Chemical structure–property relationships in nanocelluloses

Pitcher, Mica L.; Koshani, Roya; Sheikhi, Amir

doi:10.1002/pol.20230558

Title: Chemical structure–property relationships in nanocelluloses

Journal Article · 19 November 2023 · Journal of Polymer Science

DOI: https://doi.org/10.1002/pol.20230558 · OSTI ID:2217227

Pitcher, Mica L. ^[1]; Koshani, Roya ^[1];

^[1]

Pennsylvania State University, University Park, PA (United States)

Nanocelluloses, nanoscale cellulosic particles or fibrils, are an appealing class of nanomaterials with enormous potential for sustainable development. They have great promise to target some of the 17 Sustainable Development Goals outlined by the United Nations. Nanocelluloses are derived from the most abundant biopolymer in the world, cellulose, which have multiple hydroxyl groups on their surface, enabling a vast range of chemical modifications. The interplay between the chemical structure and physicochemical properties of nanocelluloses is crucial to engineering the next generation of green, functional nanomaterials. In this review paper, we provide a comprehensive account of the structure–property relationships in nanocelluloses, which may establish the basis for the design of precision bio-based materials. Chemical modifications of nanocelluloses, including hydrolysis, oxidation, esterification, amidation, and polymer grafting, provide an array of chemical and physical properties that open opportunities in a diverse spectrum of applications. We review how chemical modifications affect the physicochemical properties of nanocelluloses, such as thermal stability, hydrophobicity, and dispersibility in nonpolar media. Understanding nanocellulose chemical structure–property relationships is integral to the development of sustainable material platforms based on the most renewable biopolymer on earth.

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Research Organization:: Pennsylvania State Univ., University Park, PA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE

Grant/Contract Number:: SC0001090

OSTI ID:: 2217227

Alternate ID(s):: OSTI ID: 2217230; OSTI ID: 2377745

Journal Information:: Journal of Polymer Science, Vol. 62, Issue 1; ISSN 2642-4150

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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