A single-point modeling approach for the intercomparison and evaluation of ozone dry deposition across chemical transport models (Activity 2 of AQMEII4)

Clifton, Olivia E.; Schwede, Donna; Hogrefe, Christian; Bash, Jesse O.; Bland, Sam; Cheung, Philip; Coyle, Mhairi; Emberson, Lisa; Flemming, Johannes; Fredj, Erick; Galmarini, Stefano; Ganzeveld, Laurens; Gazetas, Orestis; Goded, Ignacio; Holmes, Christopher D.; Horváth, László; Huijnen, Vincent; Li, Qian; Makar, Paul A.; Mammarella, Ivan; Manca, Giovanni; Munger, J. William; Pérez-Camanyo, Juan L.; Pleim, Jonathan; Ran, Limei; San Jose, Roberto; Silva, Sam J.; Staebler, Ralf; Sun, Shihan; Tai, Amos P. K.; Tas, Eran; Vesala, Timo; Weidinger, Tamás; Wu, Zhiyong; Zhang, Leiming

doi:10.5194/acp-23-9911-2023

Title: A single-point modeling approach for the intercomparison and evaluation of ozone dry deposition across chemical transport models (Activity 2 of AQMEII4)

Journal Article · 06 September 2023 · Atmospheric Chemistry and Physics (Online)

DOI: https://doi.org/10.5194/acp-23-9911-2023 · OSTI ID:2424085

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NASA Goddard Inst. for Space Studies (GISS), New York, NY (United States); Columbia Univ., New York, NY (United States)
US Environmental Protection Agency (EPA), Research Triangle Park, NC (United States)
Univ. of York (United Kingdom)
Environment and Climate Change Canada, Toronto, ON (Canada)
United Kingdom Centre for Ecology and Hydrology (United Kingdom); James Hutton Institute (United Kingdom)
European Centre for Medium-Range Weather Forecasts, Reading (United Kingdom)
Jerusalem College of Technology (Israel)
European Commission (Italy). Joint Research Centre (JRC)
Wageningen Univ. (Netherlands)
European Commission (Italy). Joint Research Centre (JRC); Scottish Universities Environmental Research Centre (SUERC), East Kilbride (United Kingdom)
Florida State Univ., Tallahassee, FL (United States)
Univ. of Szeged (Hungary)
Royal Netherlands Meteorological Institute (KNMI), De Bilt (Netherlands)
Hebrew Univ. of Jerusalem (Israel)
Univ. of Helsinki (Finland)
Harvard Univ., Cambridge, MA (United States)
Technical University of Madrid (Spain)
US Dept. of Agriculture (USDA), Greensboro, NC (United States)
Univ. of Southern California, Los Angeles, CA (United States)
The Chinese University of Hong Kong (Hong Kong)
Eotvos Lorand University, Budapest (Hungary)
US Environmental Protection Agency (EPA), Research Triangle Park, NC (United States); RTI International, Research Triangle Park, NC (United States)

A primary sink of air pollutants and their precursors is dry deposition. Dry deposition estimates differ across chemical transport models, yet an understanding of the model spread is incomplete. Here, we introduce Activity 2 of the Air Quality Model Evaluation International Initiative Phase 4 (AQMEII4). We examine 18 dry deposition schemes from regional and global chemical transport models as well as standalone models used for impact assessments or process understanding. We configure the schemes as single-point models at eight Northern Hemisphere locations with observed ozone fluxes. Single-point models are driven by a common set of site-specific meteorological and environmental conditions. Five of eight sites have at least 3 years and up to 12 years of ozone fluxes. The interquartile range across models in multiyear mean ozone deposition velocities ranges from a factor of 1.2 to 1.9 annually across sites and tends to be highest during winter compared with summer. No model is within 50 % of observed multiyear averages across all sites and seasons, but some models perform well for some sites and seasons. For the first time, we demonstrate how contributions from depositional pathways vary across models. Models can disagree with respect to relative contributions from the pathways, even when they predict similar deposition velocities, or agree with respect to the relative contributions but predict different deposition velocities. Both stomatal and nonstomatal uptake contribute to the large model spread across sites. Our findings are the beginning of results from AQMEII4 Activity 2, which brings scientists who model air quality and dry deposition together with scientists who measure ozone fluxes to evaluate and improve dry deposition schemes in the chemical transport models used for research, planning, and regulatory purposes.

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Research Organization:: Oak Ridge Associated Universities (ORAU), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Biological and Environmental Research (BER)

Grant/Contract Number:: AC05-06OR23100

OSTI ID:: 2424085

Journal Information:: Atmospheric Chemistry and Physics (Online), Journal Name: Atmospheric Chemistry and Physics (Online) Journal Issue: 17 Vol. 23; ISSN 1680-7324

Publisher:: Copernicus Publications, EGUCopyright Statement

Country of Publication:: United States

Language:: English

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Canopy-Atmosphere Exchange of Carbon, Water and Energy at Harvard Forest EMS Tower since 1991 Munger, William; Wofsy, Steven Environmental Data Initiative https://doi.org/10.6073/pasta/4b565f106ffd584640c10cc66c1bc748	dataset	January 2015
Radiation Measurements at Harvard Forest EMS Tower 1991-2007 Fitzjarrald, David; Sakai, Ricardo Environmental Data Initiative https://doi.org/10.6073/pasta/f3adbe87e7e506c720d0d9ee91d2b6c4	dataset	January 2023
Urban ecosystem services: tree diversity and stability of tropospheric ozone removal Manes, Fausto; Incerti, Guido; Salvatori, Elisabetta Figshare https://doi.org/10.6084/m9.figshare.c.3295310	collection	January 2016

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