Field-induced partial disorder in a Shastry-Sutherland lattice

Marshall, Madalynn; Billingsley, Brianna R.; Bai, Xiaojian; Ma, Qianli; Kong, Tai; Cao, Huibo

doi:10.1038/s41467-023-39409-1

Title: Field-induced partial disorder in a Shastry-Sutherland lattice

Journal Article · 19 June 2023 · Nature Communications

DOI: https://doi.org/10.1038/s41467-023-39409-1 · OSTI ID:1985731

Marshall, Madalynn; Billingsley, Brianna R.; Bai, Xiaojian; Ma, Qianli;

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Abstract A 2-Q antiferromagnetic order of the ferromagnetic dimers was found below T _N = 2.9 K in the Shastry-Sutherland lattice BaNd ₂ ZnS ₅ by single crystal neutron diffraction. The magnetic order can be understood by the orthogonal arrangement of local Ising Nd spins, identified by polarized neutrons. A field was applied along [1 -1 0] to probe the observed metamagnetic transition in the magnetization measurement. The field decouples two magnetic sublattices corresponding to the propagation vectors q ₁ = (½, ½, 0) and q ₂ = (−½, ½, 0), respectively. Each sublattice shows a “stripe” order with a Néel-type arrangement in each single layer. The “stripe” order with q ₁ remains nearly intact up to 6 T, while the other one with q ₂ is suppressed at a critical field H _c ~1.7 T, indicating a partial disorder. The H _c varies with temperature and is manifested in the H - T phase diagram constructed by measuring the magnetization in BaNd ₂ ZnS ₅ .

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Sponsoring Organization:: USDOE

OSTI ID:: 1985731

Journal Information:: Nature Communications, Journal Name: Nature Communications Journal Issue: 1 Vol. 14; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United Kingdom

Language:: English

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