Challenge-driven printing strategies toward high-performance solid-state lithium batteries

Wang, Jing; Huang, Xingkang; Chen, Junhong

doi:10.1039/d1ta09322c

Title: Challenge-driven printing strategies toward high-performance solid-state lithium batteries

Journal Article · 06 January 2022 · Journal of Materials Chemistry. A

DOI: https://doi.org/10.1039/d1ta09322c · OSTI ID:1903786

Wang, Jing ^[1];

^[1];

^[1]

Univ. of Chicago, IL (United States); Argonne National Lab. (ANL), Lemont, IL (United States)

Solid-state lithium batteries (SSLBs) are promising candidates for replacing traditional liquid-based Li-ion batteries and revolutionizing battery systems for electric vehicles and portable devices. However, longstanding issues such as form factors, interfacial contact resistance, balance between ion conductivity and mechanical strength, and manufacturing processability limit their applications. In this review we present how advanced printing technologies can help to mitigate typical problems in main components of SSLBs and improve device performance. Here we first introduce the common printing techniques for energy storage devices, then focus on the issues and corresponding printing strategies for anodes, cathodes, and solid-state electrolytes to guide the construction of energy-dense, free-form SSLBs. The features and effects of the printed structures are emphasized, as well. We conclude by discussing the problems associated with printing technologies and the potential research directions for printed solid-state batteries.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: National Science Foundation (NSF); USDOE

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1903786

Journal Information:: Journal of Materials Chemistry. A, Journal Name: Journal of Materials Chemistry. A Journal Issue: 6 Vol. 10; ISSN 2050-7488

Publisher:: Royal Society of ChemistryCopyright Statement

Country of Publication:: United States

Language:: English

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25 ENERGY STORAGE

Title: Challenge-driven printing strategies toward high-performance solid-state lithium batteries

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