Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries

Tan, Sha; Shadike, Zulipiya; Cai, Xinyin; Lin, Ruoqian; Kludze, Atsu; Borodin, Oleg; Lucht, Brett L.; Wang, Chunsheng; Hu, Enyuan; Xu, Kang; Yang, Xiao-Qing

doi:10.1007/s41918-023-00199-1

Title: Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries

Journal Article · 28 November 2023 · Electrochemical Energy Reviews

DOI: https://doi.org/10.1007/s41918-023-00199-1 · OSTI ID:2228773

^[1]; Shadike, Zulipiya ^[2]; Cai, Xinyin ^[3]; Lin, Ruoqian ^[1]; Kludze, Atsu ^[4]; Borodin, Oleg ^[5]; Lucht, Brett L. ^[6]; Wang, Chunsheng ^[7]; Hu, Enyuan ^[1]; Xu, Kang ^[5];

^[1]

Brookhaven National Laboratory (BNL), Upton, NY (United States)
Brookhaven National Laboratory (BNL), Upton, NY (United States); Shanghai Jiao Tong Univ. (China)
Shanghai Jiao Tong Univ. (China)
Cornell Univ., Ithaca, NY (United States)
Army Research Lab., Adelphi, MD (United States); SolidEnergy Systems (SES), Woburn, MA (United States)
Univ. of Rhode Island, Kingston, RI (United States)
Univ. of Maryland, College Park, MD (United States)

Among various rechargeable batteries, the lithium-ion battery (LIB) stands out due to its high energy density, long cycling life, in addition to other outstanding properties. However, the capacity of LIB drops dramatically at low temperatures (LTs) below 0 °C, thus restricting its applications as a reliable power source for electric vehicles in cold climates and equipment used in the aerospace. The electrolyte engineering has proved to be one of the most effective approaches to mitigate LIB performance degradation at LTs. In this review, we summarize the important factors contributing to the deterioration in Li+ transport and capacity utilization at LTs while systematically categorize the solvents, salts and additives reported in the literature. Strategies to improve the Li⁺ transport kinetics, in the bulk electrolyte and across the interphases, are discussed. In particular, the formation mechanism of solid electrolyte interphase and its functionality for LT electrolytes are analyzed. Perspectives on the future evolution of this area are also provided.

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Research Organization:: Brookhaven National Laboratory (BNL), Upton, NY (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Office of Sustainable Transportation. Vehicle Technologies Office (VTO); USDOE

Grant/Contract Number:: SC0012704

OSTI ID:: 2228773

Alternate ID(s):: OSTI ID: 2242385

Report Number(s):: BNL-225082-2023-JAAM

Journal Information:: Electrochemical Energy Reviews, Vol. 6, Issue 1; ISSN 2520-8489

Publisher:: Springer NatureCopyright Statement

Country of Publication:: United States

Language:: English

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