DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Quantum simulation of an extended Dicke model with a magnetic solid

Journal Article · · Communications Materials
; ORCiD logo; ORCiD logo; ; ORCiD logo; ORCiD logo; ; ORCiD logo; ; ORCiD logo; ORCiD logo; ORCiD logo; ORCiD logo; ORCiD logo; ORCiD logo; ORCiD logo

Abstract The Dicke model describes the cooperative interaction of an ensemble of two-level atoms with a single-mode photonic field and exhibits a quantum phase transition as a function of light–matter coupling strength. Extending this model by incorporating short-range atom–atom interactions makes the problem intractable but is expected to produce new physical phenomena and phases. Here, we simulate such an extended Dicke model using a crystal of ErFeO 3 , where the role of atoms (photons) is played by Er 3+ spins (Fe 3+ magnons). Through terahertz spectroscopy and magnetocaloric effect measurements as a function of temperature and magnetic field, we demonstrated the existence of a novel atomically ordered phase in addition to the superradiant and normal phases that are expected from the standard Dicke model. Further, we elucidated the nature of the phase boundaries in the temperature–magnetic-field phase diagram, identifying both first-order and second-order phase transitions. These results lay the foundation for studying multiatomic quantum optics models using well-characterized many-body solid-state systems.

Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
SC0012311
OSTI ID:
2327071
Journal Information:
Communications Materials, Journal Name: Communications Materials Journal Issue: 1 Vol. 5; ISSN 2662-4443
Publisher:
Nature Publishing GroupCopyright Statement
Country of Publication:
United Kingdom
Language:
English

References (48)

Quantum phase transition for the Dicke model with the dipole–dipole interactions journal August 2006
Laser phase and amplitude fluctuations in the fluorescent Dicke model of interacting atoms journal May 1985
Ultrastrong coupling regimes of light-matter interaction journal June 2019
Review of Recent Work on the Magnetic and Spectroscopic Properties of the Rare‐Earth Orthoferrites journal March 1969
Resonance and high frequency susceptibility in canted antiferromagnetic substances journal May 1963
A reliable method for extraction of material parameters in terahertz time-domain spectroscopy journal January 1996
First-Order Quantum Phase Transition for Dicke Model Induced by Atom-Atom Interaction journal May 2017
Field-induced quantum critical point in the itinerant antiferromagnet Ti3Cu4 journal May 2022
Quantum phases in circuit QED with a superconducting qubit array journal February 2014
Observation of the Magnonic Dicke Superradiant Phase Transition preprint January 2024
Phase Transition in the Dicke Model of Superradiance journal March 1973
Quantum Chaos in the Extended Dicke Model journal October 2022
Ultrastrong coupling between light and matter journal January 2019
Emergent Universality in a Quantum Tricritical Dicke Model journal May 2019
Influence of the demagnetizing factor on the magnetocaloric effect: Critical scaling and numerical simulations journal June 2014
Spin-reorientation transitions in rare-earth magnets journal July 1976
The Dicke model in quantum optics: Dicke model revisited journal March 2011
Coupled spin waves and crystalline electric field levels in candidate multiferroic ErFeO 3 journal July 2021
High Magnetic Field Studies of the Hidden Order Transition in U R u 2 S i 2 journal December 2002
Ground-state properties for coupled Bose-Einstein condensates inside a cavity quantum electrodynamics journal October 2007
Classical dynamics of a two-species condensate driven by a quantum field journal July 2011
Temporal evolution of superradiance in a small sphere journal November 1974
Entanglement and the Phase Transition in Single-Mode Superradiance journal February 2004
Ultrastrong magnon–magnon coupling dominated by antiresonant interactions journal May 2021
Observation of Dicke cooperativity in magnetic interactions journal August 2018
Terahertz spin dynamics in rare-earth orthoferrites journal January 2022
Critical Phenomena in Light–Matter Systems with Collective Matter Interactions journal August 2022
Coherence in Spontaneous Radiation Processes journal January 1954
Universally Diverging Grüneisen Parameter and the Magnetocaloric Effect Close to Quantum Critical Points journal August 2003
Sign change of the Grüneisen parameter and magnetocaloric effect near quantum critical points journal November 2005
Perfect intrinsic squeezing at the superradiant phase transition critical point journal February 2023
Critical phenomena in an extended Dicke model journal October 2018
On the superradiant phase transition for molecules in a quantized radiation field: the dicke maser model journal April 1973
Ground state in the finite Dicke model for interacting qubits journal March 2015
Relation between the specific heat and susceptibility of an antiferromagnet journal October 1962
The magnetic structures and transitions of a potential multiferroic orthoferrite ErFeO 3 journal April 2015
Dicke superradiance in solids [Invited] journal January 2016
Quantum phase transitions in coupled two-level atoms in a single-mode cavity journal November 2010
Quantum Chaos and Effective Thermalization journal February 2012
Critical properties of entanglement in the Dicke model with the dipole–dipole interactions journal April 2009
Ising model in a light-induced quantized transverse field journal May 2020
First-Order Superradiant Phase Transitions in a Multiqubit Cavity System journal August 2004
Circuit QED and Sudden Phase Switching in a Superconducting Qubit Array journal October 2010
Quantum critical detector: amplifying weak signals using discontinuous quantum phase transitions journal April 2019
Quantum Chaos Triggered by Precursors of a Quantum Phase Transition: The Dicke Model journal January 2003
Magnonic superradiant phase transition journal January 2022
Quantum-optical properties of polariton waves journal August 1991
Submillimeter Spectroscopy of Antiferromagnetic Dielectrics: Rare-Earth Orthoferrites book August 1995