Forty years of durability assessment of nuclear waste glass by standard methods

Thorpe, Clare L.; Neeway, James J.; Pearce, Carolyn I.; Hand, Russell J.; Fisher, Adam J.; Walling, Sam A.; Hyatt, Neil C.; Kruger, Albert A.; Schweiger, Michael; Kosson, David S.; Arendt, Christina L.; Marcial, Jose; Corkhill, Claire L.

doi:10.1038/s41529-021-00210-4

Title: Forty years of durability assessment of nuclear waste glass by standard methods

Journal Article · 19 December 2021 · npj Materials Degradation

DOI: https://doi.org/10.1038/s41529-021-00210-4 · OSTI ID:1902514

;

; Fisher, Adam J.;

;

; Schweiger, Michael;

; Arendt, Christina L.; Marcial, Jose;

Abstract Standard methods to assess the durability of vitrified radioactive waste were first developed in the 1980’s and, over the last 40 years, have evolved to yield a range of responses depending on experimental conditions and glass composition. Mechanistic understanding of glass dissolution has progressed in parallel, enhancing our interpretation of the data acquired. With the implementation of subsurface disposal for vitrified radioactive waste drawing closer, it is timely to review the available standard methodologies and reflect upon their relative advantages, limitations, and how the data obtained can be interpreted to support the post-closure safety case for radioactive waste disposal.

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Sponsoring Organization:: USDOE

OSTI ID:: 1902514

Journal Information:: npj Materials Degradation, Journal Name: npj Materials Degradation Journal Issue: 1 Vol. 5; ISSN 2397-2106

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United Kingdom

Language:: English

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⁹⁹ Tc- and ²³⁹ Pu-Doped Glass Leaching Experiments: Residual Alteration Rate and Radionuclide Behavior Rolland, Séverine; Tribet, Magaly; Jégou, Christophe International Journal of Applied Glass Science, Vol. 4, Issue 4 https://doi.org/10.1111/ijag.12051	journal	October 2013
A Preliminary Investigation of the ISG Glass Vapor Hydration Abdelouas, Abdesselam; El Mendili, Yassine; Aït Chaou, Abdelouahed International Journal of Applied Glass Science, Vol. 4, Issue 4 https://doi.org/10.1111/ijag.12055	journal	October 2013
Effect of chloride ions in Tris buffer solution on bioactive glass apatite mineralization Kirste, Gloria; Brandt-Slowik, Juliane; Bocker, Christian International Journal of Applied Glass Science, Vol. 8, Issue 4 https://doi.org/10.1111/ijag.12288	journal	September 2017
Pre-Viking Swedish hillfort glass: A prospective long-term alteration analogue for vitrified nuclear waste Weaver, Jamie L.; Pearce, Carolyn I.; Sjöblom, Rolf International Journal of Applied Glass Science, Vol. 9, Issue 4 https://doi.org/10.1111/ijag.12351	journal	April 2018
Iron polyphosphate glasses for waste immobilization Brow, Richard K.; Kim, Cheol W.; Reis, Signo T. International Journal of Applied Glass Science, Vol. 11, Issue 1 https://doi.org/10.1111/ijag.13565	journal	August 2019
Effects of Al:Si and (Al+Na):Si ratios on the static corrosion of sodium‐boroaluminosilicate glasses Reiser, Joelle T.; Parruzot, Benjamin; Gin, Stéphane International Journal of Applied Glass Science, Vol. 13, Issue 1 https://doi.org/10.1111/ijag.16109	journal	June 2021
Reactions at Surfaces: A New Approach Integrating Interferometry and Kinetic Simulations: Integrating Interferometry and Kinetic Simulations Luttge, Andreas; Arvidson, Rolf S. Journal of the American Ceramic Society, Vol. 93, Issue 11 https://doi.org/10.1111/j.1551-2916.2010.04141.x	journal	November 2010
Control of Nepheline Crystallization in Nuclear Waste Glass Fox, Kevin M.; Edwards, Thomas B.; Peeler, David K. International Journal of Applied Ceramic Technology, Vol. 5, Issue 6 https://doi.org/10.1111/j.1744-7402.2008.02250.x	journal	November 2008
Durable Glass for Thousands of Years Jantzen, Carol M.; Brown, Kevin G.; Pickett, John B. International Journal of Applied Glass Science, Vol. 1, Issue 1 https://doi.org/10.1111/j.2041-1294.2010.00007.x	journal	March 2010
Nepheline Crystallization in Nuclear Waste Glasses: Progress Toward Acceptance of High-Alumina Formulations McCloy, John S.; Schweiger, Michael J.; Rodriguez, Carmen P. International Journal of Applied Glass Science, Vol. 2, Issue 3 https://doi.org/10.1111/j.2041-1294.2011.00055.x	journal	August 2011
Effects of surface initial condition on aqueous corrosion of glass-A study with a model nuclear waste glass Liu, Hongshen; Ngo, Dien; Ren, Mengguo Journal of the American Ceramic Society, Vol. 102, Issue 4 https://doi.org/10.1111/jace.16016	journal	September 2018
The initial dissolution rates of simulated UK Magnox–ThORP blend nuclear waste glass as a function of pH, temperature and waste loading Cassingham, N.; Corkhill, C. L.; Backhouse, D. J. Mineralogical Magazine, Vol. 79, Issue 6 https://doi.org/10.1180/minmag.2015.079.6.28	journal	November 2015
Corrigendum to “The dissolution rates of simulated UK Magnox – ThORP blend nuclear waste glass as a function of pH, temperature and waste loading” [ Miner. Mag . 79 , (2015) 1529–1542] Corkhill, Claire. L.; Fisher, Adam J.; Strachan, Denis M. Mineralogical Magazine, Vol. 82, Issue 4 https://doi.org/10.1180/minmag.2017.081.077	journal	February 2018
The Accelerated Weathering of a Radioactive Low-Activity Waste Glass under Hydraulically Unsaturated Conditions: Experimental Results from a Pressurized Unsaturated Flow Test Pierce, E. M.; McGrail, B. P.; Valenta, M. M. Nuclear Technology, Vol. 155, Issue 2 https://doi.org/10.13182/NT06-A3753	journal	August 2006
Waste Package Component Interactions with Savannah River Defense Waste Glass in a Low-Magnesium Salt Brine Mcgrail, B. P. Nuclear Technology, Vol. 75, Issue 2 https://doi.org/10.13182/NT86-A33859	journal	November 1986
Chemical alteration of ²³⁸ Pu-loaded borosilicate glass under saturated leaching conditions Zubekhina, Bella Yu.; Shiryaev, Andrei A.; Burakov, Boris E. Radiochimica Acta, Vol. 108, Issue 1 https://doi.org/10.1515/ract-2018-3097	journal	May 2019
The Long-Term Corrosion and Modelling of Two Simulated Belgian Reference High-Level Waste Glasses Van Iseghem, P.; Grambow, B. MRS Proceedings, Vol. 112 https://doi.org/10.1557/PROC-112-631	journal	January 1987
R7T7 Glass Initial Dissolution Rate Measurements Using a High-Temperature Soxhlet Device Delage, Fabienne; Dussossoy, J. L. MRS Proceedings, Vol. 212 https://doi.org/10.1557/PROC-212-41	journal	January 1990
Effect of Surface Finish on Nuclear Glass Dissolution Rate Dussossoy, J. L.; Dubois, C.; Vernaz, E. MRS Proceedings, Vol. 257 https://doi.org/10.1557/PROC-257-109	journal	January 1991
Accelerated Glass Reaction Under PCT Conditions Ebert, W. L.; Bates, J. K.; Buck, E. C. MRS Proceedings, Vol. 294 https://doi.org/10.1557/PROC-294-569	journal	January 1992
Effects of Container Material on PCT Leach Test Results for High-Level Nuclear Waste Glasses Xing, Shi-Ben; Pegg, Ian L. MRS Proceedings, Vol. 333 https://doi.org/10.1557/PROC-333-557	journal	January 1993
The Role of Boron in Monitoring the Leaching of Borosilicate Glass Waste Forms Scheetz, Barry E.; Freeborn, W. Phelps; Smith, Deane K. MRS Proceedings, Vol. 44 https://doi.org/10.1557/PROC-44-129	journal	January 1984
A General Rate Equation for Nuclear Waste Glass Corrosion Grambow, B. MRS Proceedings, Vol. 44 https://doi.org/10.1557/PROC-44-15	journal	January 1984
CORALUS: An Integrated In Situ Corrosion Test on α-Active Glass Iseghem, Pierre Van; Valcke, Elie; Godon, Nicole MRS Proceedings, Vol. 506 https://doi.org/10.1557/PROC-506-961	journal	January 1997
Modelling of Biochemical Processes in Rocks: Oxygen Depletion by Pyrite Oxidation – Model Development and Exploratory Simulations Sidborn, Magnus; Neretnieks, Ivars MRS Proceedings, Vol. 757 https://doi.org/10.1557/PROC-757-II11.5	journal	January 2002
Determination of the Forward Dissolution Rate for International Simple Glass in Alkaline Solutions Elia, Alice; Ferrand, Karine; Lemmens, Karel MRS Advances, Vol. 2, Issue 12 https://doi.org/10.1557/adv.2016.672	journal	January 2017
Uranium Dissolution and Geochemical Modeling in Anoxic and Oxic Solutions Jantzen, Carol M.; Trivelpiece, Cory L. MRS Advances, Vol. 2, Issue 13 https://doi.org/10.1557/adv.2017.58	journal	January 2017
Interactions between Simulant Vitrified Nuclear Wastes and high pH solutions: A Natural Analogue Approach Mann, Colleen; Thorpe, Clare; Milodowski, Antoni E. MRS Advances, Vol. 2, Issue 12 https://doi.org/10.1557/adv.2017.59	journal	January 2017
Iodosodalite Waste Forms from Low-Temperature Aqueous Process Nam, Junghune; Chong, Saehwa; Riley, Brian J. MRS Advances, Vol. 3, Issue 20 https://doi.org/10.1557/adv.2018.225	journal	February 2018
The Formation of Pitted Features on the International Simple Glass during Dynamic Experiments at Alkaline pH Fisher, Adam J.; Hyatt, Neil C.; Hand, Russell J. MRS Advances, Vol. 4, Issue 17-18 https://doi.org/10.1557/adv.2019.9	journal	January 2019
On Alteration Rate Renewal Stage of Nuclear Waste Glass Corrosion Ojovan, Michael I. MRS Advances, Vol. 5, Issue 3-4 https://doi.org/10.1557/adv.2020.36	journal	January 2020
The dissolution of simulant UK Ca/Zn-modified nuclear waste glass: Insight into Stage III behavior Fisher, Adam J.; Harrison, Mike T.; Hyatt, Neil C. MRS Advances, Vol. 5, Issue 3-4 https://doi.org/10.1557/adv.2020.50	journal	January 2020
The dissolution of simulant UK Ca/Zn-modified nuclear waste glass: the effect of increased waste loading Fisher, Adam J.; Harrison, Mike T.; Hyatt, Neil C. MRS Advances, Vol. 6, Issue 4-5 https://doi.org/10.1557/s43580-021-00025-0	journal	February 2021
Nepheline structural and chemical dependence on melt composition Marcial, José; Crum, Jarrod; Neill, Owen American Mineralogist, Vol. 101, Issue 2 https://doi.org/10.2138/am-2016-5370	journal	February 2016
Dissolution kinetics of pyrochlore ceramics for the disposition of plutonium Icenhower, Jonathan P.; Strachan, Denis M.; McGrail, B. Pete American Mineralogist, Vol. 91, Issue 1 https://doi.org/10.2138/am.2006.1709	journal	January 2006
The durability of rocks--Developing a test of rock resistance to chemical weathering Franke, W. A. American Journal of Science, Vol. 309, Issue 8 https://doi.org/10.2475/08.2009.04	journal	October 2009
Thermodynamic and kinetic constraints on reaction rates among minerals and aqueous solutions; I, Theoretical considerations Aagaard, P.; Helgeson, H. C. American Journal of Science, Vol. 282, Issue 3 https://doi.org/10.2475/ajs.282.3.237	journal	March 1982
The Role of Temperature in the Safety Case for High-Level Radioactive Waste Disposal: A Comparison of Design Concepts Heierli, Joachim; Genoni, Oliver Geosciences, Vol. 7, Issue 2 https://doi.org/10.3390/geosciences7020042	journal	June 2017
Corrosion Behavior and Microstructure Influence of Glass-Ceramic Nuclear Waste Forms Matthew Asmussen, R.; Neeway, James J.; Kaspar, Tiffany C. CORROSION, Vol. 73, Issue 11 https://doi.org/10.5006/2449	journal	June 2017

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