Nanoscale inhomogeneity and the evolution of correlation strength in FeSe$$_{1-x}$$S$$_x$$

Liu, Yu; Wang, Aifeng; Du, Qianheng; Wu, Lijun; Zhu, Yimei; Petrovic, Cedomir

doi:10.1186/s40580-023-00405-2

Title: Nanoscale inhomogeneity and the evolution of correlation strength in FeSe$$$$_{1-x}$$$$S$$$$_x$$$$

Journal Article · 21 December 2023 · Nano Convergence

DOI: https://doi.org/10.1186/s40580-023-00405-2 · OSTI ID:2251530

Liu, Yu; Wang, Aifeng; Du, Qianheng; Wu, Lijun; Zhu, Yimei;

Abstract We report a comprehensive study of the nanoscale inhomogeneity and disorder on the thermoelectric properties of FeSe $$$$_{1-x}$$$$ $_{1 - x}$ S $$$$_x$$$$ $_{x}$ ( $$$$0 \le x \le 1$$$$ $0 \leq x \leq 1$ ) single crystals and the evolution of correlation strength with S substitution. A hump-like feature in temperature-dependent thermpower is enhanced for x = 0.12 and 0.14 in the nematic region with increasing in orbital-selective electronic correlations, which is strongly suppressed across the nematic critical point and for higher S content. Nanoscale Se/S atom disorder in the tetrahedral surroundings of Fe atoms is confirmed by scanning transmission electron microscopy measurements, providing an insight into the nanostructural details and the evolution of correlation strength in FeSe $$$$_{1-x}$$$$ $_{1 - x}$ S $$$$_x$$$$ $_{x}$ .

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Research Organization:: Brookhaven National Laboratory (BNL), Upton, NY (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE)

Grant/Contract Number:: SC0012704

OSTI ID:: 2251530

Report Number(s):: BNL--225265-2024-JAAM; 59; PII: 405

Journal Information:: Nano Convergence, Journal Name: Nano Convergence Journal Issue: 1 Vol. 10; ISSN 2196-5404

Publisher:: Springer Science + Business MediaCopyright Statement

Country of Publication:: Germany

Language:: English

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Title: Nanoscale inhomogeneity and the evolution of correlation strength in FeSe$$$$_{1-x}$$$$S$$$$_x$$$$

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