DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Electrical breakdown dynamics in an argon bubble submerged in conductive liquid for nanosecond pulsed discharges

Journal Article · · Journal of Physics. D, Applied Physics

Abstract This study delves into the dynamics of cold atmospheric plasma and their interaction within conductive solutions under the unique conditions of nanosecond pulsed discharges (22 kV peak voltage, 10 ns FWHM, 4.5 kV ns −1 rate-of-rise). The research focuses on the electrical response, breakdown, and discharge propagation in an argon bubble, submerged in a NaCl solution of varying conductivity. Full or partial discharges were observed at conductivities of 1.5 µ S cm −1 (deionized water) to 1.6 mS cm −1 , but no breakdown was observed at 11.0 mS cm −1 when reducing the electrode gap. It is demonstrated that at higher conductivity electric breakdown is observed only when the gas bubble comes into direct contact with the electrode and multiple emission nodes were observed at different timescales. These nodes expanded in the central region of the bubble over timescales longer than the initial high-voltage pulse. This work offers a temporal resolution of 2 ns exposure times over the first 30 ns of the initial voltage pulse, and insight into plasma formation over decaying reflected voltage oscillations over 200 ns.

Sponsoring Organization:
USDOE
Grant/Contract Number:
AC02-09CH11466
OSTI ID:
2006880
Alternate ID(s):
OSTI ID: 2001013; OSTI ID: 2544230; OSTI ID: 2217305
Journal Information:
Journal of Physics. D, Applied Physics, Journal Name: Journal of Physics. D, Applied Physics Journal Issue: 50 Vol. 56; ISSN 0022-3727
Publisher:
IOP PublishingCopyright Statement
Country of Publication:
United Kingdom
Language:
English

References (42)

Observations of electric discharge streamer propagation and capillary oscillations on the surface of air bubbles in water journal February 2011
The influence of liquid conductivity on electrical breakdown and hydrogen peroxide production in a nanosecond pulsed plasma discharge generated in a water-film plasma reactor journal December 2018
Plasma physics of liquids—A focused review journal September 2018
Effects of Electrode Protrusion Length, Pre-Existing Bubbles, Solution Conductivity and Temperature, on Liquid Phase Pulsed Electrical Discharge journal November 2009
Structure of positive streamers inside gaseous bubbles immersed in liquids journal June 2009
Ionic mobilities of Na+ and Cl at 25°C as a function of Ewald sum parameter: a comparative molecular dynamics simulation study journal November 2019
Impulse breakdown of water with different conductivities journal October 2012
Ion-pair or ion-cloud relaxation? On the origin of small-amplitude low-frequency relaxations of weakly associating aqueous electrolytes journal December 2012
Plasma formation in underwater gas bubbles journal February 2014
Microwave Plasma Jet in Water: Effect of Water Electrical Conductivity on Plasma Characteristics journal September 2019
Ignition and propagation of nanosecond pulsed plasmas in distilled water—Negative vs positive polarity applied to a pin electrode journal June 2021
Time-resolved imaging of streamer formation inside gaseous bubbles in liquids journal October 2019
Measuring plasma-generated · OH and O atoms in liquid using EPR spectroscopy and the non-selectivity of the HTA assay journal January 2021
Plasma agriculture: Review from the perspective of the plant and its ecosystem journal September 2020
Nanosecond pulsed discharges in distilled water-Part II: line emission and plasma propagation journal August 2020
Time-resolved processes in a pulsed electrical discharge in argon bubbles in water journal November 2010
Adsorption of Na + and Cl at the charged water–platinum interface journal February 1993
Streamer breakdown in elongated, compressed and tilted bubbles immersed in water journal August 2017
Molecular dynamics simulation of ionic mobility. I. Alkali metal cations in water at 25 °C journal October 1994
Optical and Electrical Diagnostics of the Effects of Conductivity on Liquid Phase Electrical Discharge journal March 2011
Analysis of a pulsed discharge within single bubbles in water under synchronized conditions journal April 2011
Plasma breakdown in bubbles passing between two pin electrodes journal October 2022
Influence of conductivity on the generation of a radio frequency plasma surrounded by bubbles in water journal May 2011
Computation of dielectric constants of solvent mixtures and electrolyte solutions journal August 2001
A Database for the Static Dielectric Constant of Water and Steam journal January 1995
Velocity of initial propagation of positive nanosecond discharge in liquid water: dependence on high voltage amplitude and water conductivity journal February 2019
Ignition modes of nanosecond discharge with bubbles in distilled water journal September 2015
The effect of conductivity on streamer initiation and propagation between dielectric-coated sphere-plate electrodes in water journal December 2009
Electric discharge initiation in water with gas bubbles: A time scale approach journal September 2022
Analysis and Review of Chemical Reactions and Transport Processes in Pulsed Electrical Discharge Plasma Formed Directly in Liquid Water journal August 2012
Investigation of positive and negative modes of nanosecond pulsed discharge in water and electrostriction model of initiation journal August 2013
Mobility of large ions in water journal July 2020
Pulsed electrical breakdown of conductive water with air bubbles journal August 2019
Plasma-based water purification: Challenges and prospects for the future journal May 2017
Pulsed electrical discharge in conductive solution journal August 2016
White paper on the future of plasma science in environment, for gas conversion and agriculture journal July 2018
The effect of electrical conductivity on nanosecond discharges in distilled water and in methanol with argon bubbles journal April 2017
The essential role of the plasma sheath in plasma–liquid interaction and its applications—A perspective journal June 2021
Nanosecond plasmas in water: ignition, cavitation and plasma parameters journal August 2019
Propagation of positive discharges in an air bubble having an embedded water droplet journal January 2021
Direct Numerical Simulation of Bubble Formation Through a Submerged “Flute” With Experimental Validation journal September 2021
Electrical discharge in gas bubbles in gel journal October 2020