Comprehensive parametric study of CO2 sequestration in deep saline aquifers

Khanal, Aaditya; Irfan Khan, Md; Fahim Shahriar, Md

doi:10.1016/j.ces.2024.119734

Title: Comprehensive parametric study of CO₂ sequestration in deep saline aquifers

Journal Article · 11 January 2024 · Chemical Engineering Science

DOI: https://doi.org/10.1016/j.ces.2024.119734 · OSTI ID:2345114

^[1]; Irfan Khan, Md ^[2]; Fahim Shahriar, Md ^[2]

Univ. of Texas, Tyler, TX (United States); UT Tyler
Univ. of Texas, Tyler, TX (United States)

Carbon dioxide injection in deep saline aquifers is a key method for permanently sequestering anthropogenic CO₂. Here this study employs a reactive transport model to explore mineral precipitation/dissolution and its impact on reservoir properties in deep saline aquifers. We also assess capillary pressure and relative permeability hysteresis on various CO₂ trapping mechanisms. Results from this study reveal the significant influence of initial brine composition on mineral precipitation/dissolution. The dissolution and precipitation of minerals have different effects around the wellbores compared to the overall reservoir. Additionally, salt concentration (Ca⁺⁺ and Mg⁺⁺) and quartz surface area affect CO₂ mineralization, while Na⁺ impacts halite precipitation, altering flow properties. The effect of capillary pressure is significant, as including the capillary pressure in the simulation case resulted in significantly improved CO₂ trapping, achieving almost total dissolution of the injected CO₂ in around 300 years. This study offers novel insights into the interactions of reservoir minerals, brine properties, and the injected CO₂.

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Research Organization:: Univ. of Texas at Tyler, TX (United States)

Sponsoring Organization:: National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences & Biosciences Division (CSGB)

Grant/Contract Number:: SC0024642

OSTI ID:: 2345114

Journal Information:: Chemical Engineering Science, Journal Name: Chemical Engineering Science Vol. 287; ISSN 0009-2509

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
CO2 sequestration
hysteresis modeling
mineral dissolution
mineral precipitation
reservoir simulation

Title: Comprehensive parametric study of CO2 sequestration in deep saline aquifers

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References (79)

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Title: Comprehensive parametric study of CO₂ sequestration in deep saline aquifers