Quantifying the Entropy and Enthalpy of Insertion Materials for Battery Applications Via the Multi-Species, Multi-Reaction Model

Garrick, Taylor R.; Koch, Brian J.; Choi, Munnyeong; Du, Xiaoniu; Adeyinka, Adekanmi M.; Staser, John A.; Choe, Song-Yul

doi:10.1149/1945-7111/ad1d27

Title: Quantifying the Entropy and Enthalpy of Insertion Materials for Battery Applications Via the Multi-Species, Multi-Reaction Model

Journal Article · 07 February 2024 · Journal of the Electrochemical Society

DOI: https://doi.org/10.1149/1945-7111/ad1d27 · OSTI ID:2290426

; Koch, Brian J.; Choi, Munnyeong; Du, Xiaoniu; Adeyinka, Adekanmi M.;

; Choe, Song-Yul

The entropy coefficient of a battery cell is the property that governs the amount of reversible heat that is generated during operation. In this work, we propose an extension of the Multi-Species, Multi-Reaction (MSMR) model to capture the entropy coefficient of a large format lithium-ion battery cell. We utilize the hybridized time-frequency domain analysis (HTFDA) method using a multi-functional calorimeter to probe the entropy coefficient of a large format pouch type lithium-ion battery with a NMC 811 cathode and a graphite anode. The measured entropy coefficient profile of the battery cell is deconvoluted into an entropy coefficient for each active material, which is then estimated using an extension of the MSMR model. Finally, we extend the entropy of a material to individual entropy for each gallery as treated by the model.

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Sponsoring Organization:: USDOE

OSTI ID:: 2290426

Journal Information:: Journal of the Electrochemical Society, Journal Name: Journal of the Electrochemical Society Vol. 171 Journal Issue: 2; ISSN 0013-4651

Publisher:: The Electrochemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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