A Review of Online Monitoring within Used Nuclear Fuel Recycling Processes

Tse, Poki; Bessen, Nathan P.; Hall, Gabriel B.; Seiner, Brienne N.; Lumetta, Gregg J.; Bryan, Samuel A.; Lines, Amanda M.

doi:10.1080/07366299.2024.2395917

Title: A Review of Online Monitoring within Used Nuclear Fuel Recycling Processes

Journal Article · 30 September 2024 · Solvent Extraction and Ion Exchange

DOI: https://doi.org/10.1080/07366299.2024.2395917 · OSTI ID:2475143

^[1];

^[1]; Lines, Amanda M. ^[1]

Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)

The processing of used nuclear fuels and related materials is often complex and variable. The ability to quickly optimize conditions to the material being processed can aid in increasing efficiency and safety, but requires very quick determination of the conditions present in the feedstock, the process, and the product. Furthermore, accurate quantification of materials such as enriched uranium and plutonium aids in maintaining material accountancy and avoiding nuclear proliferation risks. Traditional analytical methods require process samples to be collected and analyzed in a laboratory, which often takes days to weeks. Online monitoring is suitable for collecting this information nearly instantaneously, enabling much faster optimization of the process or detection of material diversion. Online monitoring is also beneficial as it is typically based on robust and nondestructive analytical methods, so no material is removed as samples. This review examines online monitoring relevant to used nuclear fuel processing for the determination of both chemical and physical parameters. The chemical parameters include quantities such as concentration, isotopic composition, and speciation. These values are often well suited to spectroscopic or spectrometric measurements as they are fast, nondestructive, and easily implemented in an online manner. Physical quantities are often more varied and include temperature, pressure, tank fill levels, and others. Due to the specificity of these quantities, specialized instrumentation is often used. However, this instrumentation is often amendable to online monitoring.

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Research Organization:: Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA)

Grant/Contract Number:: AC05-76RL01830

OSTI ID:: 2475143

Report Number(s):: PNNL-SA--197799

Journal Information:: Solvent Extraction and Ion Exchange, Journal Name: Solvent Extraction and Ion Exchange Journal Issue: 5 Vol. 42; ISSN 0736-6299

Publisher:: Taylor and FrancisCopyright Statement

Country of Publication:: United States

Language:: English

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11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS
Used nuclear fuel reprocessing
chemometric analysis
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Title: A Review of Online Monitoring within Used Nuclear Fuel Recycling Processes

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