Kinetics of Shear-Induced Structural Ordering in Dense Colloids

He, HongRui; Lee, Jonghun; Jiang, Zhang; He, Qiming; Dinic, Jelena; Chen, Wei; Narayanan, Suresh; Lin, Xiao-Min

doi:10.1021/acs.jpcb.3c03290

Title: Kinetics of Shear-Induced Structural Ordering in Dense Colloids

Journal Article · 10 August 2023 · Journal of Physical Chemistry. B

DOI: https://doi.org/10.1021/acs.jpcb.3c03290 · OSTI ID:2404546

He, HongRui ^[1]; Lee, Jonghun ^[2]; Jiang, Zhang ^[2];

^[1];

^[1]; Narayanan, Suresh ^[2];

^[3]

Argonne National Laboratory (ANL), Argonne, IL (United States); Univ. of Chicago, IL (United States)
Argonne National Laboratory (ANL), Argonne, IL (United States). Advanced Photon Source (APS)
Argonne National Laboratory (ANL), Argonne, IL (United States). Center for Nanoscale Materials (CNM)

The macroscopic rheological response of a colloidal solution is highly correlated with the local microscopic structure, as revealed by an in situ Rheo-SAXS experiment with a high temporal resolution. Oscillatory shear can induce a strain-controlled ordering-to-disorder transition, resulting in a shear-thickening process that is different from the normal shear-thickening behavior that is driven by hydrodynamics and particle friction. Here, we reveal that there is a complex time-dependent kinetics toward structural ordering under different applied strains. When the strain amplitude reaches a critical value that starts to induce disordering in the system, the pathway toward the dynamic equilibrium can also become highly non-monotonic. Within the same oscillatory cycle, there is a strong correlation of ordering with different phases of the oscillation, with the system oscillating between two dynamic metastable states.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Laboratory Directed Research and Development (LDRD) Program; USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities (SUF)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 2404546

Journal Information:: Journal of Physical Chemistry. B, Journal Name: Journal of Physical Chemistry. B Journal Issue: 33 Vol. 127; ISSN 1520-6106

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
Chemical structure
Crystals
Kinetics
Order-to-disorder transition
Oscillation
Oscillatory shear
Rheo-SAXS
Scattering

Title: Kinetics of Shear-Induced Structural Ordering in Dense Colloids

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