Influence of biogenic emissions from boreal forests on aerosol–cloud interactions

Petäjä, T.; Tabakova, K.; Manninen, A.; Ezhova, E.; O’Connor, E.; Moisseev, D.; Sinclair, V. A.; Backman, J.; Levula, J.; Luoma, K.; Virkkula, A.; Paramonov, M.; Räty, M.; Äijälä, M.; Heikkinen, L.; Ehn, M.; Sipilä, M.; Yli-Juuti, T.; Virtanen, A.; Ritsche, M.; Hickmon, N.; Pulik, G.; Rosenfeld, D.; Worsnop, D. R.; Bäck, J.; Kulmala, M.; Kerminen, V. -M.

doi:10.1038/s41561-021-00876-0

Title: Influence of biogenic emissions from boreal forests on aerosol–cloud interactions

Journal Article · 22 December 2021 · Nature Geoscience

DOI: https://doi.org/10.1038/s41561-021-00876-0 · OSTI ID:1881026

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^[5]; Paramonov, M. ^[3];

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Univ. of Helsinki (Finland); Nanjing Univ. (China)
Univ. of Helsinki (Finland)
Univ. of Helsinki (Finland); Finnish Meteorological Inst., Helsinki (Finland)
Finnish Meteorological Inst., Helsinki (Finland); Univ. of Reading (United Kingdom)
Univ. of Helsinki (Finland); Nanjing Univ. (China); Finnish Meteorological Inst., Helsinki (Finland)
Univ. of Eastern Finland, Kuopio (Finland)
Argonne National Lab. (ANL), Lemont, IL (United States)
Hebrew Univ. of Jerusalem (Israel)
Univ. of Helsinki (Finland); Aerodyne Research Inc., Billerica, MA (United States)
Univ. of Helsinki (Finland); Nanjing Univ. (China); Beijing Univ. of Chemical Technology (BUCT) (China); Moscow State Univ. (Russia)

Boreal forest acts as a carbon sink and contributes to the formation of secondary organic aerosols via emission of aerosol precursor compounds. However, these influences on the climate system are poorly quantified. Here we show direct observational evidence that aerosol emissions from the boreal forest biosphere influence warm cloud microphysics and cloud-aerosol interactions in a scale-dependent and highly dynamic manner. Analyses of in situ and ground-based remote-sensing observations from the SMEAR II station in Finland, conducted over eight months in 2014, reveal substantial increases in aerosol load over the forest one to three days after aerosol-poor marine air enters the forest environment. We find that these changes are consistent with secondary organic aerosol formation and, together with water-vapour emissions from evapotranspiration, are associated with changes in the radiative properties of warm, low-level clouds. Here, the feedbacks between boreal forest emissions and aerosol-cloud interactions and the highly dynamic nature of these interactions in air transported over the forest over timescales of several days suggest boreal forests have the potential to mitigate climate change on a continental scale. Our findings suggest that even small changes in aerosol precursor emissions, whether due to changing climatic or anthropogenic factors, may substantially modify the radiative properties of clouds in moderately polluted environments. Emissions from the boreal forest biosphere can substantially increase aerosol load above the forest and influence the radiative properties of clouds, according to analysis of observations from a monitoring station in Finland.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: Academy of Finland; European Research Council (ERC); European Union, Horizon 2020 Research and Innovation Programme; USDOE Office of Science (SC)

Grant/Contract Number:: AC02-06CH11357; SC0010711

OSTI ID:: 1881026

Journal Information:: Nature Geoscience, Journal Name: Nature Geoscience Journal Issue: 1 Vol. 15; ISSN 1752-0894

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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