Spatiotemporal dispersion compensation for a 200-THz noncollinear optical parametric amplifier

Carbery, William P.; Bizimana, Laurie A.; Barclay, Matthew S.; Wright, Nicholas D.; Davis, Paul H.; Knowlton, William B.; Pensack, Ryan D.; Arpin, Paul C.; Turner, Daniel B.

doi:10.1063/5.0187338

Title: Spatiotemporal dispersion compensation for a 200-THz noncollinear optical parametric amplifier

Journal Article · 04 March 2024 · Review of Scientific Instruments

DOI: https://doi.org/10.1063/5.0187338 · OSTI ID:2323916

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New York University, NY (United States); Boise State University
New York University, NY (United States)
Boise State University, ID (United States)
Boise State University, ID (United States); Center for Advanced Energy Studies, Idaho Falls, ID (United States)
California State University, Chico, CA (United States)
New York University, NY (United States); Boise State University, ID (United States)

A noncollinear optical parametric amplifier (NOPA) can produce few-cycle femtosecond laser pulses that are ideally suited for time-resolved optical spectroscopy measurements. However, the nonlinear-optical process giving rise to ultrabroadband pulses is susceptible to spatiotemporal dispersion problems. Here, we detail refinements, including chirped-pulse amplification (CPA) and pulse-front matching (PFM), that minimize spatiotemporal dispersion and thereby improve the properties of ultrabroadband pulses produced by a NOPA. Here, the description includes a rationale behind the choices of optical and optomechanical components, as well as assessment protocols. We demonstrate these techniques using a 1 kHz, second-harmonic Ti:sapphire pump configuration, which produces ~5-fs duration pulses that span from about 500 to 800 nm with a bandwidth of about 200 THz. To demonstrate the utility of the CPA-PFM-NOPA, we measure vibrational quantum beats in the transient–absorption spectrum of methylene blue, a dye molecule that serves as a reference standard.

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Research Organization:: Boise State University, ID (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE)

Grant/Contract Number:: SC0020089

OSTI ID:: 2323916

Journal Information:: Review of Scientific Instruments, Journal Name: Review of Scientific Instruments Journal Issue: 3 Vol. 95; ISSN 0034-6748

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

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Noncollinear optical parametric amplifier (NOPA)
Chirped-pulse amplification (CPA)
Pulse-front matching (PFM)
Ultrabroadband pulses
Time-resolved optical spectroscopy

Title: Spatiotemporal dispersion compensation for a 200-THz noncollinear optical parametric amplifier

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