Hydrogen storage in complex hydrides: past activities and new trends

Dematteis, Erika Michela; Amdisen, Mads B.; Autrey, Tom; Barale, Jussara; Bowden, Mark E.; Buckley, Craig E.; Cho, Young Whan; Deledda, Stefano; Dornheim, Martin; de Jongh, Petra; Grinderslev, Jakob B.; Gizer, Gökhan; Gulino, Valerio; Hauback, Bjørn C.; Heere, Michael; Heo, Tae Wook; Humphries, Terry D.; Jensen, Torben R.; Kang, Shin Young; Lee, Young-Su; Li, Hai-Wen; Li, Sichi; Møller, Kasper T.; Ngene, Peter; Orimo, Shin-ichi; Paskevicius, Mark; Polanski, Marek; Takagi, Shigeyuki; Wan, Liwen; Wood, Brandon C.; Hirscher, Michael; Baricco, Marcello

doi:10.1088/2516-1083/ac7499

Title: Hydrogen storage in complex hydrides: past activities and new trends

Journal Article · 22 June 2022 · Progress in Energy

DOI: https://doi.org/10.1088/2516-1083/ac7499 · OSTI ID:1873572

;

; Deledda, Stefano;

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Abstract Intense literature and research efforts have focussed on the exploration of complex hydrides for energy storage applications over the past decades. A focus was dedicated to the determination of their thermodynamic and hydrogen storage properties, due to their high gravimetric and volumetric hydrogen storage capacities, but their application has been limited because of harsh working conditions for reversible hydrogen release and uptake. The present review aims at appraising the recent advances on different complex hydride systems, coming from the proficient collaborative activities in the past years from the research groups led by the experts of the Task 40 ‘Energy Storage and Conversion Based on Hydrogen’ of the Hydrogen Technology Collaboration Programme of the International Energy Agency. An overview of materials design, synthesis, tailoring and modelling approaches, hydrogen release and uptake mechanisms and thermodynamic aspects are reviewed to define new trends and suggest new possible applications for these highly tuneable materials.

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Sponsoring Organization:: USDOE

Grant/Contract Number:: AC52-07NA27344

OSTI ID:: 1873572

Journal Information:: Progress in Energy, Journal Name: Progress in Energy Journal Issue: 3 Vol. 4; ISSN 2516-1083

Publisher:: IOP PublishingCopyright Statement

Country of Publication:: United Kingdom

Language:: English

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Understanding and Mitigating the Effects of Stable Dodecahydro- closo -dodecaborate Intermediates on Hydrogen-Storage Reactions White, James L.; Newhouse, Rebecca J.; Zhang, Jin Z. The Journal of Physical Chemistry C, Vol. 120, Issue 45 https://doi.org/10.1021/acs.jpcc.6b09789	journal	November 2016
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Structural Insights into the Lithium Amide-Imide Solid Solution Makepeace, Joshua W.; David, William I. F. The Journal of Physical Chemistry C, Vol. 121, Issue 22 https://doi.org/10.1021/acs.jpcc.7b02441	journal	May 2017
Synthesis, Structure, and Li-Ion Conductivity of LiLa(BH ₄ ) ₃ X, X = Cl, Br, I Payandeh GharibDoust, SeyedHosein; Brighi, Matteo; Sadikin, Yolanda The Journal of Physical Chemistry C, Vol. 121, Issue 35 https://doi.org/10.1021/acs.jpcc.7b04905	journal	August 2017
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Effect of Pore Confinement of NaNH ₂ and KNH ₂ on Hydrogen Generation from Ammonia Chang, Fei; Wu, Han; Pluijm, Robby van der The Journal of Physical Chemistry C, Vol. 123, Issue 35 https://doi.org/10.1021/acs.jpcc.9b03878	journal	August 2019
Crystal Structures and Energy Storage Properties of Ammine Sodium Decahydro- closo -decaboranes (Na ₂ B ₁₀ H ₁₀ · n NH ₃ , n = 1, 2) Jørgensen, Mathias; Hansen, Bjarne R. S.; Lee, Young-Su The Journal of Physical Chemistry C, Vol. 123, Issue 33 https://doi.org/10.1021/acs.jpcc.9b06084	journal	July 2019
Analysis of Dihydrogen Bonding in Ammonium Borohydride Filippov, Stanislav; Grinderslev, Jakob B.; Andersson, Mikael S. The Journal of Physical Chemistry C, Vol. 123, Issue 47 https://doi.org/10.1021/acs.jpcc.9b08968	journal	November 2019
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Ammine Magnesium Borohydride Nanocomposites for All-Solid-State Magnesium Batteries Yan, Yigang; Grinderslev, Jakob B.; Jo̷rgensen, Mathias ACS Applied Energy Materials, Vol. 3, Issue 9 https://doi.org/10.1021/acsaem.0c01599	journal	August 2020
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Bulk-Type All-Solid-State Lithium Batteries Using Complex Hydrides Containing Cluster-Anions Unemoto, Atsushi; Yoshida, Koji; Ikeshoji, Tamio MATERIALS TRANSACTIONS, Vol. 57, Issue 9 https://doi.org/10.2320/matertrans.MAW201601	journal	January 2016
Boron Hydrogen Compounds for Hydrogen Storage and as Solid Ionic Conductors Hagemann, Hans CHIMIA International Journal for Chemistry, Vol. 73, Issue 11 https://doi.org/10.2533/chimia.2019.868	journal	November 2019
Hydrogen Sorption and Reversibility of the LiBH4-KBH4 Eutectic System Confined in a CMK-3 Type Carbon via Melt Infiltration Peru, Filippo; Payandeh, SeyedHosein; Charalambopoulou, Georgia C — Journal of Carbon Research, Vol. 6, Issue 2 https://doi.org/10.3390/c6020019	journal	March 2020
Theoretical and Experimental Study of LiBH4-LiCl Solid Solution Zavorotynska, Olena; Corno, Marta; Pinatel, Eugenio Crystals, Vol. 2, Issue 1 https://doi.org/10.3390/cryst2010144	journal	March 2012
Reactive Hydride Composite of Mg2NiH4 with Borohydrides Eutectic Mixtures Dematteis, Erika; Vaunois, Silvère; Pistidda, Claudio Crystals, Vol. 8, Issue 2 https://doi.org/10.3390/cryst8020090	journal	February 2018
Complex Metal Hydrides for Hydrogen, Thermal and Electrochemical Energy Storage Møller, Kasper; Sheppard, Drew; Ravnsbæk, Dorthe Energies, Vol. 10, Issue 10 https://doi.org/10.3390/en10101645	journal	October 2017
Rare Earth Borohydrides—Crystal Structures and Thermal Properties Frommen, Christoph; Sørby, Magnus; Heere, Michael Energies, Vol. 10, Issue 12 https://doi.org/10.3390/en10122115	journal	December 2017
Recent Progress and New Perspectives on Metal Amide and Imide Systems for Solid-State Hydrogen Storage Garroni, Sebastiano; Santoru, Antonio; Cao, Hujun Energies, Vol. 11, Issue 5 https://doi.org/10.3390/en11051027	journal	April 2018
Enhancement Effect of Bimetallic Amide K2Mn(NH2)4 and In-Situ Formed KH and Mn4N on the Dehydrogenation/Hydrogenation Properties of Li–Mg–N–H System Gizer, Gökhan; Cao, Hujun; Puszkiel, Julián Energies, Vol. 12, Issue 14 https://doi.org/10.3390/en12142779	journal	July 2019
Hydrogen Desorption in Mg(BH4)2-Ca(BH4)2 System Dematteis, Erika M.; Baricco, Marcello Energies, Vol. 12, Issue 17 https://doi.org/10.3390/en12173230	journal	August 2019
Solid-State Hydrogen Storage Systems and the Relevance of a Gender Perspective Dematteis, Erika Michela; Barale, Jussara; Corno, Marta Energies, Vol. 14, Issue 19 https://doi.org/10.3390/en14196158	journal	September 2021
Melting Behavior and Thermolysis of NaBH4−Mg(BH4)2 and NaBH4−Ca(BH4)2 Composites Ley, Morten; Roedern, Elsa; Thygesen, Peter Energies, Vol. 8, Issue 4 https://doi.org/10.3390/en8042701	journal	April 2015
Increasing Hydrogen Density with the Cation-Anion Pair BH4−-NH4+ in Perovskite-Type NH4Ca(BH4)3 Schouwink, Pascal; Morelle, Fabrice; Sadikin, Yolanda Energies, Vol. 8, Issue 8 https://doi.org/10.3390/en8088286	journal	August 2015
Metal Hydrides for High-Temperature Power Generation Rönnebro, Ewa; Whyatt, Greg; Powell, Michael Energies, Vol. 8, Issue 8 https://doi.org/10.3390/en8088406	journal	August 2015
Enhancing the Hydrogen Storage Properties of AxBy Intermetallic Compounds by Partial Substitution: A Short Review Lys, Andrii; Fadonougbo, Julien O.; Faisal, Mohammad Hydrogen, Vol. 1, Issue 1 https://doi.org/10.3390/hydrogen1010004	journal	December 2020
Hydrogen Sorption in Erbium Borohydride Composite Mixtures with LiBH4 and/or LiH Heere, Michael; GharibDoust, Seyed; Brighi, Matteo Inorganics, Vol. 5, Issue 2 https://doi.org/10.3390/inorganics5020031	journal	April 2017
Tetrahydroborates: Development and Potential as Hydrogen Storage Medium Puszkiel, Julián; Garroni, Sebastiano; Milanese, Chiara Inorganics, Vol. 5, Issue 4 https://doi.org/10.3390/inorganics5040074	journal	October 2017
Lewis Base Complexes of Magnesium Borohydride: Enhanced Kinetics and Product Selectivity upon Hydrogen Release Chong, Marina; Autrey, Tom; Jensen, Craig Inorganics, Vol. 5, Issue 4 https://doi.org/10.3390/inorganics5040089	journal	December 2017
A Review of the MSCA ITN ECOSTORE—Novel Complex Metal Hydrides for Efficient and Compact Storage of Renewable Energy as Hydrogen and Electricity Hadjixenophontos, Efi; Dematteis, Erika Michela; Berti, Nicola Inorganics, Vol. 8, Issue 3 https://doi.org/10.3390/inorganics8030017	journal	March 2020
Synthesis, Crystal Structures and Thermal Properties of Ammine Barium Borohydrides Grinderslev, Jakob B.; Amdisen, Mads B.; Jensen, Torben R. Inorganics, Vol. 8, Issue 10 https://doi.org/10.3390/inorganics8100057	journal	October 2020
Effects of Glymes on the Distribution of Mg(B10H10) and Mg(B12H12) from the Thermolysis of Mg(BH4)2 Tran, Ba L.; Allen, Tamara N.; Bowden, Mark E. Inorganics, Vol. 9, Issue 6 https://doi.org/10.3390/inorganics9060041	journal	May 2021
Mechanochemistry of Metal Hydrides: Recent Advances Huot, Jacques; Cuevas, Fermín; Deledda, Stefano Materials, Vol. 12, Issue 17 https://doi.org/10.3390/ma12172778	journal	August 2019
Metal Borohydrides beyond Groups I and II: A Review Suárez-Alcántara, Karina; Tena García, Juan Rogelio Materials, Vol. 14, Issue 10 https://doi.org/10.3390/ma14102561	journal	May 2021
Solid State Hydrogen Storage in Alanates and Alanate-Based Compounds: A Review Milanese, Chiara; Garroni, Sebastiano; Gennari, Fabiana Metals, Vol. 8, Issue 8 https://doi.org/10.3390/met8080567	journal	July 2018
Eutectic Phenomenon of LiNH2-KH Composite in MH-NH3 Hydrogen Storage System Goshome, Kiyotaka; Jain, Ankur; Miyaoka, Hiroki Molecules, Vol. 24, Issue 7 https://doi.org/10.3390/molecules24071348	journal	April 2019
Thermodynamic Database for Hydrogen Storage Materials Baricco, Marcello; Palumbo, Mauro; Pinatel, Eugenio Advances in Science and Technology, Vol. 72 https://doi.org/10.4028/www.scientific.net/AST.72.213	journal	October 2010
New Functionalities of Hydride Complexes with High Hydrogen Coordination Takagi, Shigeyuki; Orimo, Shin-ichi Journal of the Physical Society of Japan, Vol. 89, Issue 5 https://doi.org/10.7566/JPSJ.89.051010	journal	May 2020
Structure and Dynamics of Borohydrides Studied by Neutron Scattering Techniques: A Review Lohstroh, Wiebke; Heere, Michael Journal of the Physical Society of Japan, Vol. 89, Issue 5 https://doi.org/10.7566/JPSJ.89.051011	journal	May 2020

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