Optimizing the Composite Cathode Microstructure in All‐Solid‐State Batteries by Structure‐Resolved Simulations

Clausnitzer, Moritz; Mücke, Robert; Al‐Jaljouli, Fadi; Hein, Simon; Finsterbusch, Martin; Danner, Timo; Fattakhova‐Rohlfing, Dina; Guillon, Olivier; Latz, Arnulf

doi:10.1002/batt.202300167

Title: Optimizing the Composite Cathode Microstructure in All‐Solid‐State Batteries by Structure‐Resolved Simulations

Journal Article · 24 July 2023 · Batteries & Supercaps

DOI: https://doi.org/10.1002/batt.202300167 · OSTI ID:1992393

^[1]; Mücke, Robert ^[2]; Al‐Jaljouli, Fadi ^[3];

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German Aerospace Center (DLR) Institute of Engineering Thermodynamics Pfaffenwaldring 38–40 70569 Stuttgart Germany, Helmholtz Institute Ulm for Electrochemical Energy Storage (HIU) Helmholtzstraße 11 89081 Ulm Germany
Forschungszentrum Jülich GmbH Institute of Energy and Climate Research Materials Synthesis and Processing (IEK-1) Wilhelm-Johnen-Straße 52425 Jülich Germany, Jülich Aachen Research Alliance: JARA-Energy 52425 Jülich Germany
Forschungszentrum Jülich GmbH Institute of Energy and Climate Research Materials Synthesis and Processing (IEK-1) Wilhelm-Johnen-Straße 52425 Jülich Germany, Jülich Aachen Research Alliance: JARA-Energy 52425 Jülich Germany, RWTH Aachen University Institute of Mineral Engineering Department of Ceramics and Refractory Materials 52064 Aachen Germany
German Aerospace Center (DLR) Institute of Engineering Thermodynamics Pfaffenwaldring 38–40 70569 Stuttgart Germany, Helmholtz Institute Ulm for Electrochemical Energy Storage (HIU) Helmholtzstraße 11 89081 Ulm Germany, Ulm University, Institute of Electrochemistry Albert-Einstein-Allee 47 89081 Ulm Germany

Abstract All‐solid‐state batteries are considered as an enabler for applications requiring high energy and power density. However, they still fall short of their theoretical potential due to various limitations. One issue is poor charge transport kinetics resulting from both material inherit limitations and non‐optimized design. Therefore, a better understanding of the relevant properties of the cathode microstructure is necessary to improve cell performance. In this article, we identify optimization potentials of the composite cathode by structure‐resolved electrochemical 3D‐simulations. In our simulation study, we investigate the influence of cathode active material fraction, density, particle size, and active material properties on cell performance. Special focus is set on the impact of grain boundaries on the cathode design. Based on our simulation results, we can predict target values for cell manufacturing and reveal promising optimization strategies for an improved cathode design.

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Research Organization:: US DOE-German BMBF Cooperation, Washington DC (United States)

Sponsoring Organization:: USDOE

OSTI ID:: 1992393

Journal Information:: Batteries & Supercaps, Journal Name: Batteries & Supercaps Journal Issue: 11 Vol. 6; ISSN 2566-6223

Publisher:: Wiley Blackwell (John Wiley & Sons)Copyright Statement

Country of Publication:: Germany

Language:: English

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LLZO
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Title: Optimizing the Composite Cathode Microstructure in All‐Solid‐State Batteries by Structure‐Resolved Simulations

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