Aerodynamic effects on outer ash deposition rates in second generation atmospheric pressure oxy-coal combustion systems

Journal Article · Tue Jun 15 00:00:00 UTC 2021 · Fuel

DOI: https://doi.org/10.1016/j.fuel.2021.121217 · OSTI ID:1977128

Krishnamoorthy, Gautham ^[1]; Kuznia, Monika E. ^[2]; Smith, KayLee M. ^[2]; Seames, Wayne S. ^[2]; Wang, Yueming ^[3]; Wendt, Jost O.L. ^[3]

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1. University of North Dakota, Grand Forks, ND (United States); OSTI
2. University of North Dakota, Grand Forks, ND (United States)
3. University of Utah, Salt Lake City, UT (United States)

Recent measurements in scenarios representative of second generation atmospheric pressure oxy-coal combustion systems have shown a significant increase in ash deposition rates in comparison to combustion in air. However, the causative mechanisms behind this increase have not been well understood. To fill this void, well-characterized experiments including fuel and deposit particle size distributions (PSDs) were coupled with highly resolved numerical simulations to isolate the aerodynamic effects impacting the deposition process such that mechanisms could be hypothesized. Three combustion scenarios (AIR, OXY27, OXY70) spanning a factor of three variation in flue gas volumetric flow rates were simulated and the deposition characteristics (impaction rates, deposit PSD, temperature, residence times, capture rates) tracked/predicted using a customized deposition module. The measured deposit PSD was significantly different from the PSD of the parent fuel indicating significant physio-chemical transformations (coalescence and particle growth in particular) at play. The use of simplistic modeling approaches (swelling parameter variations) to model particle growth led to inaccurate deposit ash PSD and rate predictions. A more satisfactory agreement between the measurements and simulations was obtained when the functional form of the parent fuel PSD (spread parameter) was modified to conform closely to the deposit PSD while still ensuring the fidelity of temperature and velocity predictions. Based on the measured ash compositions, identical capture criteria were employed across all three scenarios. Here this study further supports the theory that the ash deposition rates in these systems are dominated by aerodynamic effects with the ash PSD playing a dominant role.

• Research Organization: University of North Dakota, Grand Forks, ND (United States)
• Sponsoring Organization: National Science Foundation (NSF); USDOE Office of Fossil Energy (FE)
• Grant/Contract Number: FE0031741
• OSTI ID: 1977128
• Journal Information: Fuel, Journal Name: Fuel Journal Issue: C Vol. 303; ISSN 0016-2361
• Publisher: ElsevierCopyright Statement
• Country of Publication: United States
• Language: English