Two-dimensional glass transition–like behavior of Janus particle–laden interface

Correia, Elton L.; Winter, H. Henning; Razavi, Sepideh

doi:10.1007/s00397-023-01389-w

Title: Two-dimensional glass transition–like behavior of Janus particle–laden interface

Journal Article · 21 March 2023 · Rheologica Acta

DOI: https://doi.org/10.1007/s00397-023-01389-w · OSTI ID:1962897

Correia, Elton L.; Winter, H. Henning;

Abstract Understanding the interactive behavior of Janus particles (JPs) is a growing field of research. The enhancement in binding energy, in comparison to homogenous particles, and the dual characteristic of JPs open up new possibilities for novel applications. In many such applications, interfacial materials become subjected to flows that produce dilational and shear stresses. Therefore, it is important to understand the impact that the Janus character brings to interfaces. In this work, we study the microstructure of two-dimensional (2D) JP monolayers formed at the air–water interface and examine the shear viscoelasticity with an interface rheometer that was adapted for in situ surface pressure control via a Langmuir trough. We extend concepts from bulk rheology to data obtained from interfacial rheology as a tool to understand and predict the monolayer’s viscoelastic behavior. Finally, by calculating the time relaxation spectrum from the measured 2D dynamic moduli, we conclude that a phenomenon similar to glass transition is taking place by analogy.

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Research Organization:: Univ. of Wisconsin, Madison, WI (United States); Universities of Wisconsin, Madison, WI (United States)

Sponsoring Organization:: American Chemical Society, Petroleum Research Fund; USDOE; USDOE Office of Energy Efficiency and Renewable Energy (EERE), Office of Sustainable Transportation. Bioenergy Technologies Office (BETO)

Grant/Contract Number:: EE0009285

OSTI ID:: 1962897

Journal Information:: Rheologica Acta, Journal Name: Rheologica Acta Journal Issue: 4 Vol. 62; ISSN 0035-4511

Publisher:: Springer Science + Business MediaCopyright Statement

Country of Publication:: Germany

Language:: English

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42 ENGINEERING
BSW spectrum
Interfacial rheology
Janus particles
Janus particles
Particle-laden fluid interfaces
Interfacial rheology
Time-pressure superposition
BSW spectrum
Particle-laden fluid interfaces
Time-pressure superposition

Title: Two-dimensional glass transition–like behavior of Janus particle–laden interface

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