Roadmap on perovskite light-emitting diodes

Chen, Ziming; Hoye, Robert L. Z.; Yip, Hin-Lap; Fiuza-Maneiro, Nadesh; López-Fernández, Iago; Otero-Martínez, Clara; Polavarapu, Lakshminarayana; Mondal, Navendu; Mirabelli, Alessandro; Anaya, Miguel; Stranks, Samuel D.; Liu, Hui; Shi, Guangyi; Xiao, Zhengguo; Kim, Nakyung; Kim, Yunna; Shin, Byungha; Shi, Jinquan; Liu, Mengxia; Zhang, Qianpeng; Fan, Zhiyong; Loy, James C.; Zhao, Lianfeng; Rand, Barry P.; Arfin, Habibul; Saikia, Sajid; Nag, Angshuman; Zou, Chen; Lin, Lih Y.; Xiang, Hengyang; Zeng, Haibo; Liu, Denghui; Su, Shi-Jian; Wang, Chenhui; Zhong, Haizheng; Xuan, Tong-Tong; Xie, Rong-Jun; Bao, Chunxiong; Gao, Feng; Gao, Xiang; Qin, Chuanjiang; Kim, Young-Hoon; Beard, Matthew C.

doi:10.1088/2515-7647/ad46a6

Title: Roadmap on perovskite light-emitting diodes

Journal Article · 11 July 2024 · JPhys Photonics

DOI: https://doi.org/10.1088/2515-7647/ad46a6 · OSTI ID:2397014

; Hoye, Robert L. Z.; Yip, Hin-Lap;

;

; Otero-Martínez, Clara; Polavarapu, Lakshminarayana;

; Mirabelli, Alessandro; Anaya, Miguel; Stranks, Samuel D.;

; Shi, Guangyi; Xiao, Zhengguo; Kim, Nakyung; Kim, Yunna;

;

; Liu, Mengxia; Zhang, Qianpeng more »

Abstract In recent years, the field of metal-halide perovskite emitters has rapidly emerged as a new community in solid-state lighting. Their exceptional optoelectronic properties have contributed to the rapid rise in external quantum efficiencies (EQEs) in perovskite light-emitting diodes (PeLEDs) from <1% (in 2014) to over 30% (in 2023) across a wide range of wavelengths. However, several challenges still hinder their commercialization, including the relatively low EQEs of blue/white devices, limited EQEs in large-area devices, poor device stability, as well as the toxicity of the easily accessible lead components and the solvents used in the synthesis and processing of PeLEDs. This roadmap addresses the current and future challenges in PeLEDs across fundamental and applied research areas, by sharing the community’s perspectives. This work will provide the field with practical guidelines to advance PeLED development and facilitate more rapid commercialization.

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Sponsoring Organization:: USDOE

Grant/Contract Number:: AC36-08GO28308

OSTI ID:: 2397014

Journal Information:: JPhys Photonics, Journal Name: JPhys Photonics Journal Issue: 3 Vol. 6; ISSN 2515-7647

Publisher:: IOP PublishingCopyright Statement

Country of Publication:: United Kingdom

Language:: English

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Spectra stable blue perovskite light-emitting diodes Jiang, Yuanzhi; Qin, Chaochao; Cui, Minghuan Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-09794-7	journal	April 2019
Ultrafast long-range spin-funneling in solution-processed Ruddlesden–Popper halide perovskites Giovanni, David; Lim, Jia Wei Melvin; Yuan, Zhongcheng Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-11251-4	journal	August 2019
Single-particle electroluminescence of CsPbBr3 perovskite nanocrystals reveals particle-selective recombination and blinking as key efficiency factors Sharma, Dharmendar Kumar; Hirata, Shuzo; Vacha, Martin Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-12512-y	journal	October 2019
Efficient sky-blue perovskite light-emitting diodes via photoluminescence enhancement Wang, Qi; Wang, Xiaoming; Yang, Zhi Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-13580-w	journal	December 2019
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245 MHz bandwidth organic light-emitting diodes used in a gigabit optical wireless data link Yoshida, Kou; Manousiadis, Pavlos P.; Bian, Rui Nature Communications, Vol. 11, Issue 1 https://doi.org/10.1038/s41467-020-14880-2	journal	March 2020
Transient circular dichroism and exciton spin dynamics in all-inorganic halide perovskites Zhao, Weijie; Su, Rui; Huang, Yuqing Nature Communications, Vol. 11, Issue 1 https://doi.org/10.1038/s41467-020-19471-9	journal	November 2020
Large-area and efficient perovskite light-emitting diodes via low-temperature blade-coating Chu, Shenglong; Chen, Wenjing; Fang, Zhibin Nature Communications, Vol. 12, Issue 1 https://doi.org/10.1038/s41467-020-20433-4	journal	January 2021
Reducing the impact of Auger recombination in quasi-2D perovskite light-emitting diodes Jiang, Yuanzhi; Cui, Minghuan; Li, Saisai Nature Communications, Vol. 12, Issue 1 https://doi.org/10.1038/s41467-020-20555-9	journal	January 2021
Interpenetrating interfaces for efficient perovskite solar cells with high operational stability and mechanical robustness Dong, Qingshun; Zhu, Chao; Chen, Min Nature Communications, Vol. 12, Issue 1 https://doi.org/10.1038/s41467-021-21292-3	journal	February 2021
Smoothing the energy transfer pathway in quasi-2D perovskite films using methanesulfonate leads to highly efficient light-emitting devices Kong, Lingmei; Zhang, Xiaoyu; Li, Yunguo Nature Communications, Vol. 12, Issue 1 https://doi.org/10.1038/s41467-021-21522-8	journal	February 2021
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Efficient and large-area all vacuum-deposited perovskite light-emitting diodes via spatial confinement Du, Peipei; Li, Jinghui; Wang, Liang Nature Communications, Vol. 12, Issue 1 https://doi.org/10.1038/s41467-021-25093-6	journal	August 2021
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Anisotropic nanocrystal superlattices overcoming intrinsic light outcoupling efficiency limit in perovskite quantum dot light-emitting diodes Kumar, Sudhir; Marcato, Tommaso; Krumeich, Frank Nature Communications, Vol. 13, Issue 1 https://doi.org/10.1038/s41467-022-29812-5	journal	April 2022
Direct in situ photolithography of perovskite quantum dots based on photocatalysis of lead bromide complexes Zhang, Pingping; Yang, Gaoling; Li, Fei Nature Communications, Vol. 13, Issue 1 https://doi.org/10.1038/s41467-022-34453-9	journal	November 2022
Suppressing phase disproportionation in quasi-2D perovskite light-emitting diodes Wang, Kang; Lin, Zih-Yu; Zhang, Zihan Nature Communications, Vol. 14, Issue 1 https://doi.org/10.1038/s41467-023-36118-7	journal	January 2023
High-efficiency, flexible and large-area red/green/blue all-inorganic metal halide perovskite quantum wires-based light-emitting diodes Cao, Yang Bryan; Zhang, Daquan; Zhang, Qianpeng Nature Communications, Vol. 14, Issue 1 https://doi.org/10.1038/s41467-023-40150-y	journal	August 2023
Charge injection engineering at organic/inorganic heterointerfaces for high-efficiency and fast-response perovskite light-emitting diodes Li, Zhenchao; Chen, Ziming; Shi, Zhangsheng Nature Communications, Vol. 14, Issue 1 https://doi.org/10.1038/s41467-023-41929-9	journal	October 2023
Metal halide perovskites for light-emitting diodes Liu, Xiao-Ke; Xu, Weidong; Bai, Sai Nature Materials, Vol. 20, Issue 1 https://doi.org/10.1038/s41563-020-0784-7	journal	September 2020
Bipolar-shell resurfacing for blue LEDs based on strongly confined perovskite quantum dots Dong, Yitong; Wang, Ya-Kun; Yuan, Fanglong Nature Nanotechnology, Vol. 15, Issue 8 https://doi.org/10.1038/s41565-020-0714-5	journal	July 2020
Nanoscale chemical heterogeneity dominates the optoelectronic response of alloyed perovskite solar cells Frohna, Kyle; Anaya, Miguel; Macpherson, Stuart Nature Nanotechnology, Vol. 17, Issue 2 https://doi.org/10.1038/s41565-021-01019-7	journal	November 2021
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Industry outlook of perovskite quantum dots for display applications Wu, Xian-gang; Ji, Honglei; Yan, Xiaolin Nature Nanotechnology, Vol. 17, Issue 8 https://doi.org/10.1038/s41565-022-01163-8	journal	July 2022
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Efficient blue light-emitting diodes based on quantum-confined bromide perovskite nanostructures Liu, Yang; Cui, Jieyuan; Du, Kai Nature Photonics, Vol. 13, Issue 11 https://doi.org/10.1038/s41566-019-0505-4	journal	August 2019
Reversible 3D laser printing of perovskite quantum dots inside a transparent medium Huang, Xiongjian; Guo, Qianyi; Yang, Dandan Nature Photonics, Vol. 14, Issue 2 https://doi.org/10.1038/s41566-019-0538-8	journal	November 2019
Best practices for measuring emerging light-emitting diode technologies Anaya, Miguel; Rand, Barry P.; Holmes, Russell J. Nature Photonics, Vol. 13, Issue 12 https://doi.org/10.1038/s41566-019-0543-y	journal	November 2019
Triplet management for efficient perovskite light-emitting diodes Qin, Chuanjiang; Matsushima, Toshinori; Potscavage, William J. Nature Photonics, Vol. 14, Issue 2 https://doi.org/10.1038/s41566-019-0545-9	journal	November 2019
Large-area near-infrared perovskite light-emitting diodes Zhao, Xiaofei; Tan, Zhi-Kuang Nature Photonics, Vol. 14, Issue 4 https://doi.org/10.1038/s41566-019-0559-3	journal	December 2019
Comprehensive defect suppression in perovskite nanocrystals for high-efficiency light-emitting diodes Kim, Young-Hoon; Kim, Sungjin; Kakekhani, Arvin Nature Photonics, Vol. 15, Issue 2 https://doi.org/10.1038/s41566-020-00732-4	journal	January 2021
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Large-scale planar and spherical light-emitting diodes based on arrays of perovskite quantum wires Zhang, Daquan; Zhang, Qianpeng; Ren, Beitao Nature Photonics, Vol. 16, Issue 4 https://doi.org/10.1038/s41566-022-00978-0	journal	March 2022
Ultrastable near-infrared perovskite light-emitting diodes Guo, Bingbing; Lai, Runchen; Jiang, Sijie Nature Photonics, Vol. 16, Issue 9 https://doi.org/10.1038/s41566-022-01046-3	journal	August 2022
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Minimizing non-radiative recombination losses in perovskite solar cells Luo, Deying; Su, Rui; Zhang, Wei Nature Reviews Materials, Vol. 5, Issue 1 https://doi.org/10.1038/s41578-019-0151-y	journal	November 2019
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Towards micro-PeLED displays Yang, Xiaoyu; Ma, Li; Li, Lei Nature Reviews Materials, Vol. 8, Issue 5 https://doi.org/10.1038/s41578-022-00522-0	journal	January 2023
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High-Efficiency Tandem White Perovskite Light-Emitting Diodes by Using an Organic/Inorganic Intermediate Connector Yan, Yu; Zhang, Qi; Wang, Zhijian Crystals, Vol. 12, Issue 9 https://doi.org/10.3390/cryst12091286	journal	September 2022
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