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Title: Physical science research needed to evaluate the viability and risks of marine cloud brightening

Journal Article · · Science Advances
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  1. National Oceanic and Atmospheric Administration (NOAA), Boulder, CO (United States)
  2. Argonne National Laboratory (ANL), Argonne, IL (United States)
  3. University of California, San Diego, CA (United States). Scripps Inst. of Oceanography
  4. University of Washington, Seattle, WA (United States)
  5. Michigan Technological University, Houghton, MI (United States)
  6. Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
  7. Florida State University, Tallahassee, FL (United States)
  8. Delft University of Technology (Netherlands)
  9. Imperial College, London (United Kingdom)
  10. University of Exeter, Devon (United Kingdom)
  11. Ludwig Maximilian University of Munich, Munich (Germany)
  12. California Institute of Technology (CalTech), Pasadena, CA (United States)
  13. National Center for Atmospheric Research (NCAR), Boulder, CO (United States)
  14. University of Wyoming, Laramie, WY (United States)
  15. Boston College, Chestnut Hill, MA (United States)
  16. Goethe Univerity, Frankfurt (Germany)
  17. National Oceanic and Atmospheric Administration (NOAA), Boulder, CO (United States). NOAA Chemical Sciences Laboratory (CSL); Univ. of Colorado, Boulder, CO (United States). Cooperative Inst. for Research in Environmental Sciences (CIRES)
  18. National Oceanic and Atmospheric Administration (NOAA), Seattle, WA (United States). Pacific Marine Environmental Lab. (PMEL)
  19. University of Colorado, Boulder, CO (United States)
  20. University of Arizona, Tucson, AZ (United States)
  21. University of Tartu (Estonia)
  22. Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)

Marine cloud brightening (MCB) is the deliberate injection of aerosol particles into shallow marine clouds to increase their reflection of solar radiation and reduce the amount of energy absorbed by the climate system. From the physical science perspective, the consensus of a broad international group of scientists is that the viability of MCB will ultimately depend on whether observations and models can robustly assess the scale-up of local-to-global brightening in today’s climate and identify strategies that will ensure an equitable geographical distribution of the benefits and risks associated with projected regional changes in temperature and precipitation. To address the physical science knowledge gaps required to assess the societal implications of MCB, we propose a substantial and targeted program of research—field and laboratory experiments, monitoring, and numerical modeling across a range of scales.

Research Organization:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States); Argonne National Laboratory (ANL), Argonne, IL (United States); Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States); Brookhaven National Laboratory (BNL), Upton, NY (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Biological and Environmental Research (BER); National Oceanic and Atmospheric Administration (NOAA); National Science Foundation (NSF); National Aeronautics and Space Administration (NASA); USDOE National Nuclear Security Administration (NNSA)
Grant/Contract Number:
AC02-06CH11357; SC0022227; SC0012704; SC0022958; AC06-76RL01830; AC52-07NA27344; SC0021045; AGS-2133229; AC05-76RL01830
OSTI ID:
2326934
Alternate ID(s):
OSTI ID: 2328494; OSTI ID: 2331522; OSTI ID: 2333673; OSTI ID: 2447749
Report Number(s):
LLNL-JRNL-853525; PNNL-SA-189954; BNL-225445-2024-JAAM
Journal Information:
Science Advances, Vol. 10, Issue 12; ISSN 2375-2548
Publisher:
AAASCopyright Statement
Country of Publication:
United States
Language:
English

References (116)

Local closure during the First Aerosol Characterization Experiment (ACE 1): Aerosol mass concentration and scattering and backscattering coefficients journal July 1998
Elucidating the Role of Anthropogenic Aerosols in Arctic Sea Ice Variations journal January 2018
To assess marine cloud brightening's technical feasibility, we need to know what to study—and when to stop journal January 2022
Evaporative Cooling Does Not Prevent Vertical Dispersion of Effervescent Seawater Aerosol for Brightening Clouds journal November 2023
Top-down and bottom-up aerosol–cloud closure: towards understanding sources of uncertainty in deriving cloud shortwave radiative flux journal August 2017
Bounding global aerosol radiative forcing of climate change journal November 2019
Detection of large-scale cloud microphysical changes within a major shipping corridor after implementation of the International Maritime Organization 2020 fuel sulfur regulations journal July 2023
The effects of timing and rate of marine cloud brightening aerosol injection on albedo changes during the diurnal cycle of marine stratocumulus clouds journal February 2013
On the efficiency of nucleation scavenging journal November 1984
On the reversibility of transitions between closed and open cellular convection journal January 2015
Cloud Property Retrievals in the ARM Program journal April 2016
Manipulating marine stratocumulus cloud amount and albedo: a process-modelling study of aerosol-cloud-precipitation interactions in response to injection of cloud condensation nuclei journal January 2011
Cloud droplet sedimentation, entrainment efficiency, and subtropical stratocumulus albedo journal January 2007
Deconvolution of boundary layer depth and aerosol constraints on cloud water path in subtropical stratocumulus decks journal January 2020
Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA) journal February 2022
Diurnal Cycles of Cumulus, Cumulonimbus, Stratus, Stratocumulus, and Fog from Surface Observations over Land and Ocean journal March 2014
Aerosols, Cloud Microphysics, and Fractional Cloudiness journal September 1989
Assessing the potential efficacy of marine cloud brightening for cooling Earth using a simple heuristic model journal January 2021
Microphysical, macrophysical, and radiative responses of subtropical marine clouds to aerosol injections journal January 2023
Morning-to-Afternoon Evolution of Marine Stratus Polluted by Underlying Ships: Implications for the Relative Lifetimes of Polluted and Unpolluted Clouds journal July 2009
Evaluation of Pulse Aerosol Forcing on Marine Stratocumulus Clouds in the Context of Marine Cloud Brightening journal June 2023
Aerosols enhance cloud lifetime and brightness along the stratus-to-cumulus transition journal July 2020
Occurrence of lower cloud albedo in ship tracks journal January 2012
Invisible ship tracks show large cloud sensitivity to aerosol journal October 2022
Turbulence, Condensation, and Liquid Water Transport in Numerically Simulated Nonprecipitating Stratocumulus Clouds journal January 2003
Estimating and tracking the remaining carbon budget for stringent climate targets journal July 2019
Weak average liquid-cloud-water response to anthropogenic aerosols journal July 2019
Meteorological Conditions Favorable for Strong Anthropogenic Aerosol Impacts on Clouds journal February 2022
Observing the timescales of aerosol–cloud interactions in snapshot satellite images journal January 2021
Ship trails and ship induced cloud dynamics journal January 1990
Problems Connected with the Condensation and Precipitation Processes in the Atmosphere * journal April 1938
Observing short timescale cloud development to constrain aerosol-cloud interactions preprint May 2022
Variability of Surface Radiation Budget Components Over the U.S. From 1996 to 2019—Has Brightening Ceased? journal April 2021
Aerosol–Cloud–Meteorology Interaction Airborne Field Investigations: Using Lessons Learned from the U.S. West Coast in the Design of ACTIVATE off the U.S. East Coast journal August 2019
The Seasonal Cycle of Low Stratiform Clouds journal August 1993
Effects of intermittent aerosol forcing on the stratocumulus-to-cumulus transition journal February 2024
Impact of global dimming and brightening on global warming journal January 2007
Constraining the aerosol influence on cloud liquid water path journal January 2019
ARM Solar and Infrared Broadband and Filter Radiometry journal April 2016
Geoengineering by cloud seeding: influence on sea ice and climate system journal October 2009
Beyond SO x reductions from shipping: assessing the impact of NO x and carbonaceous-particle controls on human health and climate journal December 2020
Emissions from Ships with respect to Their Effects on Clouds journal August 2000
Climate Impact of Biofuels in Shipping: Global Model Studies of the Aerosol Indirect Effect journal April 2011
An Intercomparison of Large‐Eddy Simulations of a Convection Cloud Chamber Using Haze‐Capable Bin and Lagrangian Cloud Microphysics Schemes journal April 2023
A multiyear tropical Pacific cooling response to recent Australian wildfires in CESM2 journal May 2023
The Geoengineering Model Intercomparison Project (GeoMIP) journal January 2011
Scaling of Turbulence and Microphysics in a Convection–Cloud Chamber of Varying Height journal February 2023
Climate intervention using marine cloud brightening (MCB) compared with stratospheric aerosol injection (SAI) in the UKESM1 climate model journal December 2023
Marine cloud brightening – as effective without clouds journal January 2017
Nonlinear climate response to regional brightening of tropical marine stratocumulus: CLIMATE RESPONSE TO CLOUD BRIGHTENING journal August 2012
Untangling causality in midlatitude aerosol–cloud adjustments journal April 2020
Observations of clouds, aerosols, precipitation, and surface radiation over the Southern Ocean: An overview of CAPRICORN, MARCUS, MICRE and SOCRATES journal November 2020
Limits to the Aerosol Indirect Radiative Effect Derived from Observations of Ship Tracks journal February 2002
The Appearance and Disappearance of Ship Tracks on Large Spatial Scales journal August 2000
Studying geoengineering with natural and anthropogenic analogs journal May 2013
Three Different Behaviors of Liquid Water Path of Water Clouds in Aerosol–Cloud Interactions journal February 2002
Hydrological Consequences of Solar Geoengineering journal May 2023
Anomalous Cloud Lines journal November 1966
Segmentation-based multi-pixel cloud optical thickness retrieval using a convolutional neural network journal September 2022
The Dependence of Ship‐Polluted Marine Cloud Properties and Radiative Forcing on Background Drop Concentrations journal April 2021
Machine learning reveals climate forcing from aerosols is dominated by increased cloud cover journal August 2022
The inclusion of water with the injected aerosol reduces the simulated effectiveness of marine cloud brightening journal May 2013
Aerosol dynamics in ship tracks journal December 1999
Simulating Aerosol Lifecycle Impacts on the Subtropical Stratocumulus‐to‐Cumulus Transition Using Large‐Eddy Simulations journal October 2022
Response to marine cloud brightening in a multi-model ensemble journal January 2018
Eastern Pacific Emitted Aerosol Cloud Experiment journal May 2013
Shipping regulations lead to large reduction in cloud perturbations journal October 2022
Comparison of Measurements of Cloud Droplets and Cloud Nuclei journal November 1967
Ocean–Cloud–Atmosphere–Land Interactions in the Southeastern Pacific: The VOCALS Program journal March 2014
The impact of humidity above stratiform clouds on indirect aerosol climate forcing journal December 2004
Control of global warming? journal September 1990
Large eddy simulation of ship tracks in the collapsed marine boundary layer: a case study from the Monterey area ship track experiment journal January 2015
Monitoring global carbon emissions in 2022 journal March 2023
The Impact of Resolving Subkilometer Processes on Aerosol‐Cloud Interactions of Low‐Level Clouds in Global Model Simulations journal November 2020
Modeling Mesoscale Cellular Structures and Drizzle in Marine Stratocumulus. Part I: Impact of Drizzle on the Formation and Evolution of Open Cells journal November 2009
Aerosol Effects on Clouds, Precipitation, and the Organization of Shallow Cumulus Convection journal February 2008
Regionally refined test bed in E3SM atmosphere model version 1 (EAMv1) and applications for high-resolution modeling journal January 2019
Crop failure rates in a geoengineered climate: impact of climate change and marine cloud brightening journal August 2015
Multisensor satellite observations of aerosol effects on warm clouds journal January 2008
Effects of ship emissions on sulphur cycling and radiative climate forcing over the ocean journal August 1999
Microphysical, macrophysical and radiative signatures of volcanic aerosols in trade wind cumulus observed by the A-Train journal January 2011
Large-scale interventions may delay decline of the Great Barrier Reef journal April 2021
Aerosol-cloud-climate cooling overestimated by ship-track data journal January 2021
The Large-Eddy Simulation (LES) Atmospheric Radiation Measurement (ARM) Symbiotic Simulation and Observation (LASSO) Activity for Continental Shallow Convection journal April 2020
Can marine cloud brightening reduce coral bleaching?: Can marine cloud brightening reduce coral bleaching? journal June 2013
Direct and Remote Sensing Observations of the Effects of Ships on Clouds journal December 1989
Corrigendum to "Aerosol indirect effects from shipping emissions: sensitivity studies with the global aerosol-climate model ECHAM-HAM" published in Atmos. Chem. Phys., 12, 5985–6007, 2012 journal January 2013
Global model simulations of the impact of ocean-going ships on aerosols, clouds, and the radiation budget journal January 2007
Importance of vertical velocity variations in the cloud droplet nucleation process of marine stratus clouds journal January 2005
Processes limiting the emergence of detectable aerosol indirect effects on tropical warm clouds in global aerosol-climate model and satellite data journal January 2014
Observations of a substantial cloud-aerosol indirect effect during the 2014-2015 Bárðarbunga-Veiðivötn fissure eruption in Iceland: VOLCANIC CLOUD-AEROSOL EFFECT journal December 2015
Opportunistic experiments to constrain aerosol effective radiative forcing journal January 2022
The Monterey Area Ship Track Experiment journal August 2000
Robust evidence for reversal of the trend in aerosol effective climate forcing journal September 2022
Aerosol-cloud drop concentration closure for clouds sampled during the International Consortium for Atmospheric Research on Transport and Transformation 2004 campaign: AEROSOL-CLOUD DROP CLOSURE journal April 2007
Evaluating climate geoengineering proposals in the context of the Paris Agreement temperature goals journal September 2018
Strong constraints on aerosol–cloud interactions from volcanic eruptions journal June 2017
Marine Cloud Brightening: an airborne concept preprint August 2023
Distinct regional meteorological influences on low-cloud albedo susceptibility over global marine stratocumulus regions journal January 2023
Cleaner fuels for ships provide public health benefits with climate tradeoffs journal February 2018
The efficacy of aerosol–cloud radiative perturbations from near-surface emissions in deep open-cell stratocumuli journal January 2018
Substantial Cloud Brightening From Shipping in Subtropical Low Clouds journal March 2020
Climate impacts of geoengineering marine stratocumulus clouds journal January 2009
Cloud–Aerosol–Turbulence Interactions: Science Priorities and Concepts for a Large-Scale Laboratory Facility journal July 2020
Detection limits of albedo changes induced by climate engineering journal January 2014
Global ship track distribution and radiative forcing from 1 year of AATSR data journal January 2007
DOE-NOAA Marine Cloud Brightening Workshop report November 2022
A Laboratory Facility to Study Gas–Aerosol–Cloud Interactions in a Turbulent Environment: The Π Chamber journal December 2016
Global reduction in ship-tracks from sulfur regulations for shipping fuel journal July 2022
Cloud Microphysical Implications for Marine Cloud Brightening: The Importance of the Seeded Particle Size Distribution journal October 2021
Tropical South Atlantic influence on Northeastern Brazil precipitation and ITCZ displacement during the past 2300 years journal February 2019
Near‐Cloud Aerosol Retrieval Using Machine Learning Techniques, and Implied Direct Radiative Effects journal October 2022
Pollution and the planetary albedo journal December 1974
Atmospheric circulation as a source of uncertainty in climate change projections journal September 2014
Albedo susceptibility of northeastern Pacific stratocumulus: the role of covarying meteorological conditions journal January 2022
Could geoengineering research help answer one of the biggest questions in climate science?: GEOENGINEERING RESEARCH journal July 2017