Title: On the mechanisms of J c increment and degradation in high-J c Ba122 tapes made by different processing methods

Journal Article · · Applied Physics Express

Abstract We compared the grain and grain boundary (GB) nanostructures in two Ba122 tapes with similarly high J c . The Ag-sheathed tape made by hot pressing has larger, more plate-like grains with better c -axis alignment but has more GBs blocked by FeAs and Ba–O. In contrast, the tape made by cold pressing with an Ag-Sn/stainless steel sheath possesses fewer plate-like grains and weaker grain alignment but has more continuous current paths with clean physically well-connected GBs. Our nanostructural comparison emphasizes the strong need to achieve both good grain alignment and clean GBs for further J c improvement of Ba122 tapes.

Research Organization:
Florida State Univ., Tallahassee, FL (United States)
Sponsoring Organization:
US National Science Foundation; USDOE; USDOE Office of Science (SC), High Energy Physics (HEP)
Grant/Contract Number:
SC0018750
OSTI ID:
2279102
Journal Information:
Applied Physics Express, Journal Name: Applied Physics Express Journal Issue: 1 Vol. 17; ISSN 1882-0778
Publisher:
IOP PublishingCopyright Statement
Country of Publication:
Japan
Language:
English

References (41)

Three-dimensional microstructure and critical current properties of ultrafine grain Ba(Fe,Co)2As2 bulk superconductors journal November 2022
Origin and elimination of excess iron particles in off-stoichiometric Ba0.6K0.5-βFe2As2+δ superconductors journal October 2023
The superconductivity at 18 K in LiFeAs system journal December 2008
Iron-Based Layered Superconductor La[O 1- x F x ]FeAs ( x = 0.05−0.12) with T c = 26 K journal March 2008
High-Tc superconducting materials for electric power applications journal November 2001
Advantageous grain boundaries in iron pnictide superconductors journal August 2011
Strongly enhanced flux pinning in one-step deposition of BaFe2(As0.66P0.33)2 superconductor films with uniformly dispersed BaZrO3 nanoparticles journal September 2013
High intergrain critical current density in fine-grain (Ba0.6K0.4)Fe2As2 wires and bulks journal May 2012
Approaching the ultimate superconducting properties of (Ba,K)Fe2As2 by naturally formed low-angle grain boundary networks journal October 2021
Effect of heat treatments on superconducting properties and connectivity in K-doped BaFe2As2 journal February 2021
Achievement of practical level critical current densities in Ba1−xKxFe2As2/Ag tapes by conventional cold mechanical deformation journal February 2014
Hot pressing to enhance the transport Jc of Sr0.6K0.4Fe2As2 superconducting tapes journal November 2014
Development of very high Jc in Ba(Fe1-xCox)2As2 thin films grown on CaF2 journal December 2014
Large transport Jc in Cu-sheathed Sr0.6K0.4Fe2As2 superconducting tape conductors journal June 2015
Effects of introducing isotropic artificial defects on the superconducting properties of differently doped Ba-122 based single crystals journal June 2016
Intergrain current flow in a randomly oriented polycrystalline SmFeAsO0.85 oxypnictide journal October 2009
Weak-link behavior of grain boundaries in superconducting Ba(Fe1−xCox)2As2 bicrystals journal November 2009
Realization of practical level current densities in Sr 0.6 K 0.4 Fe 2 As 2 tape conductors for high-field applications journal May 2014
Evidence for composition variations and impurity segregation at grain boundaries in high current-density polycrystalline K- and Co-doped BaFe 2 As 2 superconductors journal October 2014
Superconductivity in the PbO-type structure  -FeSe journal September 2008
The behavior of grain boundaries in the Fe-based superconductors journal November 2011
Mechanochemical synthesis of pnictide compounds and superconducting Ba 0.6 K 0.4 Fe 2 As 2 bulks with high critical current density journal May 2013
Enhancement of critical current densities in (Ba,K)Fe 2 As 2 wires and tapes using HIP technique journal September 2016
High critical current density over 1 MA cm −2 at 13 T in BaZrO 3 incorporated Ba(Fe,Co) 2 As 2 thin film journal July 2017
High transport J c in stainless steel/Ag-Sn double sheathed Ba122 tapes journal August 2017
High transport current superconductivity in powder-in-tube Ba 0.6 K 0.4 Fe 2 As 2 tapes at 27 T journal December 2017
Improvements of fabrication processes and enhancement of critical current densities in (Ba,K)Fe 2 As 2 HIP wires and tapes journal April 2018
The formation of defects and their influence on inter- and intra-granular current in sintered polycrystalline 122 phase Fe-based superconductors journal July 2019
Grain boundary characteristics of Fe-based superconductors journal March 2020
Synthesis routes to eliminate oxide impurity segregation and their influence on intergrain connectivity in K-doped BaFe 2 As 2 polycrystalline bulks journal July 2020
Evolution of intergranular microstructure and critical current properties of polycrystalline Co-doped BaFe 2 As 2 through high-energy milling journal August 2020
Visualization of the grain structure in high-performance Ba1−x K x Fe2As2 superconducting tapes journal March 2021
K-doped Ba122 epitaxial thin film on MgO substrate by buffer engineering journal August 2022
Significant enhancement of upper critical fields by doping and strain in iron-based superconductors journal November 2011
Artificial and self-assembled vortex-pinning centers in superconducting Ba(Fe 1 − x Co x ) 2 As 2 thin films as a route to obtaining very high critical-current densities journal December 2012
Doping-dependent critical current properties in K, Co, and P-doped BaF e 2 A s 2 single crystals journal January 2017
Superconductivity at 38 K in the Iron Arsenide ( Ba 1 − x K x ) Fe 2 As 2 journal September 2008
Superconducting Fe-Based Compounds ( A 1 − x Sr x ) Fe 2 As 2 with A = K and Cs with Transition Temperatures up to 37 K journal September 2008
Anisotropy of the Upper Critical Field in a Co-Doped BaFe 2 As 2 Single Crystal journal August 2009
Superconductivity and phase diagram in iron-based arsenic-oxides ReFeAsO 1−δ (Re = rare-earth metal) without fluorine doping journal June 2008
Chemically degraded grain boundaries in fine-grain Ba 0.6 K 0.4 Fe 2 As 2 polycrystalline bulks journal October 2020