Unveiling the orbital texture of 1T-TiTe2 using intrinsic linear dichroism in multidimensional photoemission spectroscopy

Beaulieu, Samuel; Schüler, Michael; Schusser, Jakub; Dong, Shuo; Pincelli, Tommaso; Maklar, Julian; Neef, Alexander; Reinert, Friedrich; Wolf, Martin; Rettig, Laurenz; Minár, Ján; Ernstorfer, Ralph

doi:10.1038/s41535-021-00398-3

Title: Unveiling the orbital texture of 1T-TiTe₂ using intrinsic linear dichroism in multidimensional photoemission spectroscopy

Abstract

The momentum-dependent orbital character in crystalline solids, referred to as orbital texture, is of capital importance in the emergence of symmetry-broken collective phases, such as charge density waves as well as superconducting and topological states of matter. By performing extreme ultraviolet multidimensional angle-resolved photoemission spectroscopy for two different crystal orientations linked to each other by mirror symmetry, we isolate and identify the role of orbital texture in photoemission from the transition metal dichalcogenide 1T-TiTe₂. By comparing our experimental results with theoretical calculations based on both a quantitative one-step model of photoemission and an intuitive tight-binding model, we unambiguously demonstrate the link between the momentum-dependent orbital orientation and the emergence of strong intrinsic linear dichroism in the photoelectron angular distributions. Our results represent an important step towards going beyond band structure (eigenvalues) mapping and learning about electronic wavefunction and orbital texture of solids by exploiting matrix element effects in photoemission spectroscopy.

Authors:

^[1]; Schüler, Michael ^[2];

^[3]; Dong, Shuo ^[4];

^[4]; Maklar, Julian ^[4]; Neef, Alexander ^[4]; Reinert, Friedrich ^[5]; Wolf, Martin ^[4];

^[4];

^[6];

^[7]

Univ. de Bordeaux. CMRS, CEA, CELIA, Talence (France); Fritz Haber Institute of the Max Planck Society, Berlin (Germany)
SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Institute for Materials and Energy Science (SIMES)
Univ. of Wurzburg (Germany); University of West Bohemia, Pilsen (Czech Republic)
Fritz Haber Institute of the Max Planck Society, Berlin (Germany)
Univ. of Wurzburg (Germany)
University of West Bohemia, Pilsen (Czech Republic)
Fritz Haber Institute of the Max Planck Society, Berlin (Germany); Technical Univ. of Berlin (Germany). Inst. of Optics and Atomic Physics (IOAP)

Publication Date:: Mon Nov 15 00:00:00 EST 2021

Research Org.:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES); Max Planck Society, European Research Council (ERC); German Research Foundation (DFG)

OSTI Identifier:: 1869818

Grant/Contract Number:: AC02-76SF00515; ERC-2015-CoG-682843; H2020-FETOPEN-2018-2019-2020-01; 899794; RE-3977/1

Resource Type:: Accepted Manuscript

Journal Name:: npj Quantum Materials

Additional Journal Information:: Journal Volume: 6; Journal Issue: 1; Journal ID: ISSN 2397-4648

Publisher:: Nature Publishing Group

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; 36 MATERIALS SCIENCE

Citation Formats


                    Beaulieu, Samuel, Schüler, Michael, Schusser, Jakub, Dong, Shuo, Pincelli, Tommaso, Maklar, Julian, Neef, Alexander, Reinert, Friedrich, Wolf, Martin, Rettig, Laurenz, Minár, Ján, and Ernstorfer, Ralph. Unveiling the orbital texture of 1T-TiTe2 using intrinsic linear dichroism in multidimensional photoemission spectroscopy.  United States: N. p., 2021. 
Web.  doi:10.1038/s41535-021-00398-3.

Copy to clipboard


                    Beaulieu, Samuel, Schüler, Michael, Schusser, Jakub, Dong, Shuo, Pincelli, Tommaso, Maklar, Julian, Neef, Alexander, Reinert, Friedrich, Wolf, Martin, Rettig, Laurenz, Minár, Ján, & Ernstorfer, Ralph. Unveiling the orbital texture of 1T-TiTe2 using intrinsic linear dichroism in multidimensional photoemission spectroscopy.  United States.  https://doi.org/10.1038/s41535-021-00398-3

Copy to clipboard


                    Beaulieu, Samuel, Schüler, Michael, Schusser, Jakub, Dong, Shuo, Pincelli, Tommaso, Maklar, Julian, Neef, Alexander, Reinert, Friedrich, Wolf, Martin, Rettig, Laurenz, Minár, Ján, and Ernstorfer, Ralph. Mon .  
"Unveiling the orbital texture of 1T-TiTe2 using intrinsic linear dichroism in multidimensional photoemission spectroscopy".  United States.  https://doi.org/10.1038/s41535-021-00398-3.  https://www.osti.gov/servlets/purl/1869818.

Copy to clipboard


                    
@article{osti_1869818,

  title        = {Unveiling the orbital texture of 1T-TiTe2 using intrinsic linear dichroism in multidimensional photoemission spectroscopy},

  author       = {Beaulieu, Samuel and Schüler, Michael and Schusser, Jakub and Dong, Shuo and Pincelli, Tommaso and Maklar, Julian and Neef, Alexander and Reinert, Friedrich and Wolf, Martin and Rettig, Laurenz and Minár, Ján and Ernstorfer, Ralph},

  abstractNote = {The momentum-dependent orbital character in crystalline solids, referred to as orbital texture, is of capital importance in the emergence of symmetry-broken collective phases, such as charge density waves as well as superconducting and topological states of matter. By performing extreme ultraviolet multidimensional angle-resolved photoemission spectroscopy for two different crystal orientations linked to each other by mirror symmetry, we isolate and identify the role of orbital texture in photoemission from the transition metal dichalcogenide 1T-TiTe2. By comparing our experimental results with theoretical calculations based on both a quantitative one-step model of photoemission and an intuitive tight-binding model, we unambiguously demonstrate the link between the momentum-dependent orbital orientation and the emergence of strong intrinsic linear dichroism in the photoelectron angular distributions. Our results represent an important step towards going beyond band structure (eigenvalues) mapping and learning about electronic wavefunction and orbital texture of solids by exploiting matrix element effects in photoemission spectroscopy.},

  doi          = {10.1038/s41535-021-00398-3},

  journal      = {npj Quantum Materials},

  number       = 1,

  volume       = 6,

  place        = {United States},

  year         = {Mon Nov 15 00:00:00 EST 2021},

  month        = {Mon Nov 15 00:00:00 EST 2021}

}

Copy to clipboard

Journal Article:

Free Publicly Available Full Text

Accepted Manuscript (DOE)

Publisher's Version of Record

https://doi.org/10.1038/s41535-021-00398-3

Other availability

Search WorldCat to find libraries that may hold this journal

Save / Share:

Export Metadata

Save to My Library

Works referenced in this record:

Probing band parity inversion in the topological insulator GeBi2Te4 by linear dichroism in ARPES
journal, May 2018

Sterzi, A.; Manzoni, G.; Crepaldi, A.
Journal of Electron Spectroscopy and Related Phenomena, Vol. 225
DOI: 10.1016/j.elspec.2018.03.004

Symmetry-guided nonrigid registration: The case for distortion correction in multidimensional photoemission spectroscopy
journal, July 2019

Xian, R. Patrick; Rettig, Laurenz; Ernstorfer, Ralph
Ultramicroscopy, Vol. 202
DOI: 10.1016/j.ultramic.2019.04.004

Photoemission spectroscopy in metals:
journal, October 1999

Hüfner, S.; Claessen, R.; Reinert, F.
Journal of Electron Spectroscopy and Related Phenomena, Vol. 100, Issue 1-3
DOI: 10.1016/S0368-2048(99)00047-X

An experimentalist's guide to the matrix element in angle resolved photoemission
journal, January 2017

Moser, Simon
Journal of Electron Spectroscopy and Related Phenomena, Vol. 214
DOI: 10.1016/j.elspec.2016.11.007

Profiling spin and orbital texture of a topological insulator in full momentum space
journal, April 2021

Bentmann, H.; Maaß, H.; Braun, J.
Physical Review B, Vol. 103, Issue 16
DOI: 10.1103/PhysRevB.103.L161107

Non-local dxy nematicity and the missing electron pocket in FeSe
journal, May 2021

Rhodes, Luke C.; Böker, Jakob; Müller, Marvin A.
npj Quantum Materials, Vol. 6, Issue 1
DOI: 10.1038/s41535-021-00341-6

Calculating condensed matter properties using the KKR-Green's function method—recent developments and applications
journal, August 2011

Ebert, H.; Ködderitzsch, D.; Minár, J.
Reports on Progress in Physics, Vol. 74, Issue 9
DOI: 10.1088/0034-4885/74/9/096501

Complete band-structure determination of the quasi-two-dimensional Fermi-liquid reference compound TiTe 2
journal, July 1996

Claessen, R.; Anderson, R. O.; Gweon, G. -H.
Physical Review B, Vol. 54, Issue 4
DOI: 10.1103/PhysRevB.54.2453

500 kHz OPCPA delivering tunable sub-20 fs pulses with 15 W average power based on an all-ytterbium laser
journal, January 2015

Puppin, Michele; Deng, Yunpei; Prochnow, Oliver
Optics Express, Vol. 23, Issue 2
DOI: 10.1364/OE.23.001491

Experimental Observation of Hidden Berry Curvature in Inversion-Symmetric Bulk $2 H − {WSe}_{2}$
journal, October 2018

Cho, Soohyun; Park, Jin-Hong; Hong, Jisook
Physical Review Letters, Vol. 121, Issue 18
DOI: 10.1103/PhysRevLett.121.186401

Experimental Evidence of Chiral Symmetry Breaking in Kekulé-Ordered Graphene
journal, May 2021

Bao, Changhua; Zhang, Hongyun; Zhang, Teng
Physical Review Letters, Vol. 126, Issue 20
DOI: 10.1103/PhysRevLett.126.206804

Electronic properties and superlattice formation in the semimetal ${TiSe}_{2}$
journal, November 1976

Di Salvo, F. J.; Moncton, D. E.; Waszczak, J. V.
Physical Review B, Vol. 14, Issue 10
DOI: 10.1103/PhysRevB.14.4321

ARPES study of orbital character, symmetry breaking, and pseudogaps in doped and pure ${Sr}_{2} {IrO}_{4}$
journal, November 2019

Louat, Alex; Lenz, Benjamin; Biermann, Silke
Physical Review B, Vol. 100, Issue 20
DOI: 10.1103/PhysRevB.100.205135

Ultrafast dynamical Lifshitz transition
journal, April 2021

Beaulieu, Samuel; Dong, Shuo; Tancogne-Dejean, Nicolas
Science Advances, Vol. 7, Issue 17
DOI: 10.1126/sciadv.abd9275

Multidimensional XUV Photoemission Spectroscopy of 1T-TiTe2 for different crystal orientations
dataset, January 2021

Beaulieu, Samuel; Schüler, Michael; Schusser, Jakub
Zenodo
DOI: 10.5281/zenodo.5541490

Determination of the Hole Lifetime from Photoemission: Ti $3 d$ States in ${TiTe}_{2}$
journal, May 2007

Krasovskii, E. E.; Rossnagel, K.; Fedorov, A.
Physical Review Letters, Vol. 98, Issue 21
DOI: 10.1103/PhysRevLett.98.217604

Charge-density wave transition of $1 T {- V S e}_{2}$ studied by angle-resolved photoemission spectroscopy
journal, October 2003

Terashima, K.; Sato, T.; Komatsu, H.
Physical Review B, Vol. 68, Issue 15
DOI: 10.1103/PhysRevB.68.155108

Multi-MHz time-of-flight electronic bandstructure imaging of graphene on Ir(111)
journal, June 2016

Tusche, C.; Goslawski, P.; Kutnyakhov, D.
Applied Physics Letters, Vol. 108, Issue 26
DOI: 10.1063/1.4955015

Probing the Electronic Structure of Complex Systems by ARPES
journal, January 2004

Damascelli, Andrea
Physica Scripta, Vol. T109
DOI: 10.1238/Physica.Topical.109a00061

Nature of Symmetry Breaking at the Excitonic Insulator Transition: ${Ta}_{2} {NiSe}_{5}$
journal, May 2020

Mazza, Giacomo; Rösner, Malte; Windgätter, Lukas
Physical Review Letters, Vol. 124, Issue 19
DOI: 10.1103/PhysRevLett.124.197601

Momentum-space signatures of Berry flux monopoles in the Weyl semimetal TaAs
journal, June 2021

Ünzelmann, M.; Bentmann, H.; Figgemeier, T.
Nature Communications, Vol. 12, Issue 1
DOI: 10.1038/s41467-021-23727-3

A light-induced phononic symmetry switch and giant dissipationless topological photocurrent in ZrTe5
journal, January 2021

Luo, Liang; Cheng, Di; Song, Boqun
Nature Materials, Vol. 20, Issue 3
DOI: 10.1038/s41563-020-00882-4

Direct observation of spin-polarized bulk bands in an inversion-symmetric semiconductor
journal, October 2014

Riley, J. M.; Mazzola, F.; Dendzik, M.
Nature Physics, Vol. 10, Issue 11
DOI: 10.1038/nphys3105

Importance of Matrix Elements in the ARPES Spectra of BISCO
journal, December 1999

Bansil, A.; Lindroos, M.
Physical Review Letters, Vol. 83, Issue 24
DOI: 10.1103/PhysRevLett.83.5154

Orbital textures and charge density waves in transition metal dichalcogenides
journal, March 2015

Ritschel, T.; Trinckauf, J.; Koepernik, K.
Nature Physics, Vol. 11, Issue 4
DOI: 10.1038/nphys3267

Angular Dependence of Photoemission and Atomic Orbitals in the Layer Compound $1 T - Ta {Se}_{2}$
journal, June 1974

Traum, Morton M.; Smith, Neville V.; Di Salvo, F. J.
Physical Review Letters, Vol. 32, Issue 22
DOI: 10.1103/PhysRevLett.32.1241

Three-Dimensional Electron Realm in ${VSe}_{2}$ by Soft-X-Ray Photoelectron Spectroscopy: Origin of Charge-Density Waves
journal, August 2012

Strocov, Vladimir N.; Shi, Ming; Kobayashi, Masaki
Physical Review Letters, Vol. 109, Issue 8
DOI: 10.1103/PhysRevLett.109.086401

Excitonic insulator emerging from semiconducting normal state in $1 T − {TiSe}_{2}$
journal, May 2021

Bok, Jin Mo; Hwang, Jungseek; Choi, Han-Yong
Physical Review B, Vol. 103, Issue 20
DOI: 10.1103/PhysRevB.103.205108

Ueber einen Einfluss des ultravioletten Lichtes auf die electrische Entladung
journal, January 1887

Hertz, H.
Annalen der Physik und Chemie, Vol. 267, Issue 8
DOI: 10.1002/andp.18872670827

The PseudoDojo: Training and grading a 85 element optimized norm-conserving pseudopotential table
journal, May 2018

van Setten, M. J.; Giantomassi, M.; Bousquet, E.
Computer Physics Communications, Vol. 226
DOI: 10.1016/j.cpc.2018.01.012

Ultrafast Switching to a Stable Hidden Quantum State in an Electronic Crystal
journal, April 2014

Stojchevska, L.; Vaskivskyi, I.; Mertelj, T.
Science, Vol. 344, Issue 6180
DOI: 10.1126/science.1241591

Quantitative electron spectroscopy of surfaces: A standard data base for electron inelastic mean free paths in solids
journal, February 1979

Seah, M. P.; Dench, W. A.
Surface and Interface Analysis, Vol. 1, Issue 1
DOI: 10.1002/sia.740010103

Orbital characters determined from Fermi surface intensity patterns using angle-resolved photoemission spectroscopy
journal, June 2012

Wang, X. -P.; Richard, P.; Huang, Y. -B.
Physical Review B, Vol. 85, Issue 21
DOI: 10.1103/PhysRevB.85.214518

Theory of the thickness dependence of the charge density wave transition in 1 T-TiTe ₂
journal, September 2020

Sky Zhou, Jianqiang; Bianco, Raffaello; Monacelli, Lorenzo
2D Materials, Vol. 7, Issue 4
DOI: 10.1088/2053-1583/abae7a

Charge-density-wave transitions in 1T-VSe ₂
journal, January 1986

Eaglesham, D. J.; Withers, R. L.; Bird, D. M.
Journal of Physics C: Solid State Physics, Vol. 19, Issue 3
DOI: 10.1088/0022-3719/19/3/006

Correlation, temperature and disorder: Recent developments in the one-step description of angle-resolved photoemission
journal, April 2018

Braun, Jürgen; Minár, Ján; Ebert, Hubert
Physics Reports, Vol. 740
DOI: 10.1016/j.physrep.2018.02.007

An ultrafast symmetry switch in a Weyl semimetal
journal, January 2019

Sie, Edbert J.; Nyby, Clara M.; Pemmaraju, C. D.
Nature, Vol. 565, Issue 7737
DOI: 10.1038/s41586-018-0809-4

Pressure-induced topological phase transitions and structural transition in 1T-TiTe ₂ single crystal
journal, January 2018

Zhang, Min; Wang, Xiangqi; Rahman, Azizur
Applied Physics Letters, Vol. 112, Issue 4
DOI: 10.1063/1.5012842

Local Berry curvature signatures in dichroic angle-resolved photoelectron spectroscopy from two-dimensional materials
journal, February 2020

Schüler, Michael; De Giovannini, Umberto; Hübener, Hannes
Science Advances, Vol. 6, Issue 9
DOI: 10.1126/sciadv.aay2730

Anomalous d-like surface resonances on Mo(110) analyzed by time-of-flight momentum microscopy
journal, December 2015

Chernov, S. V.; Medjanik, K.; Tusche, C.
Ultramicroscopy, Vol. 159
DOI: 10.1016/j.ultramic.2015.07.008

Angle-resolved photoemission studies of quantum materials
journal, May 2021

Sobota, Jonathan A.; He, Yu; Shen, Zhi-Xun
Reviews of Modern Physics, Vol. 93, Issue 2
DOI: 10.1103/RevModPhys.93.025006

Evidence for an Excitonic Insulator Phase in $1 T − {TiSe}_{2}$
journal, October 2007

Cercellier, H.; Monney, C.; Clerc, F.
Physical Review Letters, Vol. 99, Issue 14
DOI: 10.1103/PhysRevLett.99.146403

A quantitative comparison of time-of-flight momentum microscopes and hemispherical analyzers for time- and angle-resolved photoemission spectroscopy experiments
journal, December 2020

Maklar, J.; Dong, S.; Beaulieu, S.
Review of Scientific Instruments, Vol. 91, Issue 12
DOI: 10.1063/5.0024493

Angular-resolved ultraviolet photoemission spectroscopy and its application to the layer compounds Ta ${Se}_{2}$ and Ta $S_{2}$
journal, March 1975

Smith, N. V.; Traum, M. M.
Physical Review B, Vol. 11, Issue 6
DOI: 10.1103/PhysRevB.11.2087

Time- and angle-resolved photoemission spectroscopy of solids in the extreme ultraviolet at 500 kHz repetition rate
journal, February 2019

Puppin, M.; Deng, Y.; Nicholson, C. W.
Review of Scientific Instruments, Vol. 90, Issue 2
DOI: 10.1063/1.5081938

Orbital Rashba effect and its detection by circular dichroism angle-resolved photoemission spectroscopy
journal, May 2012

Park, Jin-Hong; Kim, Choong H.; Rhim, Jun-Won
Physical Review B, Vol. 85, Issue 19
DOI: 10.1103/PhysRevB.85.195401

Direct 3D mapping of the Fermi surface and Fermi velocity
journal, March 2017

Medjanik, K.; Fedchenko, O.; Chernov, S.
Nature Materials, Vol. 16, Issue 6
DOI: 10.1038/nmat4875

Ultrafast Electronic Band Gap Control in an Excitonic Insulator
journal, August 2017

Mor, Selene; Herzog, Marc; Golež, Denis
Physical Review Letters, Vol. 119, Issue 8
DOI: 10.1103/PhysRevLett.119.086401

Three-dimensional band structure of layered ${TiTe}_{2}$ : Photoemission final-state effects
journal, November 2006

Strocov, V. N.; Krasovskii, E. E.; Schattke, W.
Physical Review B, Vol. 74, Issue 19
DOI: 10.1103/PhysRevB.74.195125

Charge Instability in Single-Layer ${TiTe}_{2}$ Mediated by van der Waals Bonding to Substrates
journal, October 2020

Lin, Meng-Kai; Hlevyack, Joseph A.; Chen, Peng
Physical Review Letters, Vol. 125, Issue 17
DOI: 10.1103/PhysRevLett.125.176405

High-resolution angle-resolved photoemission investigation of the quasiparticle scattering processes in a model Fermi liquid: $1 T - {TiTe}_{2}$
journal, August 2001

Perfetti, L.; Rojas, C.; Reginelli, A.
Physical Review B, Vol. 64, Issue 11
DOI: 10.1103/PhysRevB.64.115102

Importance of many-body effects to the spectral function of $1 T ‐ {TiTe}_{2}$
journal, January 2006

Nicolay, G.; Eltner, B.; Hüfner, S.
Physical Review B, Vol. 73, Issue 4
DOI: 10.1103/PhysRevB.73.045116

${TiTe}_{2}$ : Inconsistency between transport properties and photoemission results
journal, November 1994

Allen, Philip B.; Chetty, N.
Physical Review B, Vol. 50, Issue 20
DOI: 10.1103/PhysRevB.50.14855

Revealing Hidden Orbital Pseudospin Texture with Time-Reversal Dichroism in Photoelectron Angular Distributions
journal, November 2020

Beaulieu, S.; Schusser, J.; Dong, S.
Physical Review Letters, Vol. 125, Issue 21
DOI: 10.1103/PhysRevLett.125.216404

Über einen die Erzeugung und Verwandlung des Lichtes betreffenden heuristischen Gesichtspunkt
journal, January 1905

Einstein, A.
Annalen der Physik, Vol. 322, Issue 6, p. 132-148
DOI: 10.1002/andp.19053220607

Fluctuation control of nonthermal orbital order
journal, June 2021

Grandi, Francesco; Eckstein, Martin
Physical Review B, Vol. 103, Issue 24
DOI: 10.1103/PhysRevB.103.245117

Momentum and Energy Dependence of the Anomalous High-Energy Dispersion in the Electronic Structure of High Temperature Superconductors
journal, December 2007

Inosov, D. S.; Fink, J.; Kordyuk, A. A.
Physical Review Letters, Vol. 99, Issue 23
DOI: 10.1103/PhysRevLett.99.237002

Fermi-liquid line shapes measured by angle-resolved photoemission spectroscopy on 1- T - ${TiTe}_{2}$
journal, August 1992

Claessen, R.; Anderson, R. O.; Allen, J. W.
Physical Review Letters, Vol. 69, Issue 5
DOI: 10.1103/PhysRevLett.69.808

Orbital- and $k_{z}$ -Selective Hybridization of Se $4 p$ and Ti $3 d$ States in the Charge Density Wave Phase of ${TiSe}_{2}$
journal, February 2019

Watson, Matthew D.; Clark, Oliver J.; Mazzola, Federico
Physical Review Letters, Vol. 122, Issue 7
DOI: 10.1103/PhysRevLett.122.076404

Computational framework chinook for angle-resolved photoemission spectroscopy
journal, November 2019

Day, Ryan P.; Zwartsenberg, Berend; Elfimov, Ilya S.
npj Quantum Materials, Vol. 4, Issue 1
DOI: 10.1038/s41535-019-0194-8

Polarization-Modulated Angle-Resolved Photoemission Spectroscopy: Toward Circular Dichroism without Circular Photons and Bloch Wave-function Reconstruction
journal, January 2022

Schüler, Michael; Pincelli, Tommaso; Dong, Shuo
Physical Review X, Vol. 12, Issue 1
DOI: 10.1103/PhysRevX.12.011019

Studying local Berry curvature in 2H-WSe2 by circular dichroism photoemission utilizing crystal mirror plane
journal, January 2021

Cho, Soohyun; Park, Jin-Hong; Huh, Soonsang
Scientific Reports, Vol. 11, Issue 1
DOI: 10.1038/s41598-020-79672-6

Emergence of charge density waves and a pseudogap in single-layer TiTe2
journal, September 2017

Chen, P.; Pai, Woei Wu; Chan, Y. -H.
Nature Communications, Vol. 8, Issue 1
DOI: 10.1038/s41467-017-00641-1

An open-source, end-to-end workflow for multidimensional photoemission spectroscopy
journal, December 2020

Xian, R. Patrick; Acremann, Yves; Agustsson, Steinn Y.
Scientific Data, Vol. 7, Issue 1
DOI: 10.1038/s41597-020-00769-8

Multidimensional XUV Photoemission Spectroscopy of 1T-TiTe2 for different crystal orientations
dataset, January 2021

Beaulieu, Samuel; Schüler, Michael; Schusser, Jakub
Zenodo
DOI: 10.5281/zenodo.5541489

Similar Records in DOE PAGES and OSTI.GOV collections:

Revealing Hidden Orbital Pseudospin Texture with Time-Reversal Dichroism in Photoelectron Angular Distributions

Journal Article Beaulieu, S. ; Schusser, J. ; Dong, S. ; ... - Physical Review Letters

We performed angle-resolved photoemission spectroscopy (ARPES) of bulk 2H-WSe₂ for different crystal orientations linked to each other by time-reversal symmetry. We introduce a new observable called time-reversal dichroism in photoelectron angular distributions (TRDAD), which quantifies the modulation of the photoemission intensity upon effective time-reversal operation. We demonstrate that the hidden orbital pseudospin texture leaves its imprint on TRDAD, due to multiple orbital interference effects in photoemission. Our experimental results are in quantitative agreement with both the tight-binding model and state-of-the-art fully relativistic calculations performed using the one-step model of photoemission. While spin-resolved ARPES probes the spin component of entangled spin-orbitalmore »« less
https://doi.org/10.1103/physrevlett.125.216404

Full Text Available
Polarization-Modulated Angle-Resolved Photoemission Spectroscopy: Toward Circular Dichroism without Circular Photons and Bloch Wave-function Reconstruction

Journal Article Schüler, Michael ; Pincelli, Tommaso ; Dong, Shuo ; ... - Physical Review. X

Angle-resolved photoemission spectroscopy (ARPES) is the most powerful technique to investigate the electronic band structure of crystalline solids. To completely characterize the electronic structure of topological materials, one needs to go beyond band structure mapping and access information about the momentum-resolved Bloch wave function, namely, orbitals, Berry curvature, and topological invariants. However, because phase information is lost in the process of measuring photoemission intensities, retrieving the complex-valued Bloch wave function from photoemission data has yet remained elusive. We introduce a novel measurement methodology and associated observable in extreme ultraviolet angle-resolved photoemission spectroscopy, based on continuous modulation of the ionizing radiationmore »« less
https://doi.org/10.1103/PhysRevX.12.011019
How Circular Dichroism in Time- and Angle-Resolved Photoemission Can Be Used to Spectroscopically Detect Transient Topological States in Graphene

Journal Article Schüler, Michael ; De Giovannini, Umberto ; Hübener, Hannes ; ... - Physical Review. X

Pumping graphene with circularly polarized light is the archetype of light-tailoring topological bands. Realizing the induced Floquet-Chern-insulator state and demonstrating clear experimental evidence for its topological nature has been a challenge, and it has become clear that scattering effects play a crucial role. We tackle this gap between theory and experiment by employing microscopic quantum kinetic calculations including realistic electron-electron and electron-phonon scattering. Our theory provides a direct link to the build up of the Floquet-Chern-insulator state in light-driven graphene and its detection in time- and angle-resolved photoemission spectroscopy (ARPES). This approach allows us to study the robustness of themore »« less
https://doi.org/10.1103/physrevx.10.041013
Strong correlations and orbital texture in single-layer 1T-TaSe₂

Journal Article Chen, Yi ; Ruan, Wei ; Wu, Meng ; ... - Nature Physics

© 2020, The Author(s), under exclusive licence to Springer Nature Limited. Strong electron correlation can induce Mott insulating behaviour and produce intriguing states of matter such as unconventional superconductivity and quantum spin liquids. Recent advances in van der Waals material synthesis enable the exploration of Mott systems in the two-dimensional limit. Here we report characterization of the local electronic properties of single- and few-layer 1T-TaSe2 via spatial- and momentum-resolved spectroscopy involving scanning tunnelling microscopy and angle-resolved photoemission. Our results indicate that electron correlation induces a robust Mott insulator state in single-layer 1T-TaSe2 that is accompanied by unusual orbital texture. Interlayermore »« less
Cited by 78
https://doi.org/10.1038/s41567-019-0744-9

Full Text Available
Coherent Electronic Band Structure of TiTe₂/TiSe₂ Moiré Bilayer

Journal Article Lin, Meng-Kai ; He, Tao ; Hlevyack, Joseph A. ; ... - ACS Nano

Here, a van der Waals bonded moiré bilayer formed by sequential growth of TiSe₂ and TiTe₂ monolayers exhibits emergent electronic structure as evidenced by angle-resolved photoemission band mapping. The two monolayers adopt the same lattice orientation but incommensurate lattice constants. Despite the lack of translational symmetry, sharp dispersive bands are observed. The dispersion relations appear distinct from those for the component monolayers alone. Theoretical calculations illustrate the formation of composite bands by coherent electronic coupling despite the weak interlayer bonding, which leads to band renormalization and energy shifts.
https://doi.org/10.1021/acsnano.0c10352

Full Text Available

Similar Records

Title: Unveiling the orbital texture of 1T-TiTe2 using intrinsic linear dichroism in multidimensional photoemission spectroscopy

Abstract

Citation Formats

Probing band parity inversion in the topological insulator GeBi2Te4 by linear dichroism in ARPES journal, May 2018

Symmetry-guided nonrigid registration: The case for distortion correction in multidimensional photoemission spectroscopy journal, July 2019

Photoemission spectroscopy in metals: journal, October 1999

An experimentalist's guide to the matrix element in angle resolved photoemission journal, January 2017

Profiling spin and orbital texture of a topological insulator in full momentum space journal, April 2021

Non-local dxy nematicity and the missing electron pocket in FeSe journal, May 2021

Calculating condensed matter properties using the KKR-Green's function method—recent developments and applications journal, August 2011

Complete band-structure determination of the quasi-two-dimensional Fermi-liquid reference compound TiTe 2 journal, July 1996

500 kHz OPCPA delivering tunable sub-20 fs pulses with 15 W average power based on an all-ytterbium laser journal, January 2015

Experimental Observation of Hidden Berry Curvature in Inversion-Symmetric Bulk 2 H − WSe 2 journal, October 2018

Experimental Evidence of Chiral Symmetry Breaking in Kekulé-Ordered Graphene journal, May 2021

Electronic properties and superlattice formation in the semimetal TiSe 2 journal, November 1976

ARPES study of orbital character, symmetry breaking, and pseudogaps in doped and pure Sr 2 IrO 4 journal, November 2019

Ultrafast dynamical Lifshitz transition journal, April 2021

Multidimensional XUV Photoemission Spectroscopy of 1T-TiTe2 for different crystal orientations dataset, January 2021

Determination of the Hole Lifetime from Photoemission: Ti 3 d States in TiTe 2 journal, May 2007

Charge-density wave transition of 1 T − V S e 2 studied by angle-resolved photoemission spectroscopy journal, October 2003

Multi-MHz time-of-flight electronic bandstructure imaging of graphene on Ir(111) journal, June 2016

Probing the Electronic Structure of Complex Systems by ARPES journal, January 2004

Nature of Symmetry Breaking at the Excitonic Insulator Transition: Ta 2 NiSe 5 journal, May 2020

Momentum-space signatures of Berry flux monopoles in the Weyl semimetal TaAs journal, June 2021

A light-induced phononic symmetry switch and giant dissipationless topological photocurrent in ZrTe5 journal, January 2021

Direct observation of spin-polarized bulk bands in an inversion-symmetric semiconductor journal, October 2014

Importance of Matrix Elements in the ARPES Spectra of BISCO journal, December 1999

Orbital textures and charge density waves in transition metal dichalcogenides journal, March 2015

Angular Dependence of Photoemission and Atomic Orbitals in the Layer Compound 1 T − Ta Se 2 journal, June 1974

Three-Dimensional Electron Realm in VSe 2 by Soft-X-Ray Photoelectron Spectroscopy: Origin of Charge-Density Waves journal, August 2012

Excitonic insulator emerging from semiconducting normal state in 1 T − TiSe 2 journal, May 2021

Ueber einen Einfluss des ultravioletten Lichtes auf die electrische Entladung journal, January 1887

The PseudoDojo: Training and grading a 85 element optimized norm-conserving pseudopotential table journal, May 2018

Ultrafast Switching to a Stable Hidden Quantum State in an Electronic Crystal journal, April 2014

Quantitative electron spectroscopy of surfaces: A standard data base for electron inelastic mean free paths in solids journal, February 1979

Orbital characters determined from Fermi surface intensity patterns using angle-resolved photoemission spectroscopy journal, June 2012

Theory of the thickness dependence of the charge density wave transition in 1 T-TiTe 2 journal, September 2020

Charge-density-wave transitions in 1T-VSe 2 journal, January 1986

Correlation, temperature and disorder: Recent developments in the one-step description of angle-resolved photoemission journal, April 2018

An ultrafast symmetry switch in a Weyl semimetal journal, January 2019

Pressure-induced topological phase transitions and structural transition in 1T-TiTe 2 single crystal journal, January 2018

Local Berry curvature signatures in dichroic angle-resolved photoelectron spectroscopy from two-dimensional materials journal, February 2020

Anomalous d-like surface resonances on Mo(110) analyzed by time-of-flight momentum microscopy journal, December 2015

Angle-resolved photoemission studies of quantum materials journal, May 2021

Evidence for an Excitonic Insulator Phase in 1 T − TiSe 2 journal, October 2007

A quantitative comparison of time-of-flight momentum microscopes and hemispherical analyzers for time- and angle-resolved photoemission spectroscopy experiments journal, December 2020

Angular-resolved ultraviolet photoemission spectroscopy and its application to the layer compounds Ta Se 2 and Ta S 2 journal, March 1975

Time- and angle-resolved photoemission spectroscopy of solids in the extreme ultraviolet at 500 kHz repetition rate journal, February 2019

Orbital Rashba effect and its detection by circular dichroism angle-resolved photoemission spectroscopy journal, May 2012

Direct 3D mapping of the Fermi surface and Fermi velocity journal, March 2017

Ultrafast Electronic Band Gap Control in an Excitonic Insulator journal, August 2017

Three-dimensional band structure of layered TiTe 2 : Photoemission final-state effects journal, November 2006

Charge Instability in Single-Layer TiTe 2 Mediated by van der Waals Bonding to Substrates journal, October 2020

High-resolution angle-resolved photoemission investigation of the quasiparticle scattering processes in a model Fermi liquid: 1 T − TiTe 2 journal, August 2001

Importance of many-body effects to the spectral function of 1 T ‐ TiTe 2 journal, January 2006

TiTe 2 : Inconsistency between transport properties and photoemission results journal, November 1994

Revealing Hidden Orbital Pseudospin Texture with Time-Reversal Dichroism in Photoelectron Angular Distributions journal, November 2020

Über einen die Erzeugung und Verwandlung des Lichtes betreffenden heuristischen Gesichtspunkt journal, January 1905

Fluctuation control of nonthermal orbital order journal, June 2021

Momentum and Energy Dependence of the Anomalous High-Energy Dispersion in the Electronic Structure of High Temperature Superconductors journal, December 2007

Fermi-liquid line shapes measured by angle-resolved photoemission spectroscopy on 1- T - TiTe 2 journal, August 1992

Orbital- and k z -Selective Hybridization of Se 4 p and Ti 3 d States in the Charge Density Wave Phase of TiSe 2 journal, February 2019

Computational framework chinook for angle-resolved photoemission spectroscopy journal, November 2019

Polarization-Modulated Angle-Resolved Photoemission Spectroscopy: Toward Circular Dichroism without Circular Photons and Bloch Wave-function Reconstruction journal, January 2022

Studying local Berry curvature in 2H-WSe2 by circular dichroism photoemission utilizing crystal mirror plane journal, January 2021

Emergence of charge density waves and a pseudogap in single-layer TiTe2 journal, September 2017

An open-source, end-to-end workflow for multidimensional photoemission spectroscopy journal, December 2020

Multidimensional XUV Photoemission Spectroscopy of 1T-TiTe2 for different crystal orientations dataset, January 2021

Title: Unveiling the orbital texture of 1T-TiTe₂ using intrinsic linear dichroism in multidimensional photoemission spectroscopy

Probing band parity inversion in the topological insulator GeBi2Te4 by linear dichroism in ARPES
journal, May 2018

Symmetry-guided nonrigid registration: The case for distortion correction in multidimensional photoemission spectroscopy
journal, July 2019

Photoemission spectroscopy in metals:
journal, October 1999

An experimentalist's guide to the matrix element in angle resolved photoemission
journal, January 2017

Profiling spin and orbital texture of a topological insulator in full momentum space
journal, April 2021

Non-local dxy nematicity and the missing electron pocket in FeSe
journal, May 2021

Calculating condensed matter properties using the KKR-Green's function method—recent developments and applications
journal, August 2011

Complete band-structure determination of the quasi-two-dimensional Fermi-liquid reference compound TiTe 2
journal, July 1996

500 kHz OPCPA delivering tunable sub-20 fs pulses with 15 W average power based on an all-ytterbium laser
journal, January 2015

Experimental Observation of Hidden Berry Curvature in Inversion-Symmetric Bulk $2 H − {WSe}_{2}$
journal, October 2018

Experimental Evidence of Chiral Symmetry Breaking in Kekulé-Ordered Graphene
journal, May 2021

Electronic properties and superlattice formation in the semimetal ${TiSe}_{2}$
journal, November 1976

ARPES study of orbital character, symmetry breaking, and pseudogaps in doped and pure ${Sr}_{2} {IrO}_{4}$
journal, November 2019

Ultrafast dynamical Lifshitz transition
journal, April 2021

Multidimensional XUV Photoemission Spectroscopy of 1T-TiTe2 for different crystal orientations
dataset, January 2021

Determination of the Hole Lifetime from Photoemission: Ti $3 d$ States in ${TiTe}_{2}$
journal, May 2007

Charge-density wave transition of $1 T {- V S e}_{2}$ studied by angle-resolved photoemission spectroscopy
journal, October 2003

Multi-MHz time-of-flight electronic bandstructure imaging of graphene on Ir(111)
journal, June 2016

Probing the Electronic Structure of Complex Systems by ARPES
journal, January 2004

Nature of Symmetry Breaking at the Excitonic Insulator Transition: ${Ta}_{2} {NiSe}_{5}$
journal, May 2020

Momentum-space signatures of Berry flux monopoles in the Weyl semimetal TaAs
journal, June 2021

A light-induced phononic symmetry switch and giant dissipationless topological photocurrent in ZrTe5
journal, January 2021

Direct observation of spin-polarized bulk bands in an inversion-symmetric semiconductor
journal, October 2014

Importance of Matrix Elements in the ARPES Spectra of BISCO
journal, December 1999

Orbital textures and charge density waves in transition metal dichalcogenides
journal, March 2015

Angular Dependence of Photoemission and Atomic Orbitals in the Layer Compound $1 T - Ta {Se}_{2}$
journal, June 1974

Three-Dimensional Electron Realm in ${VSe}_{2}$ by Soft-X-Ray Photoelectron Spectroscopy: Origin of Charge-Density Waves
journal, August 2012

Excitonic insulator emerging from semiconducting normal state in $1 T − {TiSe}_{2}$
journal, May 2021

Ueber einen Einfluss des ultravioletten Lichtes auf die electrische Entladung
journal, January 1887

The PseudoDojo: Training and grading a 85 element optimized norm-conserving pseudopotential table
journal, May 2018

Ultrafast Switching to a Stable Hidden Quantum State in an Electronic Crystal
journal, April 2014

Quantitative electron spectroscopy of surfaces: A standard data base for electron inelastic mean free paths in solids
journal, February 1979

Orbital characters determined from Fermi surface intensity patterns using angle-resolved photoemission spectroscopy
journal, June 2012

Theory of the thickness dependence of the charge density wave transition in 1 T-TiTe ₂
journal, September 2020

Charge-density-wave transitions in 1T-VSe ₂
journal, January 1986

Correlation, temperature and disorder: Recent developments in the one-step description of angle-resolved photoemission
journal, April 2018

An ultrafast symmetry switch in a Weyl semimetal
journal, January 2019

Pressure-induced topological phase transitions and structural transition in 1T-TiTe ₂ single crystal
journal, January 2018

Local Berry curvature signatures in dichroic angle-resolved photoelectron spectroscopy from two-dimensional materials
journal, February 2020

Anomalous d-like surface resonances on Mo(110) analyzed by time-of-flight momentum microscopy
journal, December 2015

Angle-resolved photoemission studies of quantum materials
journal, May 2021

Evidence for an Excitonic Insulator Phase in $1 T − {TiSe}_{2}$
journal, October 2007

A quantitative comparison of time-of-flight momentum microscopes and hemispherical analyzers for time- and angle-resolved photoemission spectroscopy experiments
journal, December 2020

Angular-resolved ultraviolet photoemission spectroscopy and its application to the layer compounds Ta ${Se}_{2}$ and Ta $S_{2}$
journal, March 1975

Time- and angle-resolved photoemission spectroscopy of solids in the extreme ultraviolet at 500 kHz repetition rate
journal, February 2019

Orbital Rashba effect and its detection by circular dichroism angle-resolved photoemission spectroscopy
journal, May 2012

Direct 3D mapping of the Fermi surface and Fermi velocity
journal, March 2017

Ultrafast Electronic Band Gap Control in an Excitonic Insulator
journal, August 2017

Three-dimensional band structure of layered ${TiTe}_{2}$ : Photoemission final-state effects
journal, November 2006

Charge Instability in Single-Layer ${TiTe}_{2}$ Mediated by van der Waals Bonding to Substrates
journal, October 2020

High-resolution angle-resolved photoemission investigation of the quasiparticle scattering processes in a model Fermi liquid: $1 T - {TiTe}_{2}$
journal, August 2001

Importance of many-body effects to the spectral function of $1 T ‐ {TiTe}_{2}$
journal, January 2006

${TiTe}_{2}$ : Inconsistency between transport properties and photoemission results
journal, November 1994

Revealing Hidden Orbital Pseudospin Texture with Time-Reversal Dichroism in Photoelectron Angular Distributions
journal, November 2020

Über einen die Erzeugung und Verwandlung des Lichtes betreffenden heuristischen Gesichtspunkt
journal, January 1905

Fluctuation control of nonthermal orbital order
journal, June 2021

Momentum and Energy Dependence of the Anomalous High-Energy Dispersion in the Electronic Structure of High Temperature Superconductors
journal, December 2007

Fermi-liquid line shapes measured by angle-resolved photoemission spectroscopy on 1- T - ${TiTe}_{2}$
journal, August 1992

Orbital- and $k_{z}$ -Selective Hybridization of Se $4 p$ and Ti $3 d$ States in the Charge Density Wave Phase of ${TiSe}_{2}$
journal, February 2019

Computational framework chinook for angle-resolved photoemission spectroscopy
journal, November 2019

Polarization-Modulated Angle-Resolved Photoemission Spectroscopy: Toward Circular Dichroism without Circular Photons and Bloch Wave-function Reconstruction
journal, January 2022

Studying local Berry curvature in 2H-WSe2 by circular dichroism photoemission utilizing crystal mirror plane
journal, January 2021

Emergence of charge density waves and a pseudogap in single-layer TiTe2
journal, September 2017

An open-source, end-to-end workflow for multidimensional photoemission spectroscopy
journal, December 2020

Multidimensional XUV Photoemission Spectroscopy of 1T-TiTe2 for different crystal orientations
dataset, January 2021