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Title: Isospin magnetism and spin-polarized superconductivity in Bernal bilayer graphene

Journal Article · · Science

In conventional superconductors, Cooper pairing occurs between electrons of opposite spin. We observe spin-polarized superconductivity in Bernal bilayer graphene when doped to a saddle-point van Hove singularity generated by a large applied perpendicular electric field. We observe a cascade of electrostatic gate-tuned transitions between electronic phases distinguished by their polarization within the isospin space defined by the combination of the spin and momentum-space valley degrees of freedom. Although all of these phases are metallic at zero magnetic field, we observe a transition to a superconducting state at finite magnetic field B≈ 150 milliteslas applied parallel to the two-dimensional sheet. Superconductivity occurs near a symmetry-breaking transition and exists exclusively above the B limit expected of a paramagnetic superconductor with the observed transition critical temperature TC ≈ 30 millikelvins, consistent with a spin-triplet order parameter.

Research Organization:
University of California, Santa Barbara, CA (United States)
Sponsoring Organization:
USDOE Office of Science (SC); Army Research Office (ARO); Gordon and Betty Moore Foundation; Packard Foundation; Ministry of Education, Culture, Sports, Science and Technology (MEXT); Japan Society for the Promotion of Science (JSPS)
Grant/Contract Number:
SC0020043
OSTI ID:
1980741
Journal Information:
Science, Journal Name: Science Journal Issue: 6582 Vol. 375; ISSN 0036-8075
Publisher:
AAASCopyright Statement
Country of Publication:
United States
Language:
English

References (47)

Theory of dirty superconductors journal September 1959
Electrode-Free Anodic Oxidation Nanolithography of Low-Dimensional Materials journal November 2018
Direct observation of a widely tunable bandgap in bilayer graphene journal June 2009
Tunable interacting composite fermion phases in a half-filled bilayer-graphene Landau level journal September 2017
Unconventional superconductivity in magic-angle graphene superlattices journal March 2018
Unconventional quantum Hall effect and Berry’s phase of 2π in bilayer graphene journal February 2006
Ising pairing in superconducting NbSe2 atomic layers journal November 2015
Inter-valley coherent order and isospin fluctuation mediated superconductivity in rhombohedral trilayer graphene journal October 2022
Superconductivity and strong correlations in moiré flat bands journal May 2020
Dynamic band-structure tuning of graphene moiré superlattices with pressure journal May 2018
Spin–orbit-driven band inversion in bilayer graphene by the van der Waals proximity effect journal June 2019
Tunable strongly coupled superconductivity in magic-angle twisted trilayer graphene journal February 2021
Pauli-limit violation and re-entrant superconductivity in moiré graphene journal July 2021
Superconductivity in rhombohedral trilayer graphene journal September 2021
Half- and quarter-metals in rhombohedral trilayer graphene journal September 2021
A note on the Maximum Critical Field of High‐Field Superconductors journal September 1962
Evidence for a spontaneous gapped state in ultraclean bilayer graphene journal June 2012
Ising pairing in atomically thin superconductors journal September 2021
Superconductivity from repulsive interactions in rhombohedral trilayer graphene: A Kohn-Luttinger-like mechanism journal February 2022
Kohn-Luttinger superconductivity and intervalley coherence in rhombohedral trilayer graphene journal April 2022
Metals, fractional metals, and superconductivity in rhombohedral trilayer graphene journal February 2022
Compressibility of the two-dimensional electron gas: Measurements of the zero-field exchange energy and fractional quantum Hall gap journal July 1994
Magnetotransport in a two-dimensional electron gas at large filling factors journal January 2004
Intrinsic and Rashba spin-orbit interactions in graphene sheets journal October 2006
Trigonal warping and Berry’s phase N π in ABC-stacked multilayer graphene journal October 2009
Band structure of A B C -stacked graphene trilayers journal July 2010
Accurate tight-binding models for the π bands of bilayer graphene journal January 2014
Universal phase diagrams with superconducting domes for electronic flat bands journal August 2017
Competition of electron-phonon mediated superconductivity and Stoner magnetism on a flat band journal August 2018
Low-Density Ferromagnetism in Biased Bilayer Graphene journal May 2008
Spontaneously Gapped Ground State in Suspended Bilayer Graphene journal February 2012
Superconductivity on the Brink of Spin-Charge Order in a Doped Honeycomb Bilayer journal April 2014
Resonance Microwave Measurements of an Intrinsic Spin-Orbit Coupling Gap in Graphene: A Possible Indication of a Topological State journal February 2019
Acoustic-Phonon-Mediated Superconductivity in Rhombohedral Trilayer Graphene journal October 2021
Unconventional Superconductivity in Systems with Annular Fermi Surfaces: Application to Rhombohedral Trilayer Graphene journal December 2021
Sliding-Mode Conductivity in Nb Se 3 : Observation of a Threshold Electric Field and Conduction Noise journal May 1979
Upper Limit for the Critical Field in Hard Superconductors journal September 1962
Pairing symmetry in cuprate superconductors journal October 2000
Magnetic Field-Induced Superconductivity in the Ferromagnet URhGe journal August 2005
Broken-Symmetry States in Doubly Gated Suspended Bilayer Graphene journal October 2010
Interaction-Driven Spectrum Reconstruction in Bilayer Graphene journal August 2011
One-Dimensional Electrical Contact to a Two-Dimensional Material journal October 2013
Evidence for two-dimensional Ising superconductivity in gated MoS2 journal November 2015
Nearly ferromagnetic spin-triplet superconductivity journal August 2019
Electric field–tunable superconductivity in alternating-twist magic-angle trilayer graphene journal February 2021
Isospin magnetism and spin-polarized superconductivity in Bernal bilayer graphene dataset January 2021
Review of U-based Ferromagnetic Superconductors: Comparison between UGe 2 , URhGe, and UCoGe journal February 2019