Title: Strain‐Control of Cycloidal Spin Order in a Metallic Van der Waals Magnet

Journal Article · · Advanced Materials
ORCiD logo [1];  [1];  [2];  [2];  [3]; ORCiD logo [1]
  1. Rutgers Center for Emergent Materials and Department of Physics and Astronomy Rutgers University Piscataway New Jersey 08854 USA
  2. Department of Physics New Jersey Institute of Technology Newark New Jersey 07102 USA
  3. Zernike Institute for Advanced Materials University of Groningen Nijenborgh 4 Groningen 9747AG The Netherlands

Abstract The manipulation of magnetism through strain control is a captivating area of research with potential applications for low‐power devices that do not require dissipative currents. Recent investigations of insulating multiferroics have unveiled tunable relationships among polar lattice distortions, Dzyaloshinskii–Moriya interactions (DMI), and cycloidal spin orders that break inversion symmetry. These findings have raised the possibility of utilizing strain or strain gradient to manipulate intricate magnetic states by changing polarization. However, the effectiveness of manipulating cycloidal spin orders in “metallic” materials with screened magnetism‐relevant electric polarization remains uncertain. In this study, the reversible strain control of cycloidal spin textures in a metallic van der Waals magnet, Cr 1/3 TaS 2 , through the modulation of polarization and DMI induced by strain is demonstrated. With thermally‐induced biaxial strains and isothermally‐applied uniaxial strains, systematic manipulation of the sign and wavelength of the cycloidal spin textures is realized, respectively. Additionally, unprecedented reflectivity reduction under strain and domain modification at a record‐low current density are also discovered. These findings establish a connection between polarization and cycloidal spins in metallic materials and present a new avenue for utilizing the remarkable tunability of cycloidal magnetic textures and optical functionality in van der Waals metals with strain.

Research Organization:
New Jersey Institute of Technology (NJIT), Newark, NJ (United States)
Sponsoring Organization:
USDOE; USDOE Office of Science (SC)
Grant/Contract Number:
SC0021188
OSTI ID:
1992944
Journal Information:
Advanced Materials, Journal Name: Advanced Materials Journal Issue: 39 Vol. 35; ISSN 0935-9648
Publisher:
Wiley Blackwell (John Wiley & Sons)Copyright Statement
Country of Publication:
Germany
Language:
English

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