Improved $$^{95}\mathrm{Mo}$$ neutron resonance parameters and astrophysical reaction rates

Journal Article · 12 May 2022 · Physical Review. C

DOI: https://doi.org/10.1103/physrevc.105.054306 · OSTI ID:1897428

Koehler, Paul E.  ^[1]

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1. Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

We report improved ⁹⁵Mo neutron resonance parameters and reaction rates are important for nuclear astrophysics, testing nuclear models, and nuclear criticality safety. However, despite many previous neutron-capture and total cross-section measurements on this nuclide, there still is much room for improvement as well as several discrepancies. For example, there are very few firm resonance spin and parity assignments; average resonance parameters are available only for each parity, the currently recommended astrophysical reaction rate results in disagreements between stellar models and meteoric isotopic anomalies, and there are substantial disagreements in the neutron-capture cross section at low energies important for nuclear criticality safety. To obtain an improved set of neutron resonance parameters and astrophysical reaction rates for ⁹⁵Mo. High-resolution neutron-capture and transmission data were measured at the Oak Ridge Electron Linear Accelerator (ORELA) using highly isotopically enriched ⁹⁵Mo samples. The neutron-capture apparatus, data reduction, and analysis were improved so that information contained in the γ-ray cascade following neutron capture were used to assign resonance J^π values. Following this, simultaneous analysis of the new neutron-capture and transmission data was used to obtain resonance energies, gamma widths, and neutron widths and their uncertainties to a maximum energy of 10 keV. Accurate neutron-capture cross sections also were obtained for the unresolved resonance region to a maximum energy of 500 keV and, together with the new resonance parameters, used to calculate the astrophysical reaction rates in the temperature range from 5 to 30 keV. A vastly improved set of 95Mo neutron resonance parameters and an astrophysical reaction rate accurate to about 3% were obtained. Firm J_π assignments were determined for 261 of the 314 observed resonances. This is a very large improvement over the previously published 32 firm J_π assignments for 108 resonances. Also, the number of resonances having both firm J_π assignments and Γ_γ values was increased by almost a factor of 24—from 11 to 261. Neutron- and total-radiation-width distributions and average resonance spacings, average total radiation widths, and neutron strength functions were obtained for the six different s- and p-wave possibilities. Parameters for the lowest s-wave resonance, which is most important for criticality benchmarks, were obtained with high accuracy. Simple modification of the neutron-capture apparatus and expansion and improvement of data analysis techniques led to a large increase in firm J_π assignments for ⁹⁵Mo neutron resonances. The resulting astrophysical reaction rate is 20%–30% larger than the currently recommended rate at s-process temperatures, which should lead to better agreement between stellar models and meteoric isotopic anomalies. The neutron-capture cross section at low energies is substantially larger than recommended in the latest evaluation, which is problematical for criticality benchmarks. The average resonance spacing as a function of spin and parity is significantly different from current models. The total-radiation-width distributions are significantly broader than predicted by theory and show significant departures from the expected Gaussian shapes.

• Research Organization: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
• Sponsoring Organization: USDOE National Nuclear Security Administration (NNSA), Nuclear Criticality Safety Program (NCSP)
• Grant/Contract Number: 89233218CNA000001
• OSTI ID: 1897428
• Report Number(s): LA-UR-21-28567; TRN: US2310787
• Journal Information: Physical Review. C, Vol. 105, Issue 5; ISSN 2469-9985
• Publisher: American Physical Society (APS)Copyright Statement
• Country of Publication: United States
• Language: English