Crystal growth, structural and electronic characterizations of zero-dimensional metal halide (TEP)InBr 4 single crystals for X-ray detection

Zhang, Zheng; Pugliano, Tony M.; Cao, Da; Kim, Doup; Annam, Roshan S.; Popy, Dilruba A.; Pinky, Tamanna; Yang, Ge; Garg, Jivtesh; Borunda, Mario F.; Saparov, Bayram

doi:10.1039/D3TC02787B

Title: Crystal growth, structural and electronic characterizations of zero-dimensional metal halide (TEP)InBr ₄ single crystals for X-ray detection

Journal Article · 09 November 2023 · Journal of Materials Chemistry C

DOI: https://doi.org/10.1039/D3TC02787B · OSTI ID:2203989

Zhang, Zheng ^[1]; Pugliano, Tony M. ^[1]; Cao, Da ^[2];

^[2]; Annam, Roshan S. ^[3]; Popy, Dilruba A. ^[1]; Pinky, Tamanna ^[1];

^[2];

^[3]; Borunda, Mario F. ^[4];

^[1]

Department of Chemistry and Biochemistry, University of Oklahoma, Norman, OK 73019, USA
Department of Nuclear Engineering, North Carolina State University, Raleigh, NC 27607, USA
School of Aerospace and Mechanical Engineering, University of Oklahoma, Norman, OK 73019, USA
Department of Physics, Oklahoma State University, Stillwater, OK 74078, USA

A new 0D metal halide (TEP)InBr ₄ is reported. Structural and electronic properties were studied. The fabricated X-ray detector using a (TEP)InBr ₄ single crystal showed a detection sensitivity of 569.85 μC Gy ⁻¹ cm ⁻² at E = 100 V mm ⁻¹ .

View Accepted Manuscript (Publisher)

Cite

Export

Save

Sponsoring Organization:: USDOE

OSTI ID:: 2203989

Journal Information:: Journal of Materials Chemistry C, Journal Name: Journal of Materials Chemistry C Vol. 11 Journal Issue: 43; ISSN 2050-7526

Publisher:: Royal Society of Chemistry (RSC)Copyright Statement

Country of Publication:: United Kingdom

Language:: English

References (39)

Generalized Gradient Approximation Made Simple Perdew, John P.; Burke, Kieron; Ernzerhof, Matthias Physical Review Letters, Vol. 77, Issue 18, p. 3865-3868 https://doi.org/10.1103/PhysRevLett.77.3865	journal	October 1996
The PseudoDojo: Training and grading a 85 element optimized norm-conserving pseudopotential table van Setten, M. J.; Giantomassi, M.; Bousquet, E. Computer Physics Communications, Vol. 226 https://doi.org/10.1016/j.cpc.2018.01.012	journal	May 2018
Trap Density Determination by Space‐Charge‐Limited Currents Bube, Richard H. Journal of Applied Physics, Vol. 33, Issue 5 https://doi.org/10.1063/1.1728818	journal	May 1962
Development of Single Crystal CsPbBr3 Radiation Detectors from Low-Cost Solution Synthesized Material Kunar, David A.; Webster, Matthew F.; Wu, Yu Crystals, Vol. 13, Issue 5 https://doi.org/10.3390/cryst13050762	journal	May 2023
Ionic current and polarization effect in TlBr Leão, Cedric Rocha; Lordi, Vincenzo Physical Review B, Vol. 87, Issue 8 https://doi.org/10.1103/PhysRevB.87.081202	journal	February 2013
Anisotropic Growth of Centimeter‐Size CsCu₂I₃ Single Crystals with Ultra‐Low Trap Density for Aspect‐Ratio‐Dependent Photodetectors Han, Sancan; Quan, Jiale; Wang, Ding Advanced Science, Vol. 10, Issue 7 https://doi.org/10.1002/advs.202206417	journal	January 2023
Revised effective ionic radii and systematic studies of interatomic distances in halides and chalcogenides Shannon, R. D. Acta Crystallographica Section A, Vol. 32, Issue 5, p. 751-767 https://doi.org/10.1107/S0567739476001551	journal	September 1976
High-Performance X-ray Detector Based on Single-Crystal β-Ga₂O₃:Mg Chen, Jiawen; Tang, Huili; Liu, Bo ACS Applied Materials & Interfaces, Vol. 13, Issue 2 https://doi.org/10.1021/acsami.0c20574	journal	January 2021
Plasma Hsp90 levels in patients with systemic sclerosis and relation to lung and skin involvement: a cross-sectional and longitudinal study Štorkánová, Hana; Oreská, Sabína; Špiritović, Maja Scientific Reports, Vol. 11, Issue 1 https://doi.org/10.1038/s41598-020-79139-8	journal	January 2021
Special points for Brillouin-zone integrations Monkhorst, Hendrik J.; Pack, James D. Physical Review B, Vol. 13, Issue 12, p. 5188-5192 https://doi.org/10.1103/PhysRevB.13.5188	journal	June 1976
High-field effects in photoconducting cadmium sulphide Many, A. Journal of Physics and Chemistry of Solids, Vol. 26, Issue 3 https://doi.org/10.1016/0022-3697(65)90133-2	journal	March 1965
Improving the Performance and High‐Field Stability of FAPbBr₃ Single Crystals in X‐Ray Detection with Chenodeoxycholic Acid Additive Jiang, Wei; Ren, Jiwei; Li, Haibin Small Methods, Vol. 7, Issue 4 https://doi.org/10.1002/smtd.202201636	journal	February 2023
Physical Properties of Candidate X-ray Detector Material Rb₄Ag₂BiBr₉ Zhang, Zheng; Ma, Ying-Zhong; Thomas, Leonard Crystal Growth & Design, Vol. 22, Issue 2 https://doi.org/10.1021/acs.cgd.1c00986	journal	December 2021
Thallium lead iodide (TlPbI3) single crystal inorganic perovskite: Electrical and optical characterization for gamma radiation detection Hany, Ibrahim; Yang, Ge; Phan, Quoc Vuong Materials Science in Semiconductor Processing, Vol. 121 https://doi.org/10.1016/j.mssp.2020.105392	journal	January 2021
Centimeter‐Sized Single Crystal of Two‐Dimensional Halide Perovskites Incorporating Straight‐Chain Symmetric Diammonium Ion for X‐Ray Detection Shen, Yue; Liu, Yucheng; Ye, Haochen Angewandte Chemie International Edition, Vol. 59, Issue 35 https://doi.org/10.1002/anie.202004160	journal	June 2020
Suppressed Halide Ion Migration in 2D Lead Halide Perovskites Cho, Junsang; DuBose, Jeffrey T.; Le, An Ngoc Thien ACS Materials Letters, Vol. 2, Issue 6 https://doi.org/10.1021/acsmaterialslett.0c00124	journal	April 2020
Thin-Film Deposition and Characterization of a Sn-Deficient Perovskite Derivative Cs ₂ SnI ₆ Saparov, Bayrammurad; Sun, Jon-Paul; Meng, Weiwei Chemistry of Materials, Vol. 28, Issue 7 https://doi.org/10.1021/acs.chemmater.6b00433	journal	March 2016
Potential lead toxicity and leakage issues on lead halide perovskite photovoltaics Ren, Meng; Qian, Xufang; Chen, Yuetian Journal of Hazardous Materials, Vol. 426 https://doi.org/10.1016/j.jhazmat.2021.127848	journal	March 2022
Ultralong Carrier Lifetime Exceeding 20 µs in Lead Halide Perovskite Film Enable Efficient Solar Cells Guo, Jiahao; Wang, Bingzhe; Lu, Di Advanced Materials, Vol. 35, Issue 28 https://doi.org/10.1002/adma.202212126	journal	May 2023
Lead-free halide perovskite photovoltaics: Challenges, open questions, and opportunities Pecunia, Vincenzo; Occhipinti, Luigi G.; Chakraborty, Abhisek APL Materials, Vol. 8, Issue 10 https://doi.org/10.1063/5.0022271	journal	October 2020
A Primer in Density Functional Theory Fiolhais, Carlos; Nogueira, Fernando; Marques, Miguel A. L. Lecture Notes in Physics https://doi.org/10.1007/3-540-37072-2	book	January 2003
Intrinsic Self‐Trapped Emission in 0D Lead‐Free (C ₄ H ₁₄ N ₂ ) ₂ In ₂ Br ₁₀ Single Crystal Zhou, Lei; Liao, Jin‐Feng; Huang, Zeng‐Guang Angewandte Chemie International Edition, Vol. 58, Issue 43 https://doi.org/10.1002/anie.201907503	journal	October 2019
Charge carrier mobility of halide perovskite single crystals for ionizing radiation detection Zhang, Zheng; Saparov, Bayram Applied Physics Letters, Vol. 119, Issue 3 https://doi.org/10.1063/5.0057411	journal	July 2021
S iesta : Recent developments and applications García, Alberto; Papior, Nick; Akhtar, Arsalan The Journal of Chemical Physics, Vol. 152, Issue 20 https://doi.org/10.1063/5.0005077	journal	May 2020
Ultralow Thermal Conductivity of Two-Dimensional Metal Halide Perovskites Giri, Ashutosh; Chen, Alexander Z.; Mattoni, Alessandro Nano Letters, Vol. 20, Issue 5 https://doi.org/10.1021/acs.nanolett.0c00214	journal	March 2020
Gamma‐Ray Detection Using Bi‐Poor Cs ₂ AgBiBr ₆ Double Perovskite Single Crystals Zhang, Zheng; Cao, Da; Huang, Zhengjie Advanced Optical Materials, Vol. 9, Issue 8 https://doi.org/10.1002/adom.202001575	journal	March 2021
Dose Rate Limitations of Integrating Survey Meters for Diagnostic X-Ray Survevs Shearer, Douglas R.; Bopaiah, Mikhil Health Physics, Vol. 79 https://doi.org/10.1097/00004032-200008001-00007	journal	January 2000
Halide Perovskite Light‐Emitting Diode Technologies Ji, Kangyu; Anaya, Miguel; Abfalterer, Anna Advanced Optical Materials https://doi.org/10.1002/adom.202002128	journal	March 2021
Ultrasensitive and stable X-ray detection using zero-dimensional lead-free perovskites Zheng, Xiaojia; Zhao, Wei; Wang, Peng Journal of Energy Chemistry, Vol. 49 https://doi.org/10.1016/j.jechem.2020.02.049	journal	October 2020
Investigation of the Solution Chemistry of Hybrid Organic–Inorganic Indium Halides for New Material Discovery Zhang, Zheng; Fattal, Hadiah; Creason, Tielyr D. Inorganic Chemistry, Vol. 61, Issue 33 https://doi.org/10.1021/acs.inorgchem.2c01161	journal	August 2022
Mobility-lifetime product and interface property in amorphous silicon solar cells Okamoto, H.; Kida, H.; Nonomura, S. Journal of Applied Physics, Vol. 54, Issue 6 https://doi.org/10.1063/1.332485	journal	June 1983
Simultaneous Control of Ionic and Electronic Conductivity in Materials: Thallium Bromide Case Study Leão, Cedric R.; Lordi, Vincenzo Physical Review Letters, Vol. 108, Issue 24 https://doi.org/10.1103/PhysRevLett.108.246604	journal	June 2012
Charge Transport and Space-Charge Formation in Cd 1 − x Zn x Te 1 − y Se y Radiation Detectors Pipek, J.; Betušiak, M.; Belas, E. Physical Review Applied, Vol. 15, Issue 5 https://doi.org/10.1103/PhysRevApplied.15.054058	journal	May 2021
High-Performance X-ray Detection Based on One-Dimensional Inorganic Halide Perovskite CsPbI ₃ Zhang, Bin-Bin; Liu, Xin; Xiao, Bao The Journal of Physical Chemistry Letters, Vol. 11, Issue 2 https://doi.org/10.1021/acs.jpclett.9b03523	journal	December 2019
Ion migration in halide perovskite solar cells: Mechanism, characterization, impact and suppression Zai, Huachao; Ma, Yue; Chen, Qi Journal of Energy Chemistry, Vol. 63 https://doi.org/10.1016/j.jechem.2021.08.006	journal	December 2021
Tolerance Factor and Cooperative Tilting Effects in Vacancy-Ordered Double Perovskite Halides Maughan, Annalise E.; Ganose, Alex M.; Almaker, Mohammed A. Chemistry of Materials, Vol. 30, Issue 11 https://doi.org/10.1021/acs.chemmater.8b01549	journal	May 2018
High-performance single crystal CH ₃ NH ₃ PbI ₃ perovskite x-ray detector Geng, Xiangshun; Zhang, Hainan; Ren, Jun Applied Physics Letters, Vol. 118, Issue 6 https://doi.org/10.1063/5.0040653	journal	February 2021
Theoretical prediction of high melting temperature for a Mo–Ru–Ta–W HCP multiprincipal element alloy Hong, Qi-Jun; Schroers, Jan; Hofmann, Douglas npj Computational Materials, Vol. 7, Issue 1 https://doi.org/10.1038/s41524-020-00473-6	journal	January 2021
Correlations Between Crystal Defects and Performance of CdZnTe Detectors Bolotnikov, A. E.; Babalola, S.; Camarda, G. S. IEEE Transactions on Nuclear Science, Vol. 58, Issue 4 https://doi.org/10.1109/TNS.2011.2160283	journal	August 2011

Similar Records

Anomalous Charge Transfer from Organic Ligands to Metal Halides in Zero‐Dimensional [(C ₆ H ₅ ) ₄ P] ₂ SbCl ₅ Enabled by Pressure‐Induced Lone Pair‐π Interaction

Journal Article · 2023 · Angewandte Chemie · OSTI ID:1998003

Luo, Hui; Bu, Kejun; Yin, Yanfeng; +14 more

Anomalous Charge Transfer from Organic Ligands to Metal Halides in Zero-Dimensional [(C₆H₅)₄P]₂SbCl₅ Enabled by Pressure-Induced Lone Pair-π Interaction

Journal Article · 2023 · Angewandte Chemie (International Edition) · OSTI ID:2423287

Luo, Hui; Bu, Kejun; Yin, Yanfeng; +14 more

Nucleation-controlled growth of superior lead-free perovskite Cs₃Bi₂I₉ single-crystals for high-performance X-ray detection

Journal Article · 2020 · Nature Communications · OSTI ID:1802375

Zhang, Yunxia; Liu, Yucheng; Xu, Zhuo; +7 more

Title: Crystal growth, structural and electronic characterizations of zero-dimensional metal halide (TEP)InBr 4 single crystals for X-ray detection

Citation Formats

References (39)

Similar Records

Related Subjects

Title: Crystal growth, structural and electronic characterizations of zero-dimensional metal halide (TEP)InBr ₄ single crystals for X-ray detection