Multielectron Organic Redoxmers for Energy-Dense Redox Flow Batteries

Fang, Xiaoting; Li, Zhiguang; Zhao, Yuyue; Yue, Diqing; Zhang, Lu; Wei, Xiaoliang

doi:10.1021/acsmaterialslett.1c00668

Title: Multielectron Organic Redoxmers for Energy-Dense Redox Flow Batteries

Journal Article · 06 January 2022 · ACS Materials Letters

DOI: https://doi.org/10.1021/acsmaterialslett.1c00668 · OSTI ID:1870819

Fang, Xiaoting ^[1]; Li, Zhiguang ^[1]; Zhao, Yuyue ^[2]; Yue, Diqing ^[3];

^[4];

^[2]

Indiana Univ.-Purdue Univ. Indianapolis (IUPUI), Indianapolis, IN (United States); Purdue Univ., West Lafayette, IN (United States); Argonne National Lab. (ANL), Lemont, IL (United States)
Indiana Univ.-Purdue Univ. Indianapolis (IUPUI), Indianapolis, IN (United States)
Indiana Univ.-Purdue Univ. Indianapolis (IUPUI), Indianapolis, IN (United States); Purdue Univ., West Lafayette, IN (United States)
Argonne National Lab. (ANL), Lemont, IL (United States)

Redox flow battery is a highly promising stationary energy storage method but the limited energy density and high chemical cost are among the main barriers for commercialization. Multi-electron organic redoxmers represent a family of structurally tailorable candidates that can achieve multiplied energy density with decreased materials consumption, potentially resulting in a viable solution to address these challenges. In this work, the recent development of organic molecules with reversible multi-redox activities in both aqueous and nonaqueous electrolytes is reviewed. The major focus is on the fundamental correlation between the chemical structures and the functional properties of reported multi-electron organic molecules. Valuable insights are offered on rational structural design strategies for improving the relevant physico- and electro-chemical properties. Finally, the current challenges are discussed to suggest future research needs along the avenue of using the multi-electron approach to achieve energy-dense, stable, cost-effective redox flow batteries.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: National Science Foundation (NSF); USDOE Laboratory Directed Research and Development (LDRD) Program; USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1870819

Journal Information:: ACS Materials Letters, Journal Name: ACS Materials Letters Journal Issue: 2 Vol. 4; ISSN 2639-4979

Publisher:: ACS PublicationsCopyright Statement

Country of Publication:: United States

Language:: English

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