Characterization of spent nuclear fuel canister surface roughness using surface replicating molds

Journal Article · 01 October 2024 · Scientific Reports

DOI: https://doi.org/10.1038/s41598-024-71992-1 · OSTI ID:2472762

Nation, Brendan L. ^[1]; Faubel, Jessica L. ^[1]; Vice, Gregory Thad ^[1]; Ohlhausen, James A. ^[1]; Durbin, Samuel ^[1]; Bryan, Charles R. ^[1]; Knight, Andrew William ^[1]

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1. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)

In this study we present a replication method to determine surface roughness and to identify surface features when a sample cannot be directly analyzed by conventional techniques. As a demonstration, this method was applied to an unused spent nuclear fuel dry storage canister to determine variation across different surface features. In this study, an initial material down-selection was performed to determine the best molding agent and determined that non-modified Polytek PlatSil23-75 provided the most accurate representation of the surface while providing good usability. Other materials that were considered include Polygel Brush-On 35 polyurethane rubber (with and without Pol-ease 2300 release agent), Polytek PlatSil73-25 silicone rubber (with and without PlatThix thickening agent and Pol-ease 2300 release agent), and Express STD vinylpolysiloxane impression putty. The ability of PlatSil73-25 to create an accurate surface replica was evaluated by creating surface molds of several locations on surface roughness standards representing ISO grade surfaces N₃, N₅, N₇, and N₈. Overall, the molds were able to accurately reproduce the expected roughness average (R_a) values, but systematically over-estimated the peak-valley maximum roughness (R_z) values. Using a 3D printed sample cell, several locations across the stainless steel spent nuclear fuel canister were sampled to determine the surface roughness. These measurements provided information regarding variability in normal surface roughness across the canister as well as a detailed evaluation on specific surface features (e.g., welds, grind marks, etc.). The results of these measurements can support development of dry storage canister ageing management programs, as surface roughness is an important factor for surface dust deposition and accumulation. This method can be applied more broadly to different surfaces beyond stainless steel to provide rapid, accurate surface replications for analytical evaluation by profilometry.

• Research Organization: Sandia National Laboratories (SNL-NM), Albuquerque, NM (United States)
• Sponsoring Organization: USDOE Office of Nuclear Energy (NE), Office of Spent Fuel and Waste Disposition; USDOE National Nuclear Security Administration (NNSA)
• Grant/Contract Number: NA0003525
• OSTI ID: 2472762
• Report Number(s): SAND--2024-13941J
• Journal Information: Scientific Reports, Journal Name: Scientific Reports Journal Issue: 1 Vol. 14; ISSN 2045-2322
• Publisher: Nature Publishing GroupCopyright Statement
• Country of Publication: United States
• Language: English