Puncture-resistant self-healing polymers with multi-cycle adhesion and rapid healability

Li, Bingrui; Ge, Sirui; Zhao, Sheng; Xing, Kunyue; Sokolov, Alexei P.; Cao, Peng-Fei; Saito, Tomonori

doi:10.1039/D3MH00481C

Title: Puncture-resistant self-healing polymers with multi-cycle adhesion and rapid healability

Journal Article · 31 July 2023 · Materials Horizons

DOI: https://doi.org/10.1039/D3MH00481C · OSTI ID:1988180

^[1];

^[2]; Zhao, Sheng ^[3]; Xing, Kunyue ^[3];

^[4];

^[5];

^[6]

The Bredesen Center for Interdisciplinary Research and Graduate Education, University of Tennessee, Knoxville, Tennessee 37996, USA
Department of Material Science and Engineering, University of Tennessee, Knoxville, Tennessee 37996, USA
Department of Chemistry, University of Tennessee, Knoxville, Tennessee 37996, USA
Department of Chemistry, University of Tennessee, Knoxville, Tennessee 37996, USA, Chemical Sciences Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37830, USA
Chemical Sciences Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37830, USA, State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing 100029, China
Chemical Sciences Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37830, USA

Tuning the chemical and physical crosslinks of poly(dimethyl siloxane)-based elastomers enables significantly enhanced puncture-resistant property with rapid self-healing capability.

View Journal Article

Cite

Export

Save

Sponsoring Organization:: USDOE

OSTI ID:: 1988180

Journal Information:: Materials Horizons, Journal Name: Materials Horizons Journal Issue: 8 Vol. 10; ISSN 2051-6347; ISSN MHAOAL

Publisher:: Royal Society of Chemistry (RSC)Copyright Statement

Country of Publication:: United Kingdom

Language:: English

References (46)

Superstretchable, Self-Healing Polymeric Elastomers with Tunable Properties Cao, Peng-Fei; Li, Bingrui; Hong, Tao Advanced Functional Materials, Vol. 28, Issue 22 https://doi.org/10.1002/adfm.201800741	journal	April 2018
Biomimetic Materials with Multiple Protective Functionalities Liu, Zenghe; Zhang, Luzhi; Guan, Qingbao Advanced Functional Materials, Vol. 29, Issue 28 https://doi.org/10.1002/adfm.201901058	journal	May 2019
Autonomous Self‐Healing Elastomers with Unprecedented Adhesion Force Zhang, Zhen; Ghezawi, Natasha; Li, Bingrui Advanced Functional Materials, Vol. 31, Issue 4 https://doi.org/10.1002/adfm.202006298	journal	October 2020
A Puncture‐Resistant and Self‐Healing Conductive Gel for Multifunctional Electronic Skin Hou, Ke‐Xin; Zhao, Shu‐Peng; Wang, Da‐Peng Advanced Functional Materials, Vol. 31, Issue 49 https://doi.org/10.1002/adfm.202107006	journal	September 2021
All Spraying Processes for the Fabrication of Robust, Self-Healing, Superhydrophobic Coatings Li, Yang; Chen, Shanshan; Wu, Mengchun Advanced Materials, Vol. 26, Issue 20 https://doi.org/10.1002/adma.201306136	journal	March 2014
Tough Self-Healing Elastomers by Molecular Enforced Integration of Covalent and Reversible Networks Wu, Jinrong; Cai, Li-Heng; Weitz, David A. Advanced Materials, Vol. 29, Issue 38 https://doi.org/10.1002/adma.201702616	journal	August 2017
Tough and Water-Insensitive Self-Healing Elastomer for Robust Electronic Skin Kang, Jiheong; Son, Donghee; Wang, Ging-Ji Nathan Advanced Materials, Vol. 30, Issue 13 https://doi.org/10.1002/adma.201706846	journal	February 2018
An Elastic Autonomous Self-Healing Capacitive Sensor Based on a Dynamic Dual Crosslinked Chemical System Zhang, Qiuhong; Niu, Simiao; Wang, Li Advanced Materials, Vol. 30, Issue 33 https://doi.org/10.1002/adma.201801435	journal	July 2018
A Highly Efficient Self‐Healing Elastomer with Unprecedented Mechanical Properties Zhang, Luzhi; Liu, Zenghe; Wu, Xueli Advanced Materials, Vol. 31, Issue 23 https://doi.org/10.1002/adma.201901402	journal	March 2019
Self‐Healing Soft Sensors: From Material Design to Implementation Khatib, Muhammad; Zohar, Orr; Haick, Hossam Advanced Materials, Vol. 33, Issue 11 https://doi.org/10.1002/adma.202004190	journal	February 2021
Molecularly Engineered Unparalleled Strength and Supertoughness of Poly(urea‐urethane) with Shape Memory and Clusterization‐Triggered Emission Wang, Xiaoyue; Xu, Jing; Zhang, Xinrui Advanced Materials, Vol. 34, Issue 45 https://doi.org/10.1002/adma.202205763	journal	October 2022
Extremely Strong and Tough Biodegradable Poly(urethane) Elastomers with Unprecedented Crack Tolerance via Hierarchical Hydrogen‐Bonding Interactions Guo, Rui; Zhang, Qiang; Wu, Youshen Advanced Materials, Vol. 35, Issue 21 https://doi.org/10.1002/adma.202212130	journal	March 2023
Super Tough and Spontaneous Water‐Assisted Autonomous Self‐Healing Elastomer for Underwater Wearable Electronics He, Cyuan‐Lun; Liang, Fang‐Cheng; Veeramuthu, Loganathan Advanced Science, Vol. 8, Issue 21 https://doi.org/10.1002/advs.202102275	journal	September 2021
Towards Dynamic but Supertough Healable Polymers through Biomimetic Hierarchical Hydrogen-Bonding Interactions Song, Yan; Liu, Yuan; Qi, Tao Angewandte Chemie International Edition, Vol. 57, Issue 42 https://doi.org/10.1002/anie.201807622	journal	September 2018
MoS2 core-shell nanoparticles prepared through liquid-phase ablation and light exfoliation of femtosecond laser for chemical sensing Zuo, Pei; Jiang, Lan; Li, Xin Science China Technological Sciences, Vol. 66, Issue 3 https://doi.org/10.1007/s11431-022-2270-9	journal	February 2023
Dual dynamic network system constructed by waterborne polyurethane for improved and recoverable performances Liang, Rihui; Zhang, Haotian; Wang, Yuhang Chemical Engineering Journal, Vol. 442 https://doi.org/10.1016/j.cej.2022.136204	journal	August 2022
A novel, high strength, ultra-fast room temperature self-healing elastomers via structural functional region optimization strategy Jing, Tu; Heng, Xu; Jingqing, Tian Chemical Engineering Journal, Vol. 465 https://doi.org/10.1016/j.cej.2023.142887	journal	June 2023
Construction of synergistic Toughening, Self-Healing Puncture-Resistant soft composites by using Fabric-Reinforced Pluronic/PMEA hydrogel Li, Ting-Ting; Xing, Mengfan; Gao, Bo Composites Part A: Applied Science and Manufacturing, Vol. 145 https://doi.org/10.1016/j.compositesa.2021.106388	journal	June 2021
The self-healing sandwich panel: Production of epoxy based self-healing capsules, self-healable sandwich panel development, and experimental measurement of self-healing performance Özer, Hakkı; Kuzu, Eslem; Özada, Çağatay Construction and Building Materials, Vol. 310 https://doi.org/10.1016/j.conbuildmat.2021.125303	journal	December 2021
A self-healing transparent polydimethylsiloxane elastomer based on imine bonds Wang, Peng; Yang, Lei; Dai, Bing European Polymer Journal, Vol. 123 https://doi.org/10.1016/j.eurpolymj.2019.109382	journal	January 2020
Intrinsically Self-Healing Polymers: From Mechanistic Insight to Current Challenges Li, Bingrui; Cao, Peng-Fei; Saito, Tomonori Chemical Reviews, Vol. 123, Issue 2 https://doi.org/10.1021/acs.chemrev.2c00575	journal	December 2022
Room-Temperature Self-Healing Polymers Based on Dynamic-Covalent Boronic Esters Cash, Jessica J.; Kubo, Tomohiro; Bapat, Abhijeet P. Macromolecules, Vol. 48, Issue 7 https://doi.org/10.1021/acs.macromol.5b00210	journal	March 2015
Mechanically Robust, Self-Healing, Polymer Blends and Polymer/Small Molecule Blend Materials with High Antibacterial Activity Du, Juan; Li, Yangyang; Wang, Jiuchun ACS Applied Materials & Interfaces, Vol. 12, Issue 24 https://doi.org/10.1021/acsami.0c06591	journal	May 2020
Extremely Tough, Puncture-Resistant, Transparent, and Photoluminescent Polyurethane Elastomers for Crack Self-Diagnose and Healing Tracking Chen, Xingxing; Zhong, Qianyun; Cui, Chenhui ACS Applied Materials & Interfaces, Vol. 12, Issue 27 https://doi.org/10.1021/acsami.0c07727	journal	June 2020
Tuning the Self-Healing Response of Poly(dimethylsiloxane)-Based Elastomers Döhler, Diana; Kang, Jiheong; Cooper, Chris Brittain ACS Applied Polymer Materials, Vol. 2, Issue 9 https://doi.org/10.1021/acsapm.0c00755	journal	August 2020
Biomimetic Tough Self-Healing Polymers Enhanced by Crystallization Nanostructures Wan, Dong; Jiang, Qingling; Song, Yan ACS Applied Polymer Materials, Vol. 2, Issue 2 https://doi.org/10.1021/acsapm.9b01094	journal	January 2020
A Tough and Self-Healing Polymer Enabled by Promoting Bond Exchange in Boronic Esters with Neighboring Hydroxyl Groups Zhao, Zi-Han; Wang, Da-Peng; Zuo, Jing-Lin ACS Materials Letters, Vol. 3, Issue 9 https://doi.org/10.1021/acsmaterialslett.1c00314	journal	August 2021
Self-Healable, Malleable, and Flexible Ionic Polyimine as an Environmental Sensor for Portable Exogenous Pollutant Detection Zhang, Guo-Hao; Zhang, Lei; Zhu, Qiu-Hong ACS Materials Letters, Vol. 4, Issue 1 https://doi.org/10.1021/acsmaterialslett.1c00687	journal	December 2021
Highly Conductive Self-Healable Rhenium Oxide–Polytetrahydrofuran Composite for Resilient Flexible Electrode Jeong, Byeong-Yong; Lee, Sojeong; Shin, Hyun Ho ACS Materials Letters, Vol. 4, Issue 10 https://doi.org/10.1021/acsmaterialslett.2c00606	journal	September 2022
DFT-Calculated IR Spectrum Amide I, II, and III Band Contributions of N-Methylacetamide Fine Components Ji, Yan; Yang, Xiaoliang; Ji, Zhi ACS Omega, Vol. 5, Issue 15 https://doi.org/10.1021/acsomega.9b04421	journal	April 2020
“Flex-Activated” Mechanophores: Using Polymer Mechanochemistry To Direct Bond Bending Activation Larsen, Michael B.; Boydston, Andrew J. Journal of the American Chemical Society, Vol. 135, Issue 22 https://doi.org/10.1021/ja403757p	journal	May 2013
Self-Healing Materials Based on Disulfide Links Canadell, Judit; Goossens, Han; Klumperman, Bert Macromolecules, Vol. 44, Issue 8 https://doi.org/10.1021/ma2001492	journal	April 2011
Self-healing and thermoreversible rubber from supramolecular assembly Cordier, Philippe; Tournilhac, François; Soulié-Ziakovic, Corinne Nature, Vol. 451, Issue 7181, p. 977-980 https://doi.org/10.1038/nature06669	journal	February 2008
Optically healable supramolecular polymers Burnworth, Mark; Tang, Liming; Kumpfer, Justin R. Nature, Vol. 472, Issue 7343, p. 334-337 https://doi.org/10.1038/nature09963	journal	April 2011
A rigid and healable polymer cross-linked by weak but abundant Zn(II)-carboxylate interactions Lai, Jian-Cheng; Li, Lan; Wang, Da-Peng Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-05285-3	journal	July 2018
Universally autonomous self-healing elastomer with high stretchability Guo, Hongshuang; Han, Yi; Zhao, Weiqiang Nature Communications, Vol. 11, Issue 1 https://doi.org/10.1038/s41467-020-15949-8	journal	April 2020
Self-healing soft electronics Kang, Jiheong; Tok, Jeffrey B. -H.; Bao, Zhenan Nature Electronics, Vol. 2, Issue 4 https://doi.org/10.1038/s41928-019-0235-0	journal	April 2019
An ultrafast self-healing polydimethylsiloxane elastomer with persistent sealing performance Wang, Da-Peng; Zhao, Zi-Han; Li, Cheng-Hui Materials Chemistry Frontiers, Vol. 3, Issue 7 https://doi.org/10.1039/C9QM00115H	journal	January 2019
Advances in intrinsic self-healing polyurethanes and related composites Willocq, Bertrand; Odent, Jérémy; Dubois, Philippe RSC Advances, Vol. 10, Issue 23 https://doi.org/10.1039/D0RA01394C	journal	January 2020
Transparent, self-recoverable, highly tough, puncture and tear resistant polyurethane supramolecular elastomer with fast self-healing capacityvia“hard–soft” hard domain design Xu, Kangming; Chen, Guoqing; Zhao, Mingjie RSC Advances, Vol. 12, Issue 5 https://doi.org/10.1039/D1RA07083E	journal	January 2022
Self-healing polymers based on thermally reversible Diels–Alder chemistry Liu, Ying-Ling; Chuo, Tsai-Wei Polymer Chemistry, Vol. 4, Issue 7 https://doi.org/10.1039/c2py20957h	journal	January 2013
Mechanical characterization of bulk Sylgard 184 for microfluidics and microengineering Johnston, I. D.; McCluskey, D. K.; Tan, C. K. L. Journal of Micromechanics and Microengineering, Vol. 24, Issue 3 https://doi.org/10.1088/0960-1317/24/3/035017	journal	February 2014
Peptidoglycan-inspired autonomous ultrafast self-healing bio-friendly elastomers for bio-integrated electronics Zhang, Luzhi; Liang, Jiahui; Jiang, Chenyu National Science Review, Vol. 8, Issue 5 https://doi.org/10.1093/nsr/nwaa154	journal	July 2020
Stretchable self-healable semiconducting polymer film for active-matrix strain-sensing array Oh, Jin Young; Son, Donghee; Katsumata, Toru Science Advances, Vol. 5, Issue 11 https://doi.org/10.1126/sciadv.aav3097	journal	November 2019
Design of tough adhesive from commodity thermoplastics through dynamic crosslinking Rahman, Md Anisur; Bowland, Christopher; Ge, Sirui Science Advances, Vol. 7, Issue 42 https://doi.org/10.1126/sciadv.abk2451	journal	October 2021
A Novel Dynamic Polymer Synthesis via Chlorinated Solvent Quenched Depolymerization Zhu, Jiadeng; Zhao, Sheng; Luo, Jiancheng CCS Chemistry https://doi.org/10.31635/ccschem.022.202202362	journal	October 2022

Similar Records

Superstretchable, Self-Healing Polymeric Elastomers with Tunable Properties

Journal Article · 2018 · Advanced Functional Materials · OSTI ID:1435198

Cao, Peng-Fei; Li, Bingrui; Hong, Tao; +8 more

Self-healing Polymers and Composites

Journal Article · · Annual Review of Materials Research · OSTI ID:1065681

Blaiszik, B. J.; Kramer, S. L. B.; Olugebefola, S. C.; +3 more

Autonomous Self-Healing Elastomers with Unprecedented Adhesion Force

Journal Article · 2020 · Advanced Functional Materials · OSTI ID:1777768

Zhang, Zhen; Ghezawi, Natasha; Li, Bingrui; +5 more

Title: Puncture-resistant self-healing polymers with multi-cycle adhesion and rapid healability

Citation Formats

References (46)

Similar Records

Related Subjects