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Title: Soft matter roadmap

Journal Article · · JPhys Materials
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  1. Univ. of Grenoble Alpes, Grenoble (France); Centre National de la Recherche Scientifique (CNRS) (France)
  2. Georgetown Univ., Washington, DC (United States)
  3. Heinrich Heine University (Germany)
  4. Univ. of Michigan, Ann Arbor, MI (United States)
  5. Utrecht University (Netherlands)
  6. New York Univ. (NYU), NY (United States)
  7. Columbia Univ., New York, NY (United States)
  8. Technical Univ. of Munich (Germany)
  9. University of Patras (Greece)
  10. Univ. of Colorado, Boulder, CO (United States); National Renewable Energy Laboratory (NREL), Golden, CO (United States). Renewable and Sustainable Energy Institute
  11. Univ. of Strasbourg (France); Centre National de la Recherche Scientifique (CNRS) (France)
  12. Univ. of Delaware, Newark, DE (United States)
  13. National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States)
  14. Emory Univ., Atlanta, GA (United States)
  15. Univ. of Vienna (Austria)
  16. Hong Kong Univ. (Hong Kong)
  17. Montpellier Univ. (France); Centre National de la Recherche Scientifique (CNRS) (France); Institut Universitaire de France (IUF) (France)
  18. Montpellier Univ. (France); Centre National de la Recherche Scientifique (CNRS) (France)
  19. Univ. of Edinburgh, Scotland (United Kingdom)
  20. Cornell Univ., Ithaca, NY (United States)
  21. Univ. of Washington, Seattle, WA (United States)
  22. Duke Univ., Durham, NC (United States)
  23. Jawaharlal Nehru Centre for Advanced Scientific Research, Bangalore (India)
  24. Indian Institute of Science, Bangalore (India)
  25. Sapienza University of Rome (Italy)
  26. Univ. of Cologne (Germany); Univ. of Bonn (Germany)
  27. Jawaharlal Nehru Centre for Advanced Scientific Research (India)
  28. Univ. of Chicago, IL (United States)
  29. Univ. of Pennsylvania, Philadelphia, PA (United States); Emory Univ., Atlanta, GA (United States)
  30. Univ. of Pennsylvania, Philadelphia, PA (United States)
  31. Univ. of Pennsylvania, Philadelphia, PA (United States); Central Glass and Ceramic Research Institute, Kolkata (India)
  32. Univ. of Pennsylvania, Philadelphia, PA (United States); City Univ. of Hong Kong (Hong Kong)
  33. Univ. of Pennsylvania, Philadelphia, PA (United States); Flatiron Institute, New York, NY (United States)
  34. Univ. of Queensland, Brisbane, QLD (Australia)
  35. Aix-Marseille Univ., Marseille (France); Univ. of Toulon (France); Centre National de la Recherche Scientifique (CNRS) (France)
  36. Aix-Marseille Univ., Marseille (France); Centre National de la Recherche Scientifique (CNRS) (France)
  37. Aix-Marseille Univ., Marseille (France); Univ. of Toulon (France); Centre National de la Recherche Scientifique (CNRS) (France); Turing Centre for Living Systems (France)
  38. Institut Laue-Langevin, Grenoble (France)
  39. Univ. of Tubingen (Germany)
  40. Univ. of Malmö (Sweden)
  41. Delft Univ. of Technology (Netherlands)
  42. Univ. of Illinois at Urbana-Champaign, IL (United States)

Soft materials are usually defined as materials made of mesoscopic entities, often self-organised, sensitive to thermal fluctuations and to weak perturbations. Archetypal examples are colloids, polymers, amphiphiles, liquid crystals, foams. The importance of soft materials in everyday commodity products, as well as in technological applications, is enormous, and controlling or improving their properties is the focus of many efforts. From a fundamental perspective, the possibility of manipulating soft material properties, by tuning interactions between constituents and by applying external perturbations, gives rise to an almost unlimited variety in physical properties. Together with the relative ease to observe and characterise them, this renders soft matter systems powerful model systems to investigate statistical physics phenomena, many of them relevant as well to hard condensed matter systems. Understanding the emerging properties from mesoscale constituents still poses enormous challenges, which have stimulated a wealth of new experimental approaches, including the synthesis of new systems with, e.g. tailored self-assembling properties, or novel experimental techniques in imaging, scattering or rheology. Theoretical and numerical methods, and coarse-grained models, have become central to predict physical properties of soft materials, while computational approaches that also use machine learning tools are playing a progressively major role in many investigations. This Roadmap intends to give a broad overview of recent and possible future activities in the field of soft materials, with experts covering various developments and challenges in material synthesis and characterisation, instrumental, simulation and theoretical methods as well as general concepts.

Research Organization:
Univ. of Colorado, Boulder, CO (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE
Grant/Contract Number:
SC0019293; SC0020963; SC0007991; 101042612; 819511; 884902; ANR-10-IDEX-0002; ANR-20-SFRI-0012
OSTI ID:
2229801
Alternate ID(s):
OSTI ID: 2203594; OSTI ID: 2341900
Journal Information:
JPhys Materials, Vol. 7, Issue 1; Conference: Joint Meeting of the Electrochemical Society, Honolulu, HI (United States), 6-11 Oct 2024; ISSN 2515-7639
Publisher:
IOP PublishingCopyright Statement
Country of Publication:
United States
Language:
English

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Direct Visual Observation of Thermal Capillary Waves journal May 2004
Premelting at Defects Within Bulk Colloidal Crystals journal August 2005
Two-step nucleation mechanism in solid–solid phase transitions journal September 2014
Directional grain growth from anisotropic kinetic roughening of grain boundaries in sheared colloidal crystals journal November 2012
Structure determines where crystallization occurs in a soft colloidal glass journal September 2020
Template-directed colloidal crystallization journal January 1997
Direct Measurements of Island Growth and Step-Edge Barriers in Colloidal Epitaxy journal January 2010
Unravelling the multilayer growth of the fullerene C60 in real time journal November 2014
Site-specific colloidal crystal nucleation by template-enhanced particle transport journal October 2016
Entropy-driven crystal formation on highly strained substrates journal May 2013
Soft epitaxy of nanocrystal superlattices journal December 2014
Lattice Mismatch in Crystalline Nanoparticle Thin Films journal December 2017
Cooperative particle rearrangements facilitate the self-organized growth of colloidal crystal arrays on strain-relief patterns journal March 2020
Heteroepitaxial fabrication of binary colloidal crystals by a balance of interparticle interaction and lattice spacing journal February 2022
Self-organized growth of nanostructure arrays on strain-relief patterns journal July 1998
Deconstructing the glass transition through critical experiments on colloids journal July 2016
Local structure in deeply supercooled liquids exhibits growing lengthscales and dynamical correlations journal August 2018
How Reproducible Are Dynamic Heterogeneities in a Supercooled Liquid? journal September 2004
Neglecting polydispersity degrades propensity measurements in supercooled liquids journal May 2021
Unveiling the predictive power of static structure in glassy systems journal April 2020
Self assembling cluster crystals from DNA based dendritic nanostructures journal December 2021
Soft heaps and clumpy crystals journal January 2013
Observation of spatially ordered structures in a two-dimensional Rydberg gas journal October 2012
Glass Transitions in Monodisperse Cluster-Forming Ensembles: Vortex Matter in Type-1.5 Superconductors journal February 2017
Intermittency Route to Rheochaos in Wormlike Micelles with Flow-Concentration Coupling journal March 2006
Experimental signatures of a nonequilibrium phase transition governing the yielding of a soft glass journal June 2014
Strength of Mechanical Memories is Maximal at the Yield Point of a Soft Glass journal April 2019
Large Low-Frequency Fluctuations in the Velocity of a Driven Vortex Lattice in a Single Crystal of 2 H − NbSe 2 Superconductor journal October 2009
Nematic Fermi Fluids in Condensed Matter Physics journal August 2010
Fractonic gauge theory of smectics journal December 2021
Zero-resistance states induced by electromagnetic-wave excitation in GaAs/AlGaAs heterostructures journal December 2002
Transition to zero resistance in a two-dimensional electron gas driven with microwaves journal June 2005
Mode-Coupling Theory of the Glass Transition: A Primer journal October 2018
Colloidal Glass Transition: Beyond Mode-Coupling Theory journal June 2003
Gelation of particles with short-range attraction journal May 2008
Dynamical Arrest in Attractive Colloids: The Effect of Long-Range Repulsion journal May 2005
Phase Diagram of Patchy Colloids: Towards Empty Liquids journal October 2006
Phase behavior and critical activated dynamics of limited-valence DNA nanostars journal September 2013
Ideal glass-glass transitions and logarithmic decay of correlations in a simple system journal February 1999
Multiple Glassy States in a Simple Model System journal April 2002
Interference of phase separation and gelation: A zeroth-order kinetic model journal June 1993
Equilibrium cluster formation in concentrated protein solutions and colloids journal November 2004
Entropic barriers, activated hopping, and the glass transition in colloidal suspensions journal July 2003
Hopping and the Stokes–Einstein relation breakdown in simple glass formers journal October 2014
Anomalous yet Brownian journal July 2009
Length Scales in Brownian yet Non-Gaussian Dynamics journal July 2021
Equilibrium gels of limited valence colloids journal July 2017
Colloidal systems with a short-range attraction and long-range repulsion: Phase diagrams, structures, and dynamics journal February 2019
On the Role of Competing Interactions in Charged Colloids with Short-Range Attraction journal March 2021
Spatially uniform dynamics in equilibrium colloidal gels journal December 2021
Liquids more stable than crystals in particles with limited valence and flexible bonds journal August 2013
Design strategies for the self-assembly of polyhedral shells journal April 2023
Designing Patchy Interactions to Self-Assemble Arbitrary Structures journal September 2020
From predictive modelling to machine learning and reverse engineering of colloidal self-assembly journal May 2021
Memory formation in matter journal July 2019
Memory formation journal June 2023
Learning Without Neurons in Physical Systems journal March 2023
Architected Multimaterial Lattices with Thermally Programmable Mechanical Response journal September 2021
Sequential snapping and pathways in a mechanical metamaterial journal May 2022
Multiple Transient Memories in Experiments on Sheared Non-Brownian Suspensions journal August 2014
Memory from coupled instabilities in unfolded crumpled sheets journal July 2022
Directed aging, memory, and nature’s greed journal December 2019
Periodic training of creeping solids journal November 2020
Memory Formation in Adaptive Networks journal July 2022
Inter-particle adhesion induced strong mechanical memory in a dense granular suspension journal June 2022
Desynchronous learning in a physics-driven learning network journal April 2022
State transition graph of the Preisach model and the role of return-point memory journal July 2020
Delicate memory structure of origami switches journal February 2022
Cooperative effects driving the multi-periodic dynamics of cyclically sheared amorphous solids journal April 2022
Mechanical annealing and memories in a disordered solid journal October 2022
Supervised perceptron learning vs unsupervised Hebbian unlearning: Approaching optimal memory retrieval in Hopfield-like networks journal March 2022
Odd elasticity journal March 2020
Topological modes bound to dislocations in mechanical metamaterials journal January 2015
Combinatorial design of textured mechanical metamaterials journal July 2016
Micrometer-sized electrically programmable shape-memory actuators for low-power microrobotics journal March 2021
Diverse and robust molecular algorithms using reprogrammable DNA self-assembly journal March 2019
A cargo-sorting DNA robot journal September 2017
Electronically integrated, mass-manufactured, microscopic robots journal August 2020
Deep physical neural networks trained with backpropagation journal January 2022
Topological structure and dynamics of three-dimensional active nematics journal March 2020
Characterising soft matter using machine learning journal January 2021
Machine learning in a data-limited regime: Augmenting experiments with synthetic data uncovers order in crumpled sheets journal April 2019
Machine learning and the physical sciences journal December 2019
Machine learning for active matter journal February 2020
Single-Particle Diffusion Characterization by Deep Learning journal July 2019
U-Net: deep learning for cell counting, detection, and morphometry journal December 2018
Deep-STORM: super-resolution single-molecule microscopy by deep learning journal January 2018
Objective comparison of methods to decode anomalous diffusion journal October 2021
Statistical Mechanics of Deep Learning journal March 2020
A high-bias, low-variance introduction to Machine Learning for physicists journal May 2019
An Artificial Neural Network Reveals the Nucleation Mechanism of a Binary Colloidal AB 13 Crystal journal February 2021
Mutual information, neural networks and the renormalization group journal March 2018
Unsupervised machine learning for detection of phase transitions in off-lattice systems. I. Foundations journal November 2018
Machine learning active-nematic hydrodynamics journal March 2021
Assessing the structural heterogeneity of supercooled liquids through community inference journal April 2020
Autonomously revealing hidden local structures in supercooled liquids journal October 2020
Recent advances in machine learning towards multiscale soft materials design journal March 2019
Inverse methods for design of soft materials journal April 2020
Designing allostery-inspired response in mechanical networks journal February 2017
Designing self-assembling kinetics with differentiable statistical physics models journal March 2021
Equilibrium Propagation: Bridging the Gap between Energy-Based Models and Backpropagation journal May 2017
Effect of directed aging on nonlinear elasticity and memory formation in a material journal November 2020
Demonstration of Decentralized Physics-Driven Learning journal July 2022
Predicting glass structure by physics-informed machine learning journal September 2022
Data-Driven Discovery of Active Nematic Hydrodynamics journal December 2022
Machine Learning Force Fields and Coarse-Grained Variables in Molecular Dynamics: Application to Materials and Biological Systems journal June 2020
JAX, M.D. A framework for differentiable physics* journal December 2021
Organic Photovoltaics over Three Decades journal June 2018
All-Polymer Solar Cells: Recent Progress, Challenges, and Prospects journal February 2019
All-polymer particulate slurry batteries journal June 2019
Stable cross-linked lyotropic gyroid mesophases from single-head/single-tail cross-linkable monomers journal January 2021
Perspectives for Polymer Electrolytes: A View from Fundamentals of Ionic Conductivity journal April 2020
Maximizing the right stuff: The trade-off between membrane permeability and selectivity journal June 2017
Materials for next-generation desalination and water purification membranes journal April 2016
Rapid Fabrication by Lyotropic Self-Assembly of Thin Nanofiltration Membranes with Uniform 1 Nanometer Pores journal March 2021
Towards single-species selectivity of membranes with subnanometre pores journal June 2020
Anomalies of Ionic/Molecular Transport in Nano and Sub-Nano Confinement journal August 2020
Microstructural tunability of co-continuous bijel-derived electrodes to provide high energy and power densities journal January 2016
Hybrid electrolytes with 3D bicontinuous ordered ceramic and polymer microchannels for all-solid-state batteries journal January 2018
Self-healing chemistry enables the stable operation of silicon microparticle anodes for high-energy lithium-ion batteries journal November 2013
Energy gels: A bio-inspired material platform for advanced energy applications journal December 2016
Molecular Dynamics Simulations of Ion-Containing Polymers Using Generic Coarse-Grained Models journal February 2021
Thermodynamics of Ion-Containing Polymer Blends and Block Copolymers journal November 2011
Direct Comparisons of X-ray Scattering and Atomistic Molecular Dynamics Simulations for Precise Acid Copolymers and Ionomers journal January 2015
Ionic Correlations in Random Ionomers journal February 2018
Radical Polymers and Their Application to Organic Electronic Devices journal September 2014
Polymer-Based Organic Batteries journal August 2016
Polypeptide organic radical batteries journal May 2021
Energy Harvesting and Storage with Soft and Stretchable Materials journal January 2021
Food structure and functionality: a soft matter perspective journal January 2008
Rheology of gelling and yielding soft matter systems journal January 2008
Food for thought journal September 2004
Understanding foods as soft materials journal October 2005
Small-angle X-Ray and neutron scattering in food colloids journal August 2019
Moving from molecules, to structure, to texture perception journal July 2017
Advances in our understanding of the structure and functionality of edible fats and fat mimetics journal January 2020
Structuring processes for meat analogues journal November 2018
Nonlinear (Large-Amplitude Oscillatory Shear) Rheological Properties and Their Impact on Food Processing and Quality journal March 2021
Spontaneous shear flow in confined cellular nematics journal April 2018
Deforming polar active matter in a scalar field gradient journal January 2023
Topological defects in the nematic order of actin fibres as organization centres of Hydra morphogenesis journal November 2020
Spatiotemporal dynamics of self-organized branching in pancreas-derived organoids journal September 2022
Active Nematic Flows over Curved Surfaces journal September 2022
Curvature gradient drives polarized tissue flow in the Drosophila embryo journal February 2023
Oscillatory cortical forces promote three dimensional cell intercalations that shape the murine mandibular arch journal April 2019
Curvature induces active velocity waves in rotating spherical tissues journal March 2023
Mechanical stress driven by rigidity sensing governs epithelial stability journal November 2022
A fresh eye on nonequilibrium systems journal April 2016
Microrheology, Stress Fluctuations, and Active Behavior of Living Cells journal November 2003
Fluctuations in Active Membranes book January 2018
Turbulent Dynamics of Epithelial Cell Cultures journal May 2018
Discovering governing equations from data by sparse identification of nonlinear dynamical systems journal March 2016
Star-convex Polyhedra for 3D Object Detection and Segmentation in Microscopy conference March 2020
Cellpose 2.0: how to train your own model journal November 2022
Quantifying forces in cell biology journal June 2017
Learning Force Fields from Stochastic Trajectories journal April 2020
Using cell deformation and motion to predict forces and collective behavior in morphogenesis journal July 2017
Theory of nematic and polar active fluid surfaces journal August 2022
Strain-triggered mechanical feedback in self-organizing optic-cup morphogenesis journal November 2018
A Three-Dimensional Numerical Model of an Active Cell Cortex in the Viscous Limit journal October 2021
A viscous active shell theory of the cell cortex journal July 2022
RNA velocity of single cells journal August 2018
Interplay of curvature and rigidity in shape-based models of confluent tissue journal June 2020
Galvanotactic control of collective cell migration in epithelial monolayers journal March 2014
Polymer physics of intracellular phase transitions journal November 2015
The physics of protein self-assembly journal April 2016
The self-assembly, aggregation and phase transitions of food protein systems in one, two and three dimensions journal March 2013
Self-assembled proteins for food applications: A review journal July 2020
Soft-Matter Approaches for Controlling Food Protein Interactions and Assembly journal March 2019
Stability matters, too – the thermodynamics of amyloid fibril formation journal January 2022
Extended law of corresponding states for protein solutions journal May 2015
Multivalent ions and biomolecules: Attempting a comprehensive perspective journal July 2020
Solution conditions determine the relative importance of nucleation and growth processes in  -synuclein aggregation journal May 2014
The physical properties of supramolecular peptide assemblies: from building block association to technological applications journal January 2014
Protein Assembly by Design journal August 2021
Dynamics of proteins in solution journal January 2019
The Statistical Mechanics of Dynamic Pathways to Self-Assembly journal April 2015
Potential and limits of a colloid approach to protein solutions journal January 2020
Patchy colloids: state of the art and perspectives journal January 2011
Protein–Calixarene Complexation: From Recognition to Assembly journal June 2022
Ion-activated attractive patches as a mechanism for controlled protein interactions journal November 2014
Characterizing protein crystal contacts and their role in crystallization: rubredoxin as a case study journal January 2014
Physics-based computational and theoretical approaches to intrinsically disordered proteins journal April 2021
FRET-based dynamic structural biology: Challenges, perspectives and an appeal for open-science practices journal March 2021
Solid-state NMR spectroscopic trends for supramolecular assemblies and protein aggregates journal October 2017
Super-Resolution Microscopy: From Single Molecules to Supramolecular Assemblies journal December 2015
Real-Time Observation of Nonclassical Protein Crystallization Kinetics journal January 2015
Assembly of Capsids from Hepatitis B Virus Core Protein Progresses through Highly Populated Intermediates in the Presence and Absence of RNA journal July 2020
New insight into the dynamical system of αB-crystallin oligomers journal July 2016
Probing Cage Relaxation in Concentrated Protein Solutions by X-Ray Photon Correlation Spectroscopy journal November 2022
Tools and strategies of systems metabolic engineering for the development of microbial cell factories for chemical production journal January 2020
Leveraging advances in biology to design biomaterials journal December 2017
Materials design by synthetic biology journal December 2020
Bioinspired structural materials journal October 2014
Living Materials Herald a New Era in Soft Robotics journal June 2019
Engineered living biomaterials journal August 2021
The living interface between synthetic biology and biomaterial design journal March 2022
Novel materials through Nature's catalysts journal October 2015
Emergent Biological Endurance Depends on Extracellular Matrix Composition of Three-Dimensionally Printed Escherichia coli Biofilms journal October 2021
Bioprinting of Regenerative Photosynthetic Living Materials journal April 2021
Taxonomy for engineered living materials journal April 2022
Engineered Living Materials: Taxonomies and Emerging Trends journal June 2021
Chitosan-polyethylene oxide/clay-alginate nanofiber hydrogel scaffold for bone tissue engineering: Preparation, physical characterization, and biomimetic mineralization journal April 2023
Recent Advances in Synthetic and Natural Biomaterials‐Based Therapy for Bone Defects journal January 2022
Nature’s hierarchical materials journal November 2007
Deciphering structural biological materials: Viewing from the mechanics perspective and their prospects journal October 2022
Nucleation and growth in solution synthesis of nanostructures – From fundamentals to advanced applications journal January 2022
Overview of the amorphous precursor phase strategy in biomineralization journal March 2009
Bioprocess inspired formation of calcite mesocrystals by cation-mediated particle attachment mechanism journal January 2023
Conversion of amorphous calcium phosphate to microcrystalline hydroxyapatite. A pH-dependent, solution-mediated, solid-solid conversion journal September 1973
Calcium Phosphate Delivery Systems for Regeneration and Biomineralization of Mineralized Tissues of the Craniofacial Complex journal January 2023
Nonenzymatic Transformation of Amorphous CaCO3 into Calcium Phosphate Mineral after Exposure to Sodium Phosphate in Vitro: Implications for in Vivo Hydroxyapatite Bone Formation journal May 2015
Calcite Growth in Hydrogels: Assessing the Mechanism of Polymer-Network Incorporation into Single Crystals journal January 2009
Incorporating polymers within a single‐crystal: From heterogeneous structure to multiple functions journal August 2021
Enzymatic mineralization generates ultrastiff and tough hydrogels with tunable mechanics journal March 2017
Biphasic monolithic osteochondral scaffolds obtained by diffusion-limited enzymatic mineralization of gellan gum hydrogel journal January 2023
Mineralization of Hydrogels for Bone Regeneration journal December 2010
Hydroxyapatite-decorated Fmoc-hydrogel as a bone-mimicking substrate for osteoclast differentiation and culture journal January 2022
Tailoring Calcite Growth through an Amorphous Precursor in a Hydrogel Environment journal May 2019
Mediating the Enhanced Interaction Between Hydroxyapatite and Agarose through Amorphous Calcium Carbonate journal August 2020

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