Nonlinear quantum interferometric spectroscopy with entangled photon pairs

Asban, Shahaf; Chernyak, Vladimir Y.; Mukamel, Shaul

doi:10.1063/5.0079049

Title: Nonlinear quantum interferometric spectroscopy with entangled photon pairs

Journal Article · 03 March 2022 · Journal of Chemical Physics

DOI: https://doi.org/10.1063/5.0079049 · OSTI ID:1979017

^[1]; Chernyak, Vladimir Y. ^[2];

^[3]

Univ. of California, Irvine, CA (United States); Wayne State Univ., Detroit, MI (United States)
Wayne State Univ., Detroit, MI (United States)
Univ. of California, Irvine, CA (United States)

Here, we develop closed expressions for a time-resolved photon counting signal induced by an entangled photon pair in an interferometric spectroscopy setup. Superoperator expressions in Liouville-space are derived that can account for relaxation and dephasing induced by coupling to a bath. Interferometric setups mix matter and light variables non-trivially, which complicates their interpretation. We provide an intuitive modular framework for this setup that simplifies its description. Based on the separation between the detection stage and the light–matter interaction processes, we show that the pair entanglement time and the interferometric time-variables control the observed physics time scale. Only a few processes contribute in the limiting case of small entanglement time with respect to the sample response, and specific contributions can be singled out.

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Research Organization:: Wayne State Univ., Detroit, MI (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF)

Grant/Contract Number:: SC0022134

OSTI ID:: 1979017

Journal Information:: Journal of Chemical Physics, Journal Name: Journal of Chemical Physics Journal Issue: 9 Vol. 156; ISSN 0021-9606

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

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Title: Nonlinear quantum interferometric spectroscopy with entangled photon pairs

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