Aerosol‐Correlated Cloud Activation for Clean Conditions in the Tropical Atlantic Boundary Layer During LASIC

Dedrick, Jeramy L.; Russell, Lynn M.; Sedlacek, III, Arthur J.; Kuang, Chongai; Zawadowicz, Maria A.; Lubin, Dan

doi:10.1029/2023GL105798

Title: Aerosol‐Correlated Cloud Activation for Clean Conditions in the Tropical Atlantic Boundary Layer During LASIC

Journal Article · 02 February 2024 · Geophysical Research Letters

DOI: https://doi.org/10.1029/2023GL105798 · OSTI ID:2284006

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^[2]; Kuang, Chongai ^[2];

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Scripps Institution of Oceanography University of California San Diego La Jolla CA USA
Environmental and Climate Sciences Department Brookhaven National Laboratory Upton NY USA

Abstract Aerosol measurements during the DOE ARM Layered Atlantic Smoke Interactions with Clouds (LASIC) campaign were used to quantify the differences between clean and smoky cloud condensation nuclei (CCN) budgets. Accumulation‐mode particles accounted for ∼70% of CCN at supersaturations <0.3% in clean and smoky conditions. Aitken‐mode particles contributed <20% and sea‐spray‐mode particles <10% at supersaturations <0.3%, but at supersaturations >0.3% Aitken particles contributions increased to 30%–40% of clean CCN. For clean conditions, the Hoppel minimum diameter was correlated to the accumulation‐mode number concentration, indicating aerosol‐correlated cloud activation was controlling the lower diameter cutoff for which particles serve as CCN. For smoky conditions, the contributions of Aitken particles increase and the correlation of cloud activation to accumulation‐mode particles is masked by the lower‐hygroscopicity smoke. These results provide the first multi‐month in situ quantitative constraints on the role of aerosol number size distributions in controlling cloud activation in the tropical Atlantic boundary layer.

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Research Organization:: Brookhaven National Laboratory (BNL), Upton, NY (United States); Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Atmospheric Radiation Measurement (ARM) Data Center

Sponsoring Organization:: USDOE; USDOE Office of Science (SC), Biological and Environmental Research (BER)

Contributing Organization:: Argonne National Laboratory (ANL); Brookhaven National Laboratory (BNL); Pacific Northwest National Laboratory (PNNL)

Grant/Contract Number:: SC0012704; SC0021045

OSTI ID:: 2284006

Report Number(s):: BNL-225448-2024-JAAM; e2023GL105798

Journal Information:: Geophysical Research Letters, Journal Name: Geophysical Research Letters Journal Issue: 3 Vol. 51; ISSN 0094-8276

Publisher:: American Geophysical Union (AGU)Copyright Statement

Country of Publication:: United States

Language:: English

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Data from: Aerosol-Limited Effects on Cloud Condensation Nuclei in Clean Conditions in the Tropical South Atlantic Boundary Layer during LASIC Dedrick, Jeramy L.; Russell, Lynn M.; J., Sedlacek III, Arthur UC San Diego Library Digital Collections https://doi.org/10.6075/J0CN7432	dataset	January 2023
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