Aerosol Vertical Turbulent Mass Flux Retrievals Through Novel Remote Sensing Algorithm

Journal Article · 24 October 2024 · Journal of Geophysical Research. Atmospheres

DOI: https://doi.org/10.1029/2023JD040322 · OSTI ID:2474254

Rasheeda Satheesh, Ajmal ^[1]; Petters, Markus D.  ^[2]; Meskhidze, Nicholas  ^[1]

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1. Department of Marine, Earth, and Atmospheric Sciences North Carolina State University Raleigh NC USA
2. Department of Marine, Earth, and Atmospheric Sciences North Carolina State University Raleigh NC USA, Now at the Department of Chemical and Environmental Engineering University of California Riverside CA USA

Abstract Integrated measurements of aerosol, radiation, cloud, and turbulent transport in the planetary boundary layer (PBL) are essential for understanding and modeling climate and air quality. Here, we developed a new technique for the identification of convective turbulent regions and deriving the vertical distribution of aerosol turbulent mass fluxes within PBL. The algorithm uses retrievals from coherent Doppler lidars and a high spectral resolution lidar. The technique was applied to study particle mass fluxes over 2 months (November–December 2020) during the campaign conducted at the DOE Atmospheric Radiation Measurement Southern Great Plains (SGP) site in Lamont, Oklahoma. The algorithm developed here is capable of continuously deriving vertically resolved (curtains) aerosol mass fluxes. Our data analysis shows that at the site, the 30‐min averaged fluxes at 135 m above the surface were mainly positive (upward) at ∼1 μg m ⁻²  s ⁻¹ , suggesting that the surface is the primary source of the particle mass supplied to the boundary layer at the SGP site. Analyses of the individual case studies have revealed that not all the derived fluxes can be linked to surface emissions. Both positive and negative values in a range of ±5 μg m ⁻²  s ⁻¹ can be caused by convective thermals interacting between the residual layer and the mixed layer and by rotation of the horizontal wind with the height. Large erroneous negative fluxes can also be caused by drizzling/precipitating clouds. We anticipate that the application of the current technique will lead to a more realistic representation of aerosol mass budgets and bidirectional mixing rates.

• Sponsoring Organization: USDOE
• OSTI ID: 2474254
• Journal Information: Journal of Geophysical Research. Atmospheres, Journal Name: Journal of Geophysical Research. Atmospheres Journal Issue: 20 Vol. 129; ISSN 2169-897X
• Publisher: American Geophysical Union (AGU)Copyright Statement
• Country of Publication: United States
• Language: English