On the Durability of Tin‐Containing Perovskite Solar Cells

Chen, Lei; Fu, Sheng; Li, You; Sun, Nannan; Yan, Yanfa; Song, Zhaoning

doi:10.1002/advs.202304811

Title: On the Durability of Tin‐Containing Perovskite Solar Cells

Journal Article · 15 November 2023 · Advanced Science

DOI: https://doi.org/10.1002/advs.202304811 · OSTI ID:2212826

Chen, Lei ^[1]; Fu, Sheng ^[1]; Li, You ^[1]; Sun, Nannan ^[1]; Yan, Yanfa ^[1];

^[1]

Univ. of Toledo, OH (United States)

Tin (Sn)-containing perovskite solar cells (PSCs) have gained significant attention in the field of perovskite optoelectronics due to lower toxicity than their lead-based counterparts and their potential for tandem applications. However, the lack of stability is a major concern that hampers their development. To achieve the long-term stability of Sn-containing PSCs, it is crucial to have a clear and comprehensive understanding of the degradation mechanisms of Sn-containing perovskites and develop mitigation strategies. This review provides a compendious overview of degradation pathways observed in Sn-containing perovskites, attributing to intrinsic factors related to the materials themselves and environmental factors such as light, heat, moisture, oxygen, and their combined effects. The impact of interface and electrode materials on the stability of Sn-containing PSCs is also discussed. Additionally, various strategies to mitigate the instability issue of Sn-containing PSCs are summarized. Lastly, the challenges and prospects for achieving durable Sn-containing PSCs are presented.

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Research Organization:: Univ. of Toledo, OH (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Office of Sustainable Transportation. Fuel Cell Technologies Office; USDOE Office of Energy Efficiency and Renewable Energy (EERE), Renewable Power Office. Solar Energy Technologies Office; USDOE

Grant/Contract Number:: EE0008753; EE0008837

OSTI ID:: 2212826

Alternate ID(s):: OSTI ID: 2280735; OSTI ID: 2472345

Journal Information:: Advanced Science, Vol. 11, Issue 1; ISSN 2198-3844

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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How SnF ₂ Impacts the Material Properties of Lead-Free Tin Perovskites Gupta, Satyajit; Cahen, David; Hodes, Gary The Journal of Physical Chemistry C, Vol. 122, Issue 25 https://doi.org/10.1021/acs.jpcc.8b01045	journal	December 2017
Thermal degradation of CH ₃ NH ₃ PbI ₃ perovskite into NH ₃ and CH ₃ I gases observed by coupled thermogravimetry–mass spectrometry analysis Juarez-Perez, Emilio J.; Hawash, Zafer; Raga, Sonia R. Energy & Environmental Science, Vol. 9, Issue 11 https://doi.org/10.1039/C6EE02016J	journal	January 2016
Investigation of Thermally Induced Degradation in CH3NH3PbI3 Perovskite Solar Cells using In-situ Synchrotron Radiation Analysis Kim, Nam-Koo; Min, Young Hwan; Noh, Seokhwan Scientific Reports, Vol. 7, Issue 1 https://doi.org/10.1038/s41598-017-04690-w	journal	July 2017
Efficient and Stable Tin Perovskite Solar Cells by Pyridine‐Functionalized Fullerene with Reduced Interfacial Energy Loss Li, Bo; Wu, Xin; Zhang, He Advanced Functional Materials, Vol. 32, Issue 39 https://doi.org/10.1002/adfm.202205870	journal	July 2022
Bifacial all-perovskite tandem solar cells Chen, Bo; Yu, Zhenhua; Onno, Arthur Science Advances, Vol. 8, Issue 47 https://doi.org/10.1126/sciadv.add0377	journal	November 2022
Tin Halide Perovskite (ASnX 3 ) Solar Cells: A Comprehensive Guide toward the Highest Power Conversion Efficiency Nasti, Giuseppe; Abate, Antonio Advanced Energy Materials https://doi.org/10.1002/aenm.201902467	journal	September 2019
Challenges and strategies toward long-term stability of lead-free tin-based perovskite solar cells Aktas, Ece; Rajamanickam, Nagalingam; Pascual, Jorge Communications Materials, Vol. 3, Issue 1 https://doi.org/10.1038/s43246-022-00327-2	journal	December 2022
High‐Performance Multilayer Encapsulation for Perovskite Photovoltaics Wong‐Stringer, Michael; Game, Onkar S.; Smith, Joel A. Advanced Energy Materials, Vol. 8, Issue 24 https://doi.org/10.1002/aenm.201801234	journal	July 2018
Multifunctional Regulation of Highly Orientated Tin–Lead Alloyed Perovskite Solar Cells Jiang, Xiafei; Li, Chongwen; Wang, Xianzhao ACS Energy Letters, Vol. 8, Issue 2 https://doi.org/10.1021/acsenergylett.2c02576	journal	January 2023
DMSO‐Free Solvent Strategy for Stable and Efficient Methylammonium‐Free Sn–Pb Alloyed Perovskite Solar Cells Zhang, Zhanfei; Liang, Jianghu; Wang, Jianli Advanced Energy Materials, Vol. 13, Issue 17 https://doi.org/10.1002/aenm.202300181	journal	March 2023
High-efficiency two-dimensional Ruddlesden–Popper perovskite solar cells Tsai, Hsinhan; Nie, Wanyi; Blancon, Jean-Christophe Nature, Vol. 536, Issue 7616 https://doi.org/10.1038/nature18306	journal	July 2016
Reducing Saturation-Current Density to Realize High-Efficiency Low-Bandgap Mixed Tin-Lead Halide Perovskite Solar Cells Li, Chongwen; Song, Zhaoning; Zhao, Dewei Advanced Energy Materials, Vol. 9, Issue 3 https://doi.org/10.1002/aenm.201803135	journal	November 2018
2D-Quasi-2D-3D Hierarchy Structure for Tin Perovskite Solar Cells with Enhanced Efficiency and Stability Wang, Fei; Jiang, Xianyuan; Chen, Hao Joule, Vol. 2, Issue 12 https://doi.org/10.1016/j.joule.2018.09.012	journal	December 2018
Lead-free tin-halide perovskite solar cells with 13% efficiency Nishimura, Kohei; Kamarudin, Muhammad Akmal; Hirotani, Daisuke Nano Energy, Vol. 74 https://doi.org/10.1016/j.nanoen.2020.104858	journal	August 2020
Chemical Reaction Kinetics of the Decomposition of Low-Bandgap Tin–Lead Halide Perovskite Films and the Effect on the Ambipolar Diffusion Length Meng, Yuhuan; Sunkari, Preetham P.; Meilă, Marina ACS Energy Letters, Vol. 8, Issue 4 https://doi.org/10.1021/acsenergylett.2c02733	journal	March 2023
Origin of Sn( ii ) oxidation in tin halide perovskites Pascual, Jorge; Nasti, Giuseppe; Aldamasy, Mahmoud H. Materials Advances, Vol. 1, Issue 5 https://doi.org/10.1039/D0MA00245C	journal	January 2020
Lead-lean and MA-free perovskite solar cells with an efficiency over 20% Zhang, Wenxiao; Li, Xiaodong; Fu, Sheng Joule, Vol. 5, Issue 11 https://doi.org/10.1016/j.joule.2021.09.008	journal	November 2021
Development of encapsulation strategies towards the commercialization of perovskite solar cells Ma, Sai; Yuan, Guizhou; Zhang, Ying Energy & Environmental Science, Vol. 15, Issue 1 https://doi.org/10.1039/D1EE02882K	journal	January 2022
Photoinduced degradation of methylammonium lead triiodide perovskite semiconductors Tang, Xiaofeng; Brandl, Marco; May, Benjamin Journal of Materials Chemistry A, Vol. 4, Issue 41 https://doi.org/10.1039/C6TA06497C	journal	January 2016
Tin perovskite solar cells with >1,300 h of operational stability in N2 through a synergistic chemical engineering approach Sanchez-Diaz, Jesús; Sánchez, Rafael S.; Masi, Sofia Joule, Vol. 6, Issue 4 https://doi.org/10.1016/j.joule.2022.02.014	journal	April 2022
Low‐Bandgap Mixed Tin‐Lead Perovskites and Their Applications in All‐Perovskite Tandem Solar Cells Wang, Changlei; Song, Zhaoning; Li, Chongwen Advanced Functional Materials, Vol. 29, Issue 47 https://doi.org/10.1002/adfm.201808801	journal	February 2019
Origin of Pronounced Nonlinear Band Gap Behavior in Lead–Tin Hybrid Perovskite Alloys Goyal, Anuj; McKechnie, Scott; Pashov, Dimitar Chemistry of Materials, Vol. 30, Issue 11 https://doi.org/10.1021/acs.chemmater.8b01695	journal	May 2018
Organic‐Free and Lead‐Free Perovskite Solar Cells with Efficiency over 11% (Adv. Energy Mater. 42/2022) Zhang, Weihai; Cai, Yating; Liu, Heng Advanced Energy Materials, Vol. 12, Issue 42 https://doi.org/10.1002/aenm.202270174	journal	November 2022
Carrier control in Sn–Pb perovskites via 2D cation engineering for all-perovskite tandem solar cells with improved efficiency and stability Tong, Jinhui; Jiang, Qi; Ferguson, Andrew J. Nature Energy, Vol. 7, Issue 7 https://doi.org/10.1038/s41560-022-01046-1	journal	June 2022
Halogen Redox Shuttle Explains Voltage-Induced Halide Redistribution in Mixed-Halide Perovskite Devices Xu, Zhaojian; Kerner, Ross A.; Harvey, Steven P. ACS Energy Letters, Vol. 8, Issue 1 https://doi.org/10.1021/acsenergylett.2c02385	journal	December 2022
Solvent-Mediated Crystallization of CH₃NH₃SnI₃ Films for Heterojunction Depleted Perovskite Solar Cells Hao, Feng; Stoumpos, Constantinos C.; Guo, Peijun Journal of the American Chemical Society, Vol. 137, Issue 35, p. 11445-11452 https://doi.org/10.1021/jacs.5b06658	journal	August 2015
Ascorbic acid as an effective antioxidant additive to enhance the efficiency and stability of Pb/Sn-based binary perovskite solar cells Xu, Xiaobao; Chueh, Chu-Chen; Yang, Zhibin Nano Energy, Vol. 34 https://doi.org/10.1016/j.nanoen.2017.02.040	journal	April 2017
Advances in the Application of Perovskite Materials Zhang, Lixiu; Mei, Luyao; Wang, Kaiyang Nano-Micro Letters, Vol. 15, Issue 1 https://doi.org/10.1007/s40820-023-01140-3	journal	July 2023
Heterogeneous FASnI3 Absorber with Enhanced Electric Field for High-Performance Lead-Free Perovskite Solar Cells Wu, Tianhao; Liu, Xiao; Luo, Xinhui Nano-Micro Letters, Vol. 14, Issue 1 https://doi.org/10.1007/s40820-022-00842-4	journal	April 2022
Importance of Reducing Vapor Atmosphere in the Fabrication of Tin-Based Perovskite Solar Cells Song, Tze-Bin; Yokoyama, Takamichi; Stoumpos, Constantinos C. Journal of the American Chemical Society, Vol. 139, Issue 2 https://doi.org/10.1021/jacs.6b10734	journal	January 2017
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Oxidation of Spiro-OMeTAD in High-Efficiency Perovskite Solar Cells Ouedraogo, Nabonswende Aida Nadege; Odunmbaku, George Omololu; Guo, Bing ACS Applied Materials & Interfaces, Vol. 14, Issue 30 https://doi.org/10.1021/acsami.2c06163	journal	July 2022
Ligand Orientation-Induced Lattice Robustness for Highly Efficient and Stable Tin-Based Perovskite Solar Cells Li, Peizhou; Dong, Hua; Xu, Jie ACS Energy Letters, Vol. 5, Issue 7 https://doi.org/10.1021/acsenergylett.0c00960	journal	June 2020
Reducing Carrier Density in Formamidinium Tin Perovskites and Its Beneficial Effects on Stability and Efficiency of Perovskite Solar Cells Lee, Seon Joo; Shin, Seong Sik; Im, Jino ACS Energy Letters, Vol. 3, Issue 1 https://doi.org/10.1021/acsenergylett.7b00976	journal	November 2017
Factors Limiting the Operational Stability of Tin–Lead Perovskite Solar Cells Huerta Hernandez, Luis; Lanzetta, Luis; Jang, Soyeong ACS Energy Letters, Vol. 8, Issue 1 https://doi.org/10.1021/acsenergylett.2c02035	journal	November 2022
Rain on Methylammonium Lead Iodide Based Perovskites: Possible Environmental Effects of Perovskite Solar Cells Hailegnaw, Bekele; Kirmayer, Saar; Edri, Eran The Journal of Physical Chemistry Letters, Vol. 6, Issue 9 https://doi.org/10.1021/acs.jpclett.5b00504	journal	April 2015
Enhancing Photostability of Sn‐Pb Perovskite Solar Cells by an Alkylammonium Pseudo‐Halogen Additive Wang, Jiantao; Uddin, Md Aslam; Chen, Bo Advanced Energy Materials, Vol. 13, Issue 15 https://doi.org/10.1002/aenm.202204115	journal	March 2023
All-perovskite tandem solar cells with 24.2% certified efficiency and area over 1 cm2 using surface-anchoring zwitterionic antioxidant Xiao, Ke; Lin, Renxing; Han, Qiaolei Nature Energy, Vol. 5, Issue 11 https://doi.org/10.1038/s41560-020-00705-5	journal	October 2020
Surface-Controlled Oriented Growth of FASnI3 Crystals for Efficient Lead-free Perovskite Solar Cells Meng, Xiangyue; Wang, Yanbo; Lin, Jianbo Joule, Vol. 4, Issue 4 https://doi.org/10.1016/j.joule.2020.03.007	journal	April 2020
Wide-bandgap, low-bandgap, and tandem perovskite solar cells Song, Zhaoning; Chen, Cong; Li, Chongwen Semiconductor Science and Technology, Vol. 34, Issue 9 https://doi.org/10.1088/1361-6641/ab27f7	journal	July 2019
Surface Reconstruction for Tin-Based Perovskite Solar Cells Li, Hui; Chang, Bohong; Wang, Lian ACS Energy Letters, Vol. 7, Issue 11 https://doi.org/10.1021/acsenergylett.2c01624	journal	October 2022

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