Radionuclide Transport Simulations Supporting Proposed Borehole Waste Disposal in Israel

Journal Article · 03 June 2023 · Geosciences

DOI: https://doi.org/10.3390/geosciences13060166 · OSTI ID:1985867

Swager, Katherine Carol ^[1]; Bourret, Suzanne Michelle  ^[1]; Bussod, Gilles Yves A.  ^[1]; Balaban, Noa ^[2]; Boukhalfa, Hakim  ^[1]; Calvo, Ran  ^[3]; Klein-BenDavid, Ofra ^[2]; Lucero, Dolan Diego ^[1]; Reznik, Itay J.  ^[3]; Rosenzweig, Ravid  ^[3]; Stauffer, Philip H.  ^[1]

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1. Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
2. Nuclear Research Center Negev (NRCN), Beer-Sheva (Israel)
3. Geological Survey of Israel, Jerusalem (Israel)

A scientific collaboration between the U.S. and Israel is underway to assess the suitability of a potential site for subsurface radioactive waste disposal in the Negev Desert, Israel. The Negev Desert has several favorable attributes for geologic disposal, including an arid climate, a deep vadose zone, interlayered low-permeability lithologies, and carbonate rocks with high uranium-sorption potential. These features may provide a robust natural barrier to radionuclide migration. Geologic and laboratory characterization data from the Negev Desert are incorporated into multiphase flow and transport models, solved using PFLOTRAN, to aid in site characterization and risk analysis that will support decision-making for waste disposal in an intermediate-depth borehole design. The lithology with the greatest uranium sorption potential at the site is phosphorite. We use modeling to evaluate the ability of this layer to impact uranium transport around a proposed disposal borehole. The current objective of the simulations is focused on characterizing hypothetical leakage from waste canisters and subsequent uranium migration under three infiltration scenarios. Here, we describe a hydrogeologic model based on data from a local exploratory borehole and present results for uranium flow and transport simulations under varying infiltration scenarios. We find that under the current climate conditions, it is likely that uranium will remain in the near-field of the borehole for thousands of years. However, under a hypothesized extreme climate scenario representing an increase in infiltration by a factor of 300x above present-day values, uranium may break through the phosphorite layer and exit the base of the model domain (~200 m above the water table) within 1000 years. Simulation results have direct implications for the planning of nuclear waste disposal in the Negev Desert, and specifically in intermediate-depth boreholes.

• Research Organization: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
• Sponsoring Organization: USDOE National Nuclear Security Administration (NNSA)
• Grant/Contract Number: 89233218CNA000001
• OSTI ID: 1985867
• Report Number(s): LA-UR-23-24315
• Journal Information: Geosciences, Vol. 13, Issue 6; ISSN 2076-3263
• Publisher: MDPICopyright Statement
• Country of Publication: United States
• Language: English