Evaluating the carbon footprint of the integrated DBD‐plasma bi‐reforming unit via laboratory scale experiments and scaled‐up process modeling

Cao, Guoqiang; Gonzalez‐Casamachin, Diego Alexander; Xiao, Yue; Chen, Chien‐Hua; Uddi, Mruthunjaya; Baltrusaitis, Jonas

doi:10.1002/ppap.202300148

Title: Evaluating the carbon footprint of the integrated DBD‐plasma bi‐reforming unit via laboratory scale experiments and scaled‐up process modeling

Journal Article · 27 October 2023 · Plasma Processes and Polymers

DOI: https://doi.org/10.1002/ppap.202300148 · OSTI ID:2203976

^[1]; Gonzalez‐Casamachin, Diego Alexander ^[2]; Xiao, Yue ^[3]; Chen, Chien‐Hua ^[3]; Uddi, Mruthunjaya ^[3];

^[2]

State Key Laboratory of Coal Conversion Chinese Academy of Sciences Taiyuan Shanxi China, Department of Chemical and Biomolecular Engineering Lehigh University Bethlehem Pennsylvania USA
Department of Chemical and Biomolecular Engineering Lehigh University Bethlehem Pennsylvania USA
Advanced Cooling Technologies, Inc. Lancaster Pennsylvania USA

Abstract Catalytic dielectric barrier discharge (DBD) plasma reactor experiments were performed in a tubular glass reactor with a 2 mm gap at 550°C to facilitate the reaction kinetics of steam added dry reforming or bireforming. The best specific energy input obtained was 11.2 eV/molecule feed at CO ₂ :CH ₄ :H ₂ O of 4.5:1:4.5 ratio and gas hour space velocity (GHSV) = 432 h ⁻¹ . This value was used to design a conceptual process and assess the environmental impact of methane steam reforming‐based H ₂ production 18.4 kmol/h CO ₂ emission processing into H ₂ :CO = 2 syngas, with an emphasis on the carbon footprint.

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Sponsoring Organization:: USDOE

OSTI ID:: 2203976

Alternate ID(s):: OSTI ID: 2281044

Journal Information:: Plasma Processes and Polymers, Journal Name: Plasma Processes and Polymers Vol. 21 Journal Issue: 1; ISSN 1612-8850

Publisher:: Wiley Blackwell (John Wiley & Sons)Copyright Statement

Country of Publication:: Germany

Language:: English

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