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Title: Kondo effect and its destruction in heterobilayer transition metal dichalcogenides

Journal Article · · Physical Review Research

Moiré structures, along with line-graph-based d -electron systems, represent a setting to realize flat bands. One form of the associated strong correlation physics is the Kondo effect. Here, we address the recently observed Kondo-driven heavy fermion state and its destruction in AB-stacked hetero-bilayer transition metal dichalcogenides, which can be controlled by the gate voltages. By studying an effective interacting Hamiltonian using the slave spin approach, we obtained a phase diagram with the total filling factor and the displacement field strength as the tunable parameters. In an extended range of the tunable displacement field, our numerical results show that the relative filling of the d orbital, which is associated with the highest moiré band from the MoTe 2 layer, is enforced to be ν d 1 by the interaction. This agrees with the experimental observation. We also argue that the observed high coherence temperature scale could be explained by the non-negligible bandwidth of the d orbital. Our results set the stage to address the amplified quantum fluctuations that the Kondo effect may produce in these structures and new regimes that the systems open up for Kondo-destruction quantum criticality. Published by the American Physical Society 2024

Sponsoring Organization:
USDOE
Grant/Contract Number:
SC0018197
OSTI ID:
2315739
Journal Information:
Physical Review Research, Journal Name: Physical Review Research Vol. 6 Journal Issue: 1; ISSN 2643-1564
Publisher:
American Physical SocietyCopyright Statement
Country of Publication:
United States
Language:
English

References (76)

Periodic Anderson model with correlated conduction electrons journal September 1997
Some comments on Kondo lattices and the Mott transition journal December 1998
Mott transition in multiorbital models for iron pnictides journal December 2011
Signatures of fractional quantum anomalous Hall states in twisted MoTe2 journal June 2023
Hall-effect evolution across a heavy-fermion quantum critical point journal December 2004
Quantum Anomalous Hall Effect from Inverted Charge Transfer Gap journal May 2022
A Drastic Change of the Fermi Surface at a Critical Pressure in CeRhIn 5 : dHvA Study under Pressure journal April 2005
Coherence Scale of the Kondo Lattice journal July 2000
Excitonic Chern insulator and kinetic ferromagnetism in a MoTe2/WSe2 moiré bilayer journal February 2023
Unconventional superconductivity in magic-angle graphene superlattices journal March 2018
Hubbard Model Physics in Transition Metal Dichalcogenide Moiré Bands journal July 2018
Maximally localized Wannier functions: Theory and applications journal October 2012
Exploring heavy fermions from macroscopic to microscopic length scales journal August 2016
Continuous Mott transition in semiconductor moiré superlattices journal September 2021
Quantum criticality and global phase diagram of magnetic heavy fermions journal March 2010
Detaching the antiferromagnetic quantum critical point from the Fermi-surface reconstruction in YbRh2Si2 journal May 2009
Quantum anomalous Hall effect from intertwined moiré bands journal December 2021
Kondo phase in twisted bilayer graphene journal January 2024
Chiral Kondo lattice in doped MoTe 2 /WSe 2 bilayers journal March 2023
Magnetic-Field Induced Quantum Critical Point in Y b R h 2 S i 2 journal July 2002
Magic-angle twisted symmetric trilayer graphene as a topological heavy-fermion problem journal July 2023
k · p theory for two-dimensional transition metal dichalcogenide semiconductors journal April 2015
Topological Superconductivity in Doped Magnetic Moiré Semiconductors journal August 2023
Quantum phases driven by strong correlations journal December 2020
Three-band tight-binding model for monolayers of group-VIB transition metal dichalcogenides journal August 2013
Hartree-Fock study of the moiré Hubbard model for twisted bilayer transition metal dichalcogenides journal August 2021
Spin-orbit coupling in transition metal dichalcogenide heterobilayer flat bands journal May 2022
Quantum Phases of the Shastry-Sutherland Kondo Lattice: Implications for the Global Phase Diagram of Heavy-Fermion Metals journal October 2014
Quantum criticality in twisted transition metal dichalcogenides journal September 2021
Nonlocal Interactions in Moiré Hubbard Systems journal May 2022
Coupled topological flat and wide bands: Quasiparticle formation and destruction journal July 2023
Kondo Insulator to Semimetal Transformation Tuned by Spin-Orbit Coupling journal June 2017
Frustration and the Kondo Effect in Heavy Fermion Materials journal September 2010
Gate-tunable heavy fermion quantum criticality in a moiré Kondo lattice journal July 2022
How do Fermi liquids get heavy and die? journal August 2001
Spin-textured Chern bands in AB-stacked transition metal dichalcogenide bilayers journal September 2021
Hopping frustration-induced flat band and strange metallicity in a kagome metal journal January 2024
Non-Fermi liquid behaviour in a correlated flat-band pyrochlore lattice journal January 2024
Topological Phases in AB-Stacked MoTe2/WSe2 : Z2 Topological Insulators, Chern Insulators, and Topological Charge Density Waves journal July 2022
Gate-tunable heavy fermions in a moiré Kondo lattice journal March 2023
Colloquium : Heavy-electron quantum criticality and single-particle spectroscopy journal March 2020
Shot noise in a strange metal journal November 2023
Kondo Destruction and Quantum Criticality in Kondo Lattice Systems journal June 2014
Weyl–Kondo semimetal in heavy-fermion systems journal December 2017
U ( 1 ) slave-spin theory and its application to Mott transition in a multiorbital model for iron pnictides journal August 2012
Composite Fermi Liquid at Zero Magnetic Field in Twisted MoTe2 journal September 2023
Orbitally selective Mott phase in electron-doped twisted transition metal-dichalcogenides: A possible realization of the Kondo lattice model journal December 2021
Onset of antiferromagnetism in heavy-fermion metals journal September 2000
Wannier90 as a community code: new features and applications journal January 2020
Isotropic quantum scattering and unconventional superconductivity journal November 2008
Topological quantum chemistry journal July 2017
Superconductivity in an extreme strange metal journal July 2021
Locally critical quantum phase transitions in strongly correlated metals journal October 2001
Moire bands in twisted double-layer graphene journal July 2011
Correlated insulator behaviour at half-filling in magic-angle graphene superlattices journal March 2018
Topological semimetal driven by strong correlations and crystalline symmetry journal September 2022
Model for a Ferromagnetic Quantum Critical Point in a 1D Kondo Lattice journal April 2018
Metallic ferromagnetism in the Kondo lattice journal August 2010
Dynamical Mean-Field Theory of Moiré Bilayer Transition Metal Dichalcogenides: Phase Diagram, Resistivity, and Quantum Criticality journal June 2022
Weak magnetism and non-Fermi liquids near heavy-fermion critical points journal January 2004
Emulating Heavy Fermions in Twisted Trilayer Graphene journal July 2021
Non-Fermi-Liquid Scaling of the Magnetic Response in UCu 5 − x Pd x ( x = 1 , 1.5 ) journal July 1995
Magic-Angle Twisted Bilayer Graphene as a Topological Heavy Fermion Problem journal July 2022
Metal-Insulator Transition in a Semiconductor Heterobilayer Model journal February 2024
Observation of fractionally quantized anomalous Hall effect journal August 2023
The Quantum Critical Point in CeRhIn 5 : A Resistivity Study journal November 2008
Kondo Lattice Model of Magic-Angle Twisted-Bilayer Graphene: Hund’s Rule, Local-Moment Fluctuations, and Low-Energy Effective Theory journal July 2023
Global magnetic phase diagram and local quantum criticality in heavy fermion metals journal May 2006
Kondo screening and coherence in kagome local-moment metals: Energy scales of heavy fermions in the presence of flat bands journal December 2023
Symmetric Kondo Lattice States in Doped Strained Twisted Bilayer Graphene journal October 2023
Kondo Lattice Model in Magic-Angle Twisted Bilayer Graphene journal July 2023
Slave spins away from half filling: Cluster mean-field theory of the Hubbard and extended Hubbard models journal January 2010
Observation of Integer and Fractional Quantum Anomalous Hall Effects in Twisted Bilayer MoTe2 journal September 2023
Singular charge fluctuations at a magnetic quantum critical point journal January 2020
Hidden magnetism and quantum criticality in the heavy fermion superconductor CeRhIn5 journal March 2006
Twisted bilayer graphene as topological heavy fermion: II. Analytical approximations of the model parameters journal June 2023