenter, L. J. Atmospheric Chemistry and Physics, Vol. 16, Issue 2 https://doi.org/10.5194/acp-16-1161-2016	journal	January 2016
The UV-visible absorption cross-sections of IONO₂ Mössinger, J. C.; Rowley, D. M.; Cox, R. A. Atmospheric Chemistry and Physics, Vol. 2, Issue 3 https://doi.org/10.5194/acp-2-227-2002	journal	September 2002
Absolute absorption cross-section and photolysis rate of I₂ Saiz-Lopez, A.; Saunders, R. W.; Joseph, D. M. Atmospheric Chemistry and Physics, Vol. 4, Issue 5 https://doi.org/10.5194/acp-4-1443-2004	journal	January 2004
Evaluated kinetic and photochemical data for atmospheric chemistry: Volume III – gas phase reactions of inorganic halogens Atkinson, R.; Baulch, D. L.; Cox, R. A. Atmospheric Chemistry and Physics, Vol. 7, Issue 4 https://doi.org/10.5194/acp-7-981-2007	journal	January 2007
Influence of the acidity of the Iodous acid solution system on the kinetics of the disproportionation reaction Marković, Smiljana Bulletin of Natural Sciences Research, Vol. 11, Issue 2 https://doi.org/10.5937/bnsr11-29311	journal	January 2021

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