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Title: Does plasma jet sintering follow an Arrhenius-type expression?

Abstract

Abstract Atmospheric pressure, ambient temperature plasma jets have become a promising candidate for material processing in parallel with developments in additive manufacturing. Recent work has shown that plasma jets can be used to sinter printed nanoparticles at temperatures much lower than typically required for conventional thermal sintering. Here, we conduct a mechanistic study on plasma jet sintering that correlates specific energy input with the electrical conductivity of printed silver films after sintering. Increasing the specific energy input accelerated the sintering process following an Arrhenius‐like exponential trend across a large range of conditions, including both helium and argon plasma jets. Although an exponential relationship is also found with the plasma heated substrate temperature, independent studies indicate that heating is not the primary mechanism. These results suggest there is a general behavior that couples the plasma jet with the surface.

Authors:
ORCiD logo [1];  [1];  [1];  [1]
  1. University of Notre Dame, IN (United States)
Publication Date:
Research Org.:
University of Notre Dame, IN (United States)
Sponsoring Org.:
USDOE Office of Energy Efficiency and Renewable Energy (EERE); US Air Force Office of Scientific Research (AFOSR); National Science Foundation (NSF)
OSTI Identifier:
1976372
Alternate Identifier(s):
OSTI ID: 1866497
Grant/Contract Number:  
EE0009103; FA9550- 18-1-0157; CMMI-1747685; DEEE0009103
Resource Type:
Accepted Manuscript
Journal Name:
Plasma Processes and Polymers
Additional Journal Information:
Journal Volume: 19; Journal Issue: 8; Journal ID: ISSN 1612-8850
Publisher:
Wiley
Country of Publication:
United States
Language:
English
Subject:
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; 70 PLASMA PHYSICS AND FUSION TECHNOLOGY; plasma jet; specific energy input; sintering

Citation Formats

Turan, Nazli, Saeidi‐Javash, Mortaza, Zhang, Yanliang, and Go, David B. Does plasma jet sintering follow an Arrhenius-type expression?. United States: N. p., 2022. Web. doi:10.1002/ppap.202200011.
Turan, Nazli, Saeidi‐Javash, Mortaza, Zhang, Yanliang, & Go, David B. Does plasma jet sintering follow an Arrhenius-type expression?. United States. https://doi.org/10.1002/ppap.202200011
Turan, Nazli, Saeidi‐Javash, Mortaza, Zhang, Yanliang, and Go, David B. Wed . "Does plasma jet sintering follow an Arrhenius-type expression?". United States. https://doi.org/10.1002/ppap.202200011. https://www.osti.gov/servlets/purl/1976372.
@article{osti_1976372,
title = {Does plasma jet sintering follow an Arrhenius-type expression?},
author = {Turan, Nazli and Saeidi‐Javash, Mortaza and Zhang, Yanliang and Go, David B.},
abstractNote = {Abstract Atmospheric pressure, ambient temperature plasma jets have become a promising candidate for material processing in parallel with developments in additive manufacturing. Recent work has shown that plasma jets can be used to sinter printed nanoparticles at temperatures much lower than typically required for conventional thermal sintering. Here, we conduct a mechanistic study on plasma jet sintering that correlates specific energy input with the electrical conductivity of printed silver films after sintering. Increasing the specific energy input accelerated the sintering process following an Arrhenius‐like exponential trend across a large range of conditions, including both helium and argon plasma jets. Although an exponential relationship is also found with the plasma heated substrate temperature, independent studies indicate that heating is not the primary mechanism. These results suggest there is a general behavior that couples the plasma jet with the surface.},
doi = {10.1002/ppap.202200011},
journal = {Plasma Processes and Polymers},
number = 8,
volume = 19,
place = {United States},
year = {2022},
month = {5}
}

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