Photoelectron spectroscopy in molecular physical chemistry

Fischer, Ingo; Pratt, Stephen T.

doi:10.1039/d1cp04984d

Title: Photoelectron spectroscopy in molecular physical chemistry

Journal Article · 05 January 2022 · Physical Chemistry Chemical Physics. PCCP

DOI: https://doi.org/10.1039/d1cp04984d · OSTI ID:1878601

^[1];

^[2]

Univ. of Würzburg, Am Hubland, D-97074 Würzburg, Germany
Argonne National Lab. (ANL), Lemont, IL (United States)

Photoelectron spectroscopy has long been a powerful method in the toolbox of experimental physical chemistry and molecular physics. Recent improvements in coincidence methods, charged-particle imaging, and electron energy resolution have greatly expanded the variety of environments in which photoelectron spectroscopy can be applied, as well as the range of questions that can now be addressed. In this Perspectives Article, we focus on selected recent studies that highlight these advances and research areas. Furthermore, the topics include reactive intermediates and new thermochemical data, high-resolution comparisons of experiment and theory using methods based on pulsed-field ionisation (PFI), and the application of photoelectron spectroscopy as an analytical tool to monitor chemical reactions in complex environments, like model flames, catalytic or high-temperature reactors.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences & Biosciences Division; Deutsche Forschungsgemeinschaft (DFG)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1878601

Journal Information:: Physical Chemistry Chemical Physics. PCCP, Journal Name: Physical Chemistry Chemical Physics. PCCP Journal Issue: 4 Vol. 24; ISSN 1463-9076

Publisher:: Royal Society of ChemistryCopyright Statement

Country of Publication:: United States

Language:: English

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