A compact approach to higher-resolution resonant inelastic x-ray scattering detection using photoelectrons

Schunck, Jan O.; Buck, Jens; Engel, Robin Y.; Kruse, Simon R.; Marotzke, Simon; Scholz, Markus; Mahatha, Sanjoy K.; Huang, Meng-Jie; Rønnow, Henrik M.; Dakovski, Georgi; Hoesch, Moritz; Kalläne, Matthias; Rossnagel, Kai; Beye, Martin

doi:10.1088/1367-2630/ad4206

Title: A compact approach to higher-resolution resonant inelastic x-ray scattering detection using photoelectrons

Journal Article · 08 May 2024 · New Journal of Physics

DOI: https://doi.org/10.1088/1367-2630/ad4206 · OSTI ID:2396965

^[1]; Buck, Jens ^[2];

^[3]; Kruse, Simon R. ^[4];

^[2];

^[5]; Mahatha, Sanjoy K. ^[5];

^[5]; Rønnow, Henrik M. ^[6]; Dakovski, Georgi ^[7]; Hoesch, Moritz ^[5]; Kalläne, Matthias ^[8];

^[2];

^[3]

Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany); Univ. of Hamburg (Germany); SLAC
Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany); Christian-Albrechts-Universität zu Kiel (Germany)
Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany); Univ. of Hamburg (Germany); Stockholm Univ. (Sweden)
Univ. of Hamburg (Germany)
Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany)
Ecole Polytechnique Federale Lausanne (EPFL) (Switzerland)
SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
Christian-Albrechts-Universität zu Kiel (Germany)

The detection of inelastically scattered soft x-rays with high energy resolution usually requires large grating spectrometers. Recently, photoelectron spectrometry for analysis of x-rays (PAX) has been rediscovered for modern spectroscopy experiments at synchrotron light sources. By converting scattered photons to electrons and using an electron energy analyser, the energy resolution for resonant inelastic x-ray scattering (RIXS) becomes decoupled from the x-ray spot size and instrument length. In this work, we develop PAX towards high energy resolution using a modern photoemission spectroscopy setup studying Ba₂Cu₃O₄Cl₂ at the Cu L₃-edge. We measure a momentum transfer range of 24% of the first Brillouin zone simultaneously. Our results hint at the observation of a magnon excitation below 100 meV energy transfer and show intensity variations related to the dispersion of dd-excitations. With dedicated setups, PAX can complement the best and largest RIXS instruments, while at the same time opening new opportunities to acquire RIXS at a range of momentum transfers simultaneously and combine it with angle-resolved photoemission spectroscopy in a single instrument.

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Research Organization:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC); Helmholtz Association of German Research Centres

Grant/Contract Number:: AC02-76SF00515

OSTI ID:: 2396965

Journal Information:: New Journal of Physics, Journal Name: New Journal of Physics Journal Issue: 5 Vol. 26; ISSN 1367-2630

Publisher:: IOP PublishingCopyright Statement

Country of Publication:: United States

Language:: English

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Title: A compact approach to higher-resolution resonant inelastic x-ray scattering detection using photoelectrons

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