HIDALGO: A FUN object from the earliest epoch of the solar system’s history

Liu, Ming-Chang; Matsuda, Nozomi; McKeegan, Kevin D.; Dunham, Emilie T.; McCain, Kaitlyn A.

doi:10.1016/j.gca.2024.08.015

Title: HIDALGO: A FUN object from the earliest epoch of the solar system’s history

Journal Article · 17 August 2024 · Geochimica et Cosmochimica Acta

DOI: https://doi.org/10.1016/j.gca.2024.08.015 · OSTI ID:2432476

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Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States); Univ. of California, Los Angeles, CA (United States)
Univ. of California, Los Angeles, CA (United States)

Chemical and isotopic measurements of HIDALGO, a stoichiometrically pure hibonite inclusion found in the matrix of the Dar al Gani 027 meteorite, were conducted by secondary ion mass spectrometry to investigate its origin and evolution. HIDALGO is characterized by large mass-dependent isotope fractionations in O, Ca, and Ti, as well as large negative anomalies in neutron-rich ⁴⁸Ca and ⁵⁰Ti, making it the newest member of the HAL-type FUN inclusions. The highly fractionated Ca and Ti isotopes but unfractionated Mg isotopes are consistent with HIDALGO being a residue from an extensive evaporation event, during which large fractions of initial Ca and Ti, and essentially all the initial Mg, in the precursor material were lost. HIDALGO appears to have incorporated live ²⁶Al at a higher level than other HAL-type inclusions, but still at a lower amount compared to the Solar System’s initial ²⁶Al abundance typically found in non-FUN CAIs. Interestingly, the inferred ¹⁰Be abundance in HIDALGO is comparable to the values observed in the majority of CV3 CAIs but ~ 2.5 times higher than those in HAL-type samples. HIDALGO’s unusual ²⁶Al/²⁷Al and ¹⁰Be/⁹Be ratios, together with the ⁴⁸Ca-⁵⁰Ti anomalies, can be best explained by the formation of its precursor material in the isotopically heterogeneous solar nebula. Finally, large ⁷Li excesses correlating with Be/Li were found in HIDALGO, a behavior that can be interpreted as due to in-situ decay of live ⁷Be. Charged particle spallation of initially Li-free HIDALGO can simultaneously account for the inferred ⁷Be abundance and the measured Li elemental concentration. The consistency between the measurement and spallation calculation results provides support for the prior existence of ⁷Be in HIDALGO, possibly produced by irradiation close to the Sun.

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Research Organization:: Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)

Sponsoring Organization:: National Aeronautics and Space Administration (NASA); USDOE; USDOE Laboratory Directed Research and Development (LDRD) Program; USDOE National Nuclear Security Administration (NNSA)

Grant/Contract Number:: AC52-07NA27344

OSTI ID:: 2432476

Report Number(s):: LLNL--JRNL-856658; 1086293

Journal Information:: Geochimica et Cosmochimica Acta, Journal Name: Geochimica et Cosmochimica Acta Vol. 386; ISSN 0016-7037

Publisher:: Elsevier; The Geochemical Society; The Meteoritical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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