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Title: Symmetry Control of Unconventional Spin–Orbit Torques in IrO 2

Journal Article · · Advanced Materials
 [1];  [2];  [2];  [3];  [4];  [4];  [5];  [6];  [2];  [7];  [8];  [9];  [10]; ORCiD logo [1]
  1. Department of Materials Science and Engineering University of Wisconsin‐Madison Madison WI 53706 USA
  2. Department of Physics and Astronomy &, Nebraska Center for Materials and Nanoscience University of Nebraska Lincoln NE 68588 USA
  3. Department of Materials Science and Engineering Pohang University of Science and Technology Pohang Gyeongbuk 37673 Republic of Korea
  4. Cornell University Ithaca NY 14853 USA
  5. X‐Ray Science Division Argonne National Laboratory Argonne IL 60439 USA
  6. X‐Ray Science Division Argonne National Laboratory Argonne IL 60439 USA, School of Physical Sciences Dublin City University Dublin 9 Ireland
  7. Department of Materials Science and Engineering Pohang University of Science and Technology Pohang Gyeongbuk 37673 Republic of Korea, Center for Van der Waals Quantum Solids Institute for Basic Science (IBS) Pohang 37673 Republic of Korea, Semiconductor Engineering Pohang University of Science and Technology (POSTECH) Pohang 37673 Republic of Korea
  8. Cornell University Ithaca NY 14853 USA, Kavli Institute at Cornell for Nanoscale Science Ithaca NY 14853 USA
  9. Department of Physics University of Wisconsin‐Madison Madison WI 53706 USA
  10. School of Integrated Circuits and Beijing National Research Center for Information Science and Technology (BNRist) Tsinghua University Beijing 100084 China

Abstract Spin–orbit torques generated by a spin current are key to magnetic switching in spintronic applications. The polarization of the spin current dictates the direction of switching required for energy‐efficient devices. Conventionally, the polarizations of these spin currents are restricted to be along a certain direction due to the symmetry of the material allowing only for efficient in‐plane magnetic switching. Unconventional spin–orbit torques arising from novel spin current polarizations, however, have the potential to switch other magnetization orientations such as perpendicular magnetic anisotropy, which is desired for higher density spintronic‐based memory devices. Here, it is demonstrated that low crystalline symmetry is not required for unconventional spin–orbit torques and can be generated in a nonmagnetic high symmetry material, iridium dioxide (IrO 2 ), using epitaxial design. It is shown that by reducing the relative crystalline symmetry with respect to the growth direction large unconventional spin currents can be generated and hence spin–orbit torques. Furthermore, the spin polarizations detected in (001), (110), and (111) oriented IrO 2 thin films are compared to show which crystal symmetries restrict unconventional spin transport. Understanding and tuning unconventional spin transport generation in high symmetry materials can provide a new route towards energy‐efficient magnetic switching in spintronic devices.

Sponsoring Organization:
USDOE
Grant/Contract Number:
SC0017671; FG02-06ER46327
OSTI ID:
1991651
Alternate ID(s):
OSTI ID: 2404917; OSTI ID: 2203553; OSTI ID: 1995878
Journal Information:
Advanced Materials, Journal Name: Advanced Materials Journal Issue: 39 Vol. 35; ISSN 0935-9648
Publisher:
Wiley Blackwell (John Wiley & Sons)Copyright Statement
Country of Publication:
Germany
Language:
English

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