Large anomalous Hall conductivity induced by spin chirality fluctuation in an ultraclean frustrated antiferromagnet PdCrO2

Jeon, Hoseong; Seo, Hyeongwoo; Seo, Junho; Kim, Yong Hyun; Choi, Eun Sang; Jo, Younjung; Lee, Ho Nyung; Ok, Jong Mok; Kim, Jun Sung

doi:10.1038/s42005-024-01652-3

Title: Large anomalous Hall conductivity induced by spin chirality fluctuation in an ultraclean frustrated antiferromagnet PdCrO₂

Journal Article · 21 May 2024 · Communications Physics

DOI: https://doi.org/10.1038/s42005-024-01652-3 · OSTI ID:2441081

Jeon, Hoseong ^[1];

^[1]; Seo, Junho ^[1]; Kim, Yong Hyun ^[1]; Choi, Eun Sang ^[2]; Jo, Younjung ^[3];

^[4];

^[5];

^[1]

Institute for Basic Science (IBS), Pohang (Korea, Republic of); Pohang Univ. of Science and Technology (POSTECH) (Korea, Republic of)
Florida State Univ., Tallahassee, FL (United States)
Kyungpook National Univ., Daegu (Korea, Republic of)
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Pusan National Univ., Busan (Korea, Republic of)

Magnetic frustration, realized in the special geometrical arrangement of localized spins, often promotes topologically nontrivial spin textures in the real space and induces significantly large unconventional Hall responses. This spin Berry curvature effect in itinerant frustrated magnets mainly works with a static spin order, limiting the effective temperature range below the magnetic transition temperature and yielding the typical anomalous Hall conductivity below ~ 10³ Ω^-1cm^-1. Here we show that an ultraclean triangular-lattice antiferromagnet PdCrO₂ exhibits a large anomalous Hall conductivity up to ~ 10⁶ Ω^-1cm^-1 in the paramagnetic state, which is maintained far above the Neel temperature (T_N) up to ~ 4T_N. The reported enhancement of anomalous Hall response above T_N is attributed to the skew scattering of highly mobile Pd electrons to fluctuating but locally-correlated Cr spins with a finite spin chirality. Our findings point at an alternative route to realizing high-temperature giant anomalous Hall responses, exploiting magnetic frustration in the ultraclean regime.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE); National Science Foundation (NSF)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 2441081

Journal Information:: Communications Physics, Journal Name: Communications Physics Journal Issue: 1 Vol. 7; ISSN 2399-3650

Publisher:: Springer NatureCopyright Statement

Country of Publication:: United States

Language:: English

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