Exceptionally High Perfluorooctanoic Acid Uptake in Water by a Zirconium-Based Metal–Organic Framework through Synergistic Chemical and Physical Adsorption

Liang, Rong-Ran; Xu, Shunqi; Han, Zongsu; Yang, Yihao; Wang, Kun-Yu; Huang, Zhehao; Rushlow, Joshua; Cai, Peiyu; Samorì, Paolo; Zhou, Hong-Cai

doi:10.1021/jacs.3c14487

Title: Exceptionally High Perfluorooctanoic Acid Uptake in Water by a Zirconium-Based Metal–Organic Framework through Synergistic Chemical and Physical Adsorption

Journal Article · 25 March 2024 · Journal of the American Chemical Society

DOI: https://doi.org/10.1021/jacs.3c14487 · OSTI ID:2328650

Liang, Rong-Ran ^[1]; Xu, Shunqi ^[2]; Han, Zongsu ^[1]; Yang, Yihao ^[1]; Wang, Kun-Yu ^[1];

^[3]; Rushlow, Joshua ^[1]; Cai, Peiyu ^[1];

^[2];

^[1]

Department of Chemistry, Texas A&M University, College Station, Texas 77843, United States
Université de Strasbourg, CNRS, ISIS, 8 alleé Gaspard Monge, 67000 Strasbourg, France
Department of Materials and Environmental Chemistry, Stockholm University, SE-106 91 Stockholm, Sweden

Not Available

View Journal Article

Cite

Export

Save

Sponsoring Organization:: USDOE Office of Fossil Energy and Carbon Management (FECM)

Grant/Contract Number:: FE0032108

OSTI ID:: 2328650

Alternate ID(s):: OSTI ID: 2335871

Journal Information:: Journal of the American Chemical Society, Journal Name: Journal of the American Chemical Society Journal Issue: 14 Vol. 146; ISSN 0002-7863

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

References (41)

Multi-Photon Absorption in Metal-Organic Frameworks Medishetty, Raghavender; Nemec, Lydia; Nalla, Venkatram Angewandte Chemie International Edition, Vol. 56, Issue 46 https://doi.org/10.1002/anie.201706492	journal	October 2017
Luminescent Functional Metal–Organic Frameworks Cui, Yuanjing; Yue, Yanfeng; Qian, Guodong Chemical Reviews, Vol. 112, Issue 2 https://doi.org/10.1021/cr200101d	journal	June 2011
Integrated Photocatalytic Reduction and Oxidation of Perfluorooctanoic Acid by Metal–Organic Frameworks: Key Insights into the Degradation Mechanisms Wen, Yinghao; Rentería-Gómez, Ángel; Day, Gregory S. Journal of the American Chemical Society, Vol. 144, Issue 26 https://doi.org/10.1021/jacs.2c04341	journal	June 2022
Lanthanide–Organic Frameworks Featuring Three-Dimensional Inorganic Connectivity for Multipurpose Hydrocarbon Separation Wang, Xinxin; Yue, Lianglan; Zhou, Ping Inorganic Chemistry, Vol. 60, Issue 22 https://doi.org/10.1021/acs.inorgchem.1c02614	journal	October 2021
Power of Infrared and Raman Spectroscopies to Characterize Metal-Organic Frameworks and Investigate Their Interaction with Guest Molecules Hadjiivanov, Konstantin I.; Panayotov, Dimitar A.; Mihaylov, Mihail Y. Chemical Reviews, Vol. 121, Issue 3 https://doi.org/10.1021/acs.chemrev.0c00487	journal	December 2020
Removal of GenX and Perfluorinated Alkyl Substances from Water by Amine-Functionalized Covalent Organic Frameworks Ji, Woojung; Xiao, Leilei; Ling, Yuhan Journal of the American Chemical Society, Vol. 140, Issue 40 https://doi.org/10.1021/jacs.8b06958	journal	September 2018
Biological Utility of Fluorinated Compounds: from Materials Design to Molecular Imaging, Therapeutics and Environmental Remediation Zhang, Cheng; Yan, Kai; Fu, Changkui Chemical Reviews, Vol. 122, Issue 1 https://doi.org/10.1021/acs.chemrev.1c00632	journal	October 2021
Per- and polyfluoroalkyl substances in the environment Evich, Marina G.; Davis, Mary J. B.; McCord, James P. Science, Vol. 375, Issue 6580 https://doi.org/10.1126/science.abg9065	journal	February 2022
Low-temperature mineralization of perfluorocarboxylic acids Trang, Brittany; Li, Yuli; Xue, Xiao-Song Science, Vol. 377, Issue 6608, p. 839-845 https://doi.org/10.1126/science.abm8868	journal	August 2022
Metal-organic frameworks as platforms for the removal of per- and polyfluoroalkyl substances from contaminated waters Li, Rui; Adarsh, Nayarassery N.; Lu, Hui Matter, Vol. 5, Issue 10 https://doi.org/10.1016/j.matt.2022.07.028	journal	October 2022
A stable zirconium based metal-organic framework for specific recognition of representative polychlorinated dibenzo-p-dioxin molecules Wang, Bin; Wang, Peilong; Xie, Lin-Hua Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-11912-4	journal	August 2019
Sustainable environmental remediation via biomimetic multifunctional lignocellulosic nano-framework Li, Jinghao; Li, Xiaohan; Da, Yabin Nature Communications, Vol. 13, Issue 1 https://doi.org/10.1038/s41467-022-31881-5	journal	July 2022
Cationic covalent organic framework for efficient removal of PFOA substitutes from aqueous solution Wang, Wei; Zhou, Ziming; Shao, Haipei Chemical Engineering Journal, Vol. 412 https://doi.org/10.1016/j.cej.2020.127509	journal	May 2021
Highly Selective Removal of Perfluorinated Contaminants by Adsorption on All‐Silica Zeolite Beta Van den Bergh, Matthias; Krajnc, Andraž; Voorspoels, Stefan Angewandte Chemie International Edition, Vol. 59, Issue 33 https://doi.org/10.1002/anie.202002953	journal	May 2020
Efficient Removal of Per- and Polyfluoroalkyl Substances from Water with Zirconium-Based Metal–Organic Frameworks Li, Rui; Alomari, Shefa; Stanton, Robert Chemistry of Materials, Vol. 33, Issue 9 https://doi.org/10.1021/acs.chemmater.1c00324	journal	April 2021
Systematic Study on the Removal of Per- and Polyfluoroalkyl Substances from Contaminated Groundwater Using Metal–Organic Frameworks Li, Rui; Alomari, Shefa; Islamoglu, Timur Environmental Science & Technology, Vol. 55, Issue 22 https://doi.org/10.1021/acs.est.1c03974	journal	October 2021
β-Cyclodextrin Polymer Network Sequesters Perfluorooctanoic Acid at Environmentally Relevant Concentrations Xiao, Leilei; Ling, Yuhan; Alsbaiee, Alaaeddin Journal of the American Chemical Society, Vol. 139, Issue 23 https://doi.org/10.1021/jacs.7b02381	journal	May 2017
Reticular Chemistry for Highly Porous Metal–Organic Frameworks: The Chemistry and Applications Chen, Zhijie; Kirlikovali, Kent O.; Li, Peng Accounts of Chemical Research, Vol. 55, Issue 4 https://doi.org/10.1021/acs.accounts.1c00707	journal	February 2022
Understanding the Adsorption of PFOA on MIL-101(Cr)-Based Anionic-Exchange Metal–Organic Frameworks: Comparing DFT Calculations with Aqueous Sorption Experiments Liu, Kai; Zhang, Siyu; Hu, Xiyue Environmental Science & Technology, Vol. 49, Issue 14 https://doi.org/10.1021/acs.est.5b00802	journal	July 2015
Making large single crystals of 2D MOFs Dong, Renhao; Feng, Xinliang Nature Materials, Vol. 20, Issue 2 https://doi.org/10.1038/s41563-020-00912-1	journal	January 2021
Cooperative insertion of CO2 in diamine-appended metal-organic frameworks McDonald, Thomas M.; Mason, Jarad A.; Kong, Xueqian Nature, Vol. 519, Issue 7543 https://doi.org/10.1038/nature14327	journal	March 2015
Confined water–encapsulated activated carbon for capturing short-chain perfluoroalkyl and polyfluoroalkyl substances from drinking water Shi, Yuanji; Mu, Hongxin; You, Jiaqian Proceedings of the National Academy of Sciences, Vol. 120, Issue 27 https://doi.org/10.1073/pnas.2219179120	journal	June 2023
Taming Multiscale Structural Complexity in Porous Skeletons: From Open Framework Materials to Micro/Nanoscaffold Architectures Liu, Hao; Yao, Yifan; Samorì, Paolo Small Methods, Vol. 7, Issue 10 https://doi.org/10.1002/smtd.202300468	journal	July 2023
Accelerated crystallization of zeolites via hydroxyl free radicals Feng, Guodong; Cheng, Peng; Yan, Wenfu Science, Vol. 351, Issue 6278 https://doi.org/10.1126/science.aaf1559	journal	March 2016
Introduction to Metal–Organic Frameworks Zhou, Hong-Cai; Long, Jeffrey R.; Yaghi, Omar M. Chemical Reviews, Vol. 112, Issue 2, p. 673-674 https://doi.org/10.1021/cr300014x	journal	September 2011
Insights to perfluorooctanoic acid adsorption micro-mechanism over Fe-based metal organic frameworks: Combining computational calculation with response surface methodology Yang, Yiqiong; Zheng, Zenghui; Ji, Wenqing Journal of Hazardous Materials, Vol. 395 https://doi.org/10.1016/j.jhazmat.2020.122686	journal	August 2020
Improving Ethane/Ethylene Separation Performance of Isoreticular Metal–Organic Frameworks via Substituent Engineering Zhou, Ping; Yue, Lianglan; Wang, Xinxin ACS Applied Materials & Interfaces, Vol. 13, Issue 45 https://doi.org/10.1021/acsami.1c17818	journal	November 2021
Installation of synergistic binding sites onto porous organic polymers for efficient removal of perfluorooctanoic acid Liu, Xiongli; Zhu, Changjia; Yin, Jun Nature Communications, Vol. 13, Issue 1 https://doi.org/10.1038/s41467-022-29816-1	journal	April 2022
Removal and destruction of perfluoroalkyl ether carboxylic acids (PFECAs) in an anion exchange resin and electrochemical oxidation treatment train Fang, Yida; Meng, Pingping; Schaefer, Charles Water Research, Vol. 230 https://doi.org/10.1016/j.watres.2022.119522	journal	February 2023
Imparting Selective Fluorophilic Interactions in Redox Copolymers for the Electrochemically Mediated Capture of Short-Chain Perfluoroalkyl Substances Román Santiago, Anaira; Yin, Song; Elbert, Johannes Journal of the American Chemical Society, Vol. 145, Issue 17 https://doi.org/10.1021/jacs.2c10963	journal	March 2023
Efficient Recognition and Removal of Persistent Organic Pollutants by a Bifunctional Molecular Material Chen, Zhonghang; Lu, Yi-Lin; Wang, Liang Journal of the American Chemical Society, Vol. 145, Issue 1 https://doi.org/10.1021/jacs.2c09866	journal	December 2022
Lining up metal–organic frameworks Champness, Neil R. Nature Materials, Vol. 16, Issue 3 https://doi.org/10.1038/nmat4859	journal	February 2017
The Chemistry and Applications of Metal-Organic Frameworks Furukawa, H.; Cordova, K. E.; O'Keeffe, M. Science, Vol. 341, Issue 6149, p. 1230444-1230444 https://doi.org/10.1126/science.1230444	journal	August 2013
Linker Desymmetrization: Access to a Series of Rare-Earth Tetracarboxylate Frameworks with Eight-Connected Hexanuclear Nodes Lv, Xiu-Liang; Feng, Liang; Xie, Lin-Hua Journal of the American Chemical Society, Vol. 143, Issue 7 https://doi.org/10.1021/jacs.0c11546	journal	January 2021
Improving MOF stability: approaches and applications Ding, Meili; Cai, Xuechao; Jiang, Hai-Long Chemical Science, Vol. 10, Issue 44 https://doi.org/10.1039/C9SC03916C	journal	January 2019
Functionalization of Zirconium‐Based Metal–Organic Layers with Tailored Pore Environments for Heterogeneous Catalysis Qiao, Guan‐Yu; Yuan, Shuai; Pang, Jiandong Angewandte Chemie International Edition, Vol. 59, Issue 41 https://doi.org/10.1002/anie.202007781	journal	August 2020
Unique fluorophilic pores engineering within porous aromatic frameworks for trace perfluorooctanoic acid removal Zhang, Chi; Dong, Junchao; Zhang, Panpan National Science Review, Vol. 10, Issue 10 https://doi.org/10.1093/nsr/nwad191	journal	July 2023
Endowing Porphyrinic Metal–Organic Frameworks with High Stability by a Linker Desymmetrization Strategy Han, Wentao; Ma, Xing; Wang, Jingxue Journal of the American Chemical Society, Vol. 145, Issue 17 https://doi.org/10.1021/jacs.3c00957	journal	April 2023
Could the world go PFAS-free? Proposal to ban ‘forever chemicals’ fuels debate Lim, XiaoZhi Nature, Vol. 620, Issue 7972 https://doi.org/10.1038/d41586-023-02444-5	journal	August 2023
The regulation of endocrine-disrupting chemicals to minimize their impact on health Duh-Leong, Carol; Maffini, Maricel V.; Kassotis, Christopher D. Nature Reviews Endocrinology, Vol. 19, Issue 10 https://doi.org/10.1038/s41574-023-00872-x	journal	August 2023
Molecular Cu Electrocatalyst Escalates Ambient Perfluorooctanoic Acid Degradation Sinha, Soumalya; Chaturvedi, Ashwin; Gautam, Rajeev K. Journal of the American Chemical Society, Vol. 145, Issue 50 https://doi.org/10.1021/jacs.3c08352	journal	December 2023

Similar Records

Zirconium‐Based Metal–Organic Frameworks with Free Hydroxy Groups for Enhanced Perfluorooctanoic Acid Uptake in Water

Journal Article · 2024 · Advanced Materials · OSTI ID:2377866

Liang, Rong‐Ran; Yang, Yihao; Han, Zongsu; +5 more

A New Class of Metal-Cyclam-Based Zirconium Metal–Organic Frameworks for CO₂ Adsorption and Chemical Fixation

Journal Article · 2017 · Journal of the American Chemical Society · OSTI ID:1421945

Zhu, Jie; Usov, Pavel M.; Xu, Wenqian; +10 more

A high surface area Zr(IV)-based metal–organic framework showing stepwise gas adsorption and selective dye uptake

Journal Article · 2015 · Journal of Solid State Chemistry · OSTI ID:22475543

Lv, Xiu-Liang; Tong, Minman; Huang, Hongliang; +5 more

Title: Exceptionally High Perfluorooctanoic Acid Uptake in Water by a Zirconium-Based Metal–Organic Framework through Synergistic Chemical and Physical Adsorption

Citation Formats

References (41)

Similar Records

Related Subjects