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Title: Mapping twist-tuned multiband topology in bilayer WSe2

Journal Article · · Science
ORCiD logo [1]; ORCiD logo [2]; ORCiD logo [3]; ORCiD logo [3]; ORCiD logo [4]; ORCiD logo [4]; ORCiD logo [3]; ORCiD logo [5]
  1. Stanford Univ., CA (United States); SLAC
  2. Stanford Univ., CA (United States)
  3. Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)
  4. National Institute for Materials Science (NIMS), Tsukuba (Japan)
  5. Stanford Univ., CA (United States); SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States). Stanford Institute for Materials and Energy Science (SIMES)

Semiconductor moiré superlattices have been shown to host a wide array of interaction-driven ground states. However, twisted homobilayers have been difficult to study in the limit of large moiré wavelengths, where interactions are most dominant. In this study, we conducted local electronic compressibility measurements of twisted bilayer WSe2 (tWSe2) at small twist angles. We demonstrated multiple topological bands that host a series of Chern insulators at zero magnetic field near a “magic angle” around 1.23°. Using a locally applied electric field, we induced a topological quantum-phase transition at one hole per moiré unit cell. Finally, our work establishes the topological phase diagram of a generalized Kane-Mele-Hubbard model in tWSe2, demonstrating a tunable platform for strongly correlated topological phases.

Research Organization:
SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
Sponsoring Organization:
US Air Force Office of Scientific Research (AFOSR); USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC02-76SF00515; SC0023109
OSTI ID:
2440966
Journal Information:
Science, Journal Name: Science Journal Issue: 6693 Vol. 384; ISSN 0036-8075
Publisher:
AAASCopyright Statement
Country of Publication:
United States
Language:
English

References (71)

High-Mobility Holes in Dual-Gated WSe 2 Field-Effect Transistors journal September 2015
Correlated insulator behaviour at half-filling in magic-angle graphene superlattices journal March 2018
Unconventional superconductivity in magic-angle graphene superlattices journal March 2018
Valley- and spin-polarized Landau levels in monolayer WSe2 journal October 2016
Quantum simulations with ultracold quantum gases journal April 2012
Lattice reconstruction induced multiple ultra-flat bands in twisted bilayer WSe2 journal September 2021
Magic in twisted transition metal dichalcogenide bilayers journal November 2021
Rotational and dilational reconstruction in transition metal dichalcogenide moiré bilayers journal May 2023
1/4 is the new 1/2 when topology is intertwined with Mottness journal September 2023
Interaction-driven spontaneous ferromagnetic insulating states with odd Chern numbers journal March 2023
Graphene bilayers with a twist journal November 2020
Correlated electronic phases in twisted bilayer transition metal dichalcogenides journal June 2020
Excitons in strain-induced one-dimensional moiré potentials at transition metal dichalcogenide heterojunctions journal July 2020
Tunable spin and valley excitations of correlated insulators in Γ-valley moiré bands journal April 2023
Visualization of moiré superlattices journal June 2020
Charge-order-enhanced capacitance in semiconductor moiré superlattices journal August 2021
Semiconductor moiré materials journal July 2022
A tunable bilayer Hubbard model in twisted WSe2 journal August 2022
Moiré heterostructures as a condensed-matter quantum simulator journal February 2021
Superconductivity and strong correlations in moiré flat bands journal May 2020
Flat bands in twisted bilayer transition metal dichalcogenides journal July 2020
Deep moiré potentials in twisted transition metal dichalcogenide bilayers journal February 2021
Unconventional sequence of correlated Chern insulators in magic-angle twisted bilayer graphene journal September 2021
Correlated Hofstadter spectrum and flavour phase diagram in magic-angle twisted bilayer graphene journal April 2022
Intrinsic spin Hall torque in a moiré Chern magnet journal March 2023
Hofstadter states and re-entrant charge order in a semiconductor moiré lattice journal September 2023
Realization of the Haldane Chern insulator in a moiré lattice journal January 2024
Maximized electron interactions at the magic angle in twisted bilayer graphene journal July 2019
Tunable correlated Chern insulator and ferromagnetism in a moiré superlattice journal March 2020
Simulation of Hubbard model physics in WSe2/WS2 moiré superlattices journal March 2020
Mott and generalized Wigner crystal states in WSe2/WS2 moiré superlattices journal March 2020
Mapping the twist-angle disorder and Landau levels in magic-angle graphene journal May 2020
Cascade of phase transitions and Dirac revivals in magic-angle graphene journal June 2020
Correlated insulating states at fractional fillings of moiré superlattices journal November 2020
Electrical switching of magnetic order in an orbital Chern insulator journal November 2020
Quantum criticality in twisted transition metal dichalcogenides journal September 2021
Continuous Mott transition in semiconductor moiré superlattices journal September 2021
Quantum anomalous Hall effect from intertwined moiré bands journal December 2021
Reproducibility in the fabrication and physics of moiré materials journal February 2022
Signatures of fractional quantum anomalous Hall states in twisted MoTe2 journal June 2023
Thermodynamic evidence of fractional Chern insulator in moiré MoTe2 journal July 2023
Observation of fractionally quantized anomalous Hall effect journal August 2023
Spin-textured Chern bands in AB-stacked transition metal dichalcogenide bilayers journal September 2021
Theory of quantised Hall conductivity in two dimensions journal August 1982
Flat band properties of twisted transition metal dichalcogenide homo- and heterobilayers of MoS2, MoSe2, WS2 and WSe2 journal August 2021
Moiré quantum chemistry: Charge transfer in transition metal dichalcogenide superlattices journal November 2020
Spin-orbit coupling in transition metal dichalcogenide heterobilayer flat bands journal May 2022
Symmetry origin of lattice vibration modes in twisted multilayer graphene: Phasons versus moiré phonons journal August 2022
Excitonic Chern insulator and kinetic ferromagnetism in a MoTe2/WSe2 moiré bilayer journal February 2023
Anomalous Hall metal and fractional Chern insulator in twisted transition metal dichalcogenides journal May 2023
Compressibility of the two-dimensional electron gas: Measurements of the zero-field exchange energy and fractional quantum Hall gap journal July 1994
Phonons and electron-phonon scattering in carbon nanotubes journal May 2002
Lattice relaxation and energy band modulation in twisted bilayer graphene journal August 2017
Strain Engineering of Graphene’s Electronic Structure journal July 2009
Hubbard Model Physics in Transition Metal Dichalcogenide Moiré Bands journal July 2018
Topological Insulators in Twisted Transition Metal Dichalcogenide Homobilayers journal February 2019
Stacking Domains and Dislocation Networks in Marginally Twisted Bilayers of Transition Metal Dichalcogenides journal May 2020
Competing Zero-Field Chern Insulators in Superconducting Twisted Bilayer Graphene journal November 2021
Valley-Polarized Quantum Anomalous Hall State in Moiré MoTe 2 / WSe 2 Heterobilayers journal January 2022
Topological Phases in AB-Stacked MoTe2/WSe2 : Z2 Topological Insulators, Chern Insulators, and Topological Charge Density Waves journal July 2022
Negative compressibility of interacting two-dimensional electron and quasiparticle gases journal February 1992
Quantum Spin Hall Effect in Graphene journal November 2005
Band topology, Hubbard model, Heisenberg model, and Dzyaloshinskii-Moriya interaction in twisted bilayer WSe 2 journal July 2020
Pressure-enhanced fractional Chern insulators along a magic line in moiré transition metal dichalcogenides journal August 2023
Quantum Anomalous Hall Effect from Inverted Charge Transfer Gap journal May 2022
Observation of Integer and Fractional Quantum Anomalous Hall Effects in Twisted Bilayer MoTe2 journal September 2023
Interaction-Driven Topological Phase Diagram of Twisted Bilayer MoTe2 journal November 2023
Valley-Coherent Quantum Anomalous Hall State in AB-Stacked MoTe2/WSe2 Bilayers journal January 2024
Berry phase effects on electronic properties journal July 2010
Colloquium: Topological insulators journal November 2010
Intrinsic quantized anomalous Hall effect in a moiré heterostructure journal December 2019