Angular‐Momentum Transfer Mediated by a Vibronic‐Bound‐State

Pai, Yun‐Yi; Marvinney, Claire E.; Pokharel, Ganesh; Xing, Jie; Li, Haoxiang; Li, Xun; Chilcote, Michael; Brahlek, Matthew; Lindsay, Lucas; Miao, Hu; Sefat, Athena S.; Parker, David; Wilson, Stephen D.; Gardner, Jason S.; Liang, Liangbo; Lawrie, Benjamin J.

doi:10.1002/advs.202304698

Title: Angular‐Momentum Transfer Mediated by a Vibronic‐Bound‐State

Journal Article · 08 November 2023 · Advanced Science

DOI: https://doi.org/10.1002/advs.202304698 · OSTI ID:2205391

Pai, Yun‐Yi ^[1]; Marvinney, Claire E. ^[2]; Pokharel, Ganesh ^[3]; Xing, Jie ^[2]; Li, Haoxiang ^[2]; Li, Xun ^[2]; Chilcote, Michael ^[2]; Brahlek, Matthew ^[2]; Lindsay, Lucas ^[2]; Miao, Hu ^[2]; Sefat, Athena S. ^[2]; Parker, David ^[2]; Wilson, Stephen D. ^[3]; Gardner, Jason S. ^[2]; Liang, Liangbo ^[4];

^[2]

Materials Science and Technology Division Oak Ridge National Laboratory Oak Ridge TN 37831 USA, Materials Department University of California Santa Barbara Santa Barbara CA 93106 USA
Materials Science and Technology Division Oak Ridge National Laboratory Oak Ridge TN 37831 USA
Materials Department University of California Santa Barbara Santa Barbara CA 93106 USA
Center for Nanophase Materials Sciences Oak Ridge National Laboratory Oak Ridge TN 37831 USA

Abstract The notion that phonons can carry pseudo‐angular momentum has many major consequences, including topologically protected phonon chirality, Berry curvature of phonon band structure, and the phonon Hall effect. When a phonon is resonantly coupled to an orbital state split by its crystal field environment, a so‐called vibronic bound state forms. Here, a vibronic bound state is observed in NaYbSe ₂ , a quantum spin liquid candidate. In addition, field and polarization dependent Raman microscopy is used to probe an angular momentum transfer of Δ J _z = ±ℏ between phonons and the crystalline electric field mediated by the vibronic bound stat. This angular momentum transfer between electronic and lattice subsystems provides new pathways for selective optical addressability of phononic angular momentum via electronic ancillary states.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States); Univ. of California, Santa Barbara, CA (United States)

Sponsoring Organization:: USDOE; USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE); USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities (SUF)

Grant/Contract Number:: AC05-00OR22725; SC0017752

OSTI ID:: 2205391

Journal Information:: Advanced Science, Journal Name: Advanced Science Journal Issue: 2 Vol. 11; ISSN 2198-3844

Publisher:: Wiley Blackwell (John Wiley & Sons)Copyright Statement

Country of Publication:: Germany

Language:: English

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Title: Angular‐Momentum Transfer Mediated by a Vibronic‐Bound‐State

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