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Title: Aqueous phosphate detection using Eu(acac)3

Journal Article · · Applied Physics. B, Lasers and Optics
 [1];  [2];  [2];  [3]
  1. Washington State Univ., Spokane, WA (United States). Institute for Shock Physics; ExMat Research
  2. Washington State Univ., Spokane, WA (United States). Institute for Shock Physics
  3. ExMat Research Inc., Spokane, WA (United States)

Currently, the majority of phosphate-sensitive phosphors reported in literature are metal-based complexes that require complicated and expensive synthesis to prepare. Here, in this study, we investigate the phosphate detecting capabilities of an inexpensive off-the-shelf phosphor: Eu(acac)3. We characterize its phosphate sensitivity as a function of sensor concentration and find that the quenching coefficient is inversely proportional to sensor concentration. This results in the limit-of-detection scaling linearly with sensor concentration. We determine its concentration-independent sensitivity to be 1.558 ± 0.012, which results in our lowest sensor concentration (44 μM) having a limit-of-detection of 3.39 ± 0.68 μM. We also find that for phosphate concentrations less than the sensor concentration, the fluorescence intensity ratio behaves linearly, but transitions to a non-linear functionality as the phosphate concentration exceeds the sensor concentration.

Research Organization:
ExMat Research Inc., Spokane, WA (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Biological and Environmental Research (BER). Biological Systems Science (BSS)
Grant/Contract Number:
SC0022391
OSTI ID:
2345191
Journal Information:
Applied Physics. B, Lasers and Optics, Journal Name: Applied Physics. B, Lasers and Optics Journal Issue: 12 Vol. 129; ISSN 0946-2171
Publisher:
SpringerCopyright Statement
Country of Publication:
United States
Language:
English

References (30)

Postsynthetic Metalation Metal–Organic Framework as a Fluorescent Probe for the Ultrasensitive and Reversible Detection of PO43– Ions journal August 2018
Metal–organic frameworks with inherent recognition sites for selective phosphate sensing through their coordination-induced fluorescence enhancement effect journal January 2015
Controlled synthesis of EuPO4 nano/microstructures and core–shell SiO2@EuPO4 nanostructures with improved photoluminescence journal January 2017
Dynamic Vertical Profiles of Peat Porewater Chemistry in a Northern Peatland journal October 2016
Rapid photobleaching of organic laser dyes in continuously operated devices journal April 1971
Phosphorus Retention in Streams and Wetlands: A Review journal January 1999
A Specific Turn-On Fluorescent Sensing for Ultrasensitive and Selective Detection of Phosphate in Environmental Samples Based on Antenna Effect-Improved FRET by Surfactant journal July 2018
Metal–organic frameworks (MOFs) combined with ZnO quantum dots as a fluorescent sensing platform for phosphate journal July 2014
Fluorescence detection of phosphate in an aqueous environment by an aluminum-based metal-organic framework with amido functionalized ligands journal July 2022
Molecular Photobleaching Kinetics of Rhodamine 6G by One‐ and Two‐Photon Induced Confocal Fluorescence Microscopy journal April 2005
Eutrophication of U.S. Freshwaters: Analysis of Potential Economic Damages journal January 2009
Europium-Based Metal–Organic Framework as a Dual Luminescence Sensor for the Selective Detection of the Phosphate Anion and Fe3+ Ion in Aqueous Media journal September 2018
Phosphorus Forms in Sediments of a River-Dominated Estuary journal September 2018
A design for detecting phosphate ions in aqueous solution by luminescent Tb-coordination polymer journal January 2021
Emerging Tools for Continuous Nutrient Monitoring Networks: Sensors Advancing Science and Water Resources Protection journal February 2016
Rational design of a highly sensitive and selective “turn-on” fluorescent sensor for PO43− detection journal January 2015
Spectroscopic properties of Eu:Y(acac)3(DPEPO) and characterization of its photo- and thermal- degradation journal November 2022
Synthesis and Spectral Characterization of EuPO4 and LaPO4:Eu Nanorods journal March 2010
A dual functional MOF-based fluorescent sensor for intracellular phosphate and extracellular 4-nitrobenzaldehyde journal January 2019
Photobleaching of Rhodamine 6G in polyacrylonitrile matrix journal July 1974
Highly Selective and Sensitive Detection of PO43– Ions in Aqueous Solution by a Luminescent Terbium Metal–Organic Framework journal September 2019
Soil phosphorus flux from emergent marsh wetlands and surrounding grazed pasture uplands journal October 2010
Complete Transmetalation in a Metal–Organic Framework by Metal Ion Metathesis in a Single Crystal for Selective Sensing of Phosphate Ions in Aqueous Media journal August 2016
Fluorescence detection for phosphate monitoring using reverse injection analysis journal July 2014
Photobleaching quantum yields of an aqueous-micellar solution of rhodamine 6g during continuous and pulsed irradiation journal November 1987
A water-stable lanthanide-organic framework as a recyclable luminescent probe for detecting pollutant phosphorus anions journal January 2015
Highly sensitive and selective fluorescent detection of phosphate in water environment by a functionalized coordination polymer journal October 2019
Basics of Lanthanide Photophysics book January 2010
Trace Quantity Detection of H 2 PO 4 by Fluorescent Metal–Organic Framework (F-MOF) and Bioimaging Study journal September 2020
Phosphorus sorption on tropical soils with relevance to Earth system model needs journal January 2019