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Title: Proximity-Induced Superconductivity in a 2D Kondo Lattice of an f-Electron-Based Surface Alloy

Journal Article · · Nano Letters
ORCiD logo [1];  [2];  [3]
  1. University of Hamburg (Germany); Surface and Interface Science Laboratory, Saitama (Japan)
  2. University of Illinois at Chicago, IL (United States)
  3. University of Hamburg (Germany)

Realizing hybrids of low-dimensional Kondo lattices and superconducting substrates leads to fascinating platforms for studying the exciting physics of strongly correlated electron systems with induced superconducting pairing. Here, we report a scanning tunneling microscopy and spectroscopy study of a new type of two-dimensional (2D) La–Ce alloy grown epitaxially on a superconducting Re(0001) substrate. We observe the characteristic spectroscopic signature of a hybridization gap evidencing the coherent spin screening in the 2D Kondo lattice realized by the ultrathin La–Ce alloy film on normal conducting Re(0001). Upon lowering the temperature below the critical temperature of rhenium, a superconducting gap is induced exhibiting an energy asymmetry of the coherence peaks that arises from the interaction of residual unscreened magnetic moments with the superconducting substrate. A positive correlation between the Kondo hybridization gap and the asymmetry of the coherence peaks is found.

Research Organization:
University of Hamburg (Germany)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
FG02-05ER46225
OSTI ID:
2474305
Journal Information:
Nano Letters, Journal Name: Nano Letters Journal Issue: 44 Vol. 24; ISSN 1530-6984
Publisher:
American Chemical SocietyCopyright Statement
Country of Publication:
United States
Language:
English

References (48)

Heavy Fermions: Electrons at the Edge of Magnetism book December 2007
Pair-breaking effects in the superconducting Kondo alloy LaCe journal August 1971
Scanning tunneling microscopy study of Fe, Co and Cr growth on Re(0001) journal December 2014
Building Complex Kondo Impurities by Manipulating Entangled Spin Chains journal October 2017
Molecular Kondo Chain journal May 2012
Imaging the Fano lattice to ‘hidden order’ transition in URu2Si2 journal June 2010
Visualizing heavy fermions emerging in a quantum critical Kondo lattice journal June 2012
Coherent long-range magnetic bound states in a superconductor journal October 2015
Quantum engineered Kondo lattices journal December 2019
Perfect Andreev reflection due to the Klein paradox in a topological superconducting state journal June 2019
Quantum phases driven by strong correlations journal December 2020
Visualizing the formation of the Kondo lattice and the hidden order in URu2Si2 journal May 2010
Hybridization gap and Fano resonance in SmB 6 journal March 2014
Unconventional superconductivity journal April 2017
On the solution of the Coqblin-Schreiffer Hamiltonian by the large-N expansion technique journal June 1983
From Kondo lattices to Kondo superlattices journal June 2016
Theory of scanning tunneling spectroscopy: from Kondo impurities to heavy fermion materials journal November 2016
Spectroscopic manifestations of the Kondo effect on single adatoms journal December 2008
Coverage-dependent self-organization: from individual adatoms to adatom superlattices journal February 2004
Structural and electrical characterization of the monolayer Kondo-lattice compound CePt6/Pt(111) journal October 2021
New approach to the mixed-valence problem journal March 1984
Superexchange mechanism and d -wave superconductivity journal September 1988
Temperature-Dependent Pair Breaking inLaCeandLaGd journal August 1972
LaAu2and CeAu2surface intermetallic compounds grown by high-temperature deposition on Au(111) journal September 2013
Atomically resolved magnetic structure of a Gd-Au surface alloy journal May 2019
Electron Cotunneling into a Kondo Lattice journal November 2009
Differential Conductance and Quantum Interference in Kondo Systems journal May 2010
Tunneling into Clean Heavy Fermion Compounds: Origin of the Fano Line Shape journal December 2010
Evolution of Kondo Resonance from a Single Impurity Molecule to the Two-Dimensional Lattice journal May 2011
Kondo Scattering Observed at a Single Magnetic Impurity journal March 1998
Creation of an Atomic Superlattice by Immersing Metallic Adatoms in a Two-Dimensional Electron Sea journal January 2004
Scanning-Tunneling Spectroscopy of Surface-State Electrons Scattered by a Slightly Disordered Two-Dimensional Dilute “Solid”: Ce on Ag(111) journal September 2004
Observation of the Superconducting Proximity Effect in the Surface State of SmB 6 Thin Films journal August 2016
Mixed-valence compounds journal April 1976
Heavy-fermion systems journal October 1984
Review of techniques in the large- N expansion for dilute magnetic alloys journal October 1987
Correlated electrons in high-temperature superconductors journal July 1994
Impurity-induced states in conventional and unconventional superconductors journal May 2006
Fermi-liquid instabilities at magnetic quantum phase transitions journal August 2007
Superconducting phases of f -electron compounds journal November 2009
Atomic-scale interface engineering of Majorana edge modes in a 2D magnet-superconductor hybrid system journal July 2019
Tuning the Dimensionality of the Heavy Fermion Compound CeIn3 journal February 2010
The Lowdown on Heavy Fermions journal February 2010
Tunneling into a Single Magnetic Atom: Spectroscopic Evidence of the Kondo Resonance journal April 1998
Resistance Minimum in Dilute Magnetic Alloys journal July 1964
Classical Spins in Superconductors journal September 1968
The Effects of Impurities on Superconductors with Kondo Effect journal June 1977
Bound State in Superconductors with Paramagnetic Impurities journal January 1965